A double-acceptor as a superior organic dye design for p-type DSSCs: high photocurrents and the observed light soaking effect
Herein, we report three novel single donor double acceptor dyes, BH2, 4, and 6, for use in p-type dye sensitized solar cells (DSSCs). BH4 yields one of the highest photocurrents, 7.4 mA cm(-2), to date. The high performance is achieved via a shorter synthetic route and no exotic materials or cell-bu...
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| Published in | Physical chemistry chemical physics : PCCP Vol. 16; no. 47; pp. 26103 - 26111 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
21.12.2014
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| Abstract | Herein, we report three novel single donor double acceptor dyes, BH2, 4, and 6, for use in p-type dye sensitized solar cells (DSSCs). BH4 yields one of the highest photocurrents, 7.4 mA cm(-2), to date. The high performance is achieved via a shorter synthetic route and no exotic materials or cell-building techniques. We suggest a structural principle when building dyes whereby one adopts a double acceptor/single anchor when a triphenylamine moiety is incorporated into a dye for p-type DSSCs. This strategy increases the molar extinction coefficient while simultaneously reducing the number of synthetic steps. The molar extinction coefficients (99 980 M(-1) cm(-1)) reported herein are among the highest reported. Finally, we report the first-ever-observed light soaking effect in p-type DSSCs. |
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| AbstractList | Herein, we report three novel single donor double acceptor dyes, BH2, 4, and 6, for use in p-type dye sensitized solar cells (DSSCs). BH4 yields one of the highest photocurrents, 7.4 mA cm
−2
, to date. The high performance is achieved
via
a shorter synthetic route and no exotic materials or cell-building techniques. We suggest a structural principle when building dyes whereby one adopts a double acceptor/single anchor when a triphenylamine moiety is incorporated into a dye for p-type DSSCs. This strategy increases the molar extinction coefficient while simultaneously reducing the number of synthetic steps. The molar extinction coefficients (99 980 M
−1
cm
−1
) reported herein are among the highest reported. Finally, we report the first-ever-observed light soaking effect in p-type DSSCs. Herein, we report three novel single donor double acceptor dyes, BH2, 4, and 6, for use in p-type dye sensitized solar cells (DSSCs). BH4 yields one of the highest photocurrents, 7.4 mA cm super(-2), to date. The high performance is achieved viaa shorter synthetic route and no exotic materials or cell-building techniques. We suggest a structural principle when building dyes whereby one adopts a double acceptor/single anchor when a triphenylamine moiety is incorporated into a dye for p-type DSSCs. This strategy increases the molar extinction coefficient while simultaneously reducing the number of synthetic steps. The molar extinction coefficients (99 980 M super(-1) cm super(-1)) reported herein are among the highest reported. Finally, we report the first-ever-observed light soaking effect in p-type DSSCs. Herein, we report three novel single donor double acceptor dyes, BH2, 4, and 6, for use in p-type dye sensitized solar cells (DSSCs). BH4 yields one of the highest photocurrents, 7.4 mA cm(-2), to date. The high performance is achieved via a shorter synthetic route and no exotic materials or cell-building techniques. We suggest a structural principle when building dyes whereby one adopts a double acceptor/single anchor when a triphenylamine moiety is incorporated into a dye for p-type DSSCs. This strategy increases the molar extinction coefficient while simultaneously reducing the number of synthetic steps. The molar extinction coefficients (99 980 M(-1) cm(-1)) reported herein are among the highest reported. Finally, we report the first-ever-observed light soaking effect in p-type DSSCs. |
| Author | Beauchamp, Damian R Garrett, Benjamin R Huang, Zhongjie Wu, Yiying Click, Kevin A Hadad, Christopher M |
| Author_xml | – sequence: 1 givenname: Kevin A surname: Click fullname: Click, Kevin A email: wu@chemistry.ohio-state.edu organization: Department of Chemistry and Biochemistry, The Ohio State University, 100 West 18th Avenue Columbus, Ohio 43210, USA. wu@chemistry.ohio-state.edu – sequence: 2 givenname: Damian R surname: Beauchamp fullname: Beauchamp, Damian R – sequence: 3 givenname: Benjamin R surname: Garrett fullname: Garrett, Benjamin R – sequence: 4 givenname: Zhongjie surname: Huang fullname: Huang, Zhongjie – sequence: 5 givenname: Christopher M surname: Hadad fullname: Hadad, Christopher M – sequence: 6 givenname: Yiying surname: Wu fullname: Wu, Yiying |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/25360820$$D View this record in MEDLINE/PubMed |
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