Decoupling of lattice and orbital degrees of freedom in an iron-pnictide superconductor

• Published in: Physical review research Vol. 3; no. 2; p. 023220
• Main Authors: Matt, C. E., Ivashko, O., Horio, M., Choi, J., Wang, Q., Sutter, D., Dennler, N., Fischer, M. H., Katrych, S., Forro, L., Ma, J., Fu, B., Lv, B. Q., Zimmermann, M. v., Kim, T. K., Plumb, N. C., Xu, N., Shi, M., Chang, J.
• Format: Journal Article
• Language: English
• Published: American Physical Society 01.06.2021
• DOI: 10.1103/PhysRevResearch.3.023220
• ISSN: 2643-1564

The interplay between structural and electronic phases in iron-based superconductors is a central theme in the search for the superconducting pairing mechanism. While electronic nematicity is competing with superconductivity, the effect of purely structural orthorhombic order is unexplored. Here, using x-ray diffraction and angle-resolved photoemission spectroscopy, we reveal a structural orthorhombic phase in the electron-doped iron-pnictide superconductor Pr_{4}Fe_{2}As_{2}Te_{0.88}O_{4} (T_{c}=25 K), which is distinct from orthorhombicity in the nematic phase in underdoped pnictides. Despite the high electron doping we find an exceptionally high orthorhombic onset temperature (T_{ort}∼250 K), no signatures of phase competition with superconductivity, and absence of electronic nematic order as the driving mechanism for orthorhombicity. Combined, our results establish a high-temperature phase in the phase diagram of iron-pnictide superconductors and impose strong constraints for the modeling of their superconducting pairing mechanism.