Effect of CeO2 nanoparticles on dielectric properties of PVB/CeO2 polymer nanodielectrics: a positron lifetime study

To produce a polymer nanodielectric material with low dielectric constant for high speed communication network cables, polymer nanodielectrics of Polyvinyl butyral (PVB) with (0.2, 0.4, 0.6, 0.8, and 1 wt%) of CeO 2 nanoparticles are prepared. Cerium dioxide (CeO 2 ) nanoparticles were synthesized b...

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Published inJournal of materials science. Materials in electronics Vol. 33; no. 2; pp. 1063 - 1077
Main Authors Raghavendra, M., Jagadish, K., Srikantaswamy, S., Pradeep, T. M., Gnana Prakash, A. P., Ravikumar, H. B.
Format Journal Article
LanguageEnglish
Published New York Springer US 2022
Springer Nature B.V
Subjects
Cables
Cerium oxides
Characterization and Evaluation of Materials
Chemistry and Materials Science
Dielectric properties
Dipoles
Ionic mobility
Materials Science
Nanoparticles
Optical and Electronic Materials
Permittivity
Photon correlation spectroscopy
Polymers
Polystyrene resins
Polyvinyl acetal resins
Polyvinyl butyral
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Abstract To produce a polymer nanodielectric material with low dielectric constant for high speed communication network cables, polymer nanodielectrics of Polyvinyl butyral (PVB) with (0.2, 0.4, 0.6, 0.8, and 1 wt%) of CeO 2 nanoparticles are prepared. Cerium dioxide (CeO 2 ) nanoparticles were synthesized by hydrothermal technique. The average size of CeO 2 nanoparticles determined by Dynamic Light Scattering studies is 60 nm. The dependence of free volume and crystallinity on dielectric properties of PVB/CeO 2 polymer nanodielectrics is explored. The positron lifetime parameters viz., o-Ps lifetime ( τ 3 ) and free volume size ( V f ) show minimum value for 1.0 wt% of CeO 2 nanoparticles loading. The reduced free volume is attributed to the increased chemical interaction between CeO 2 nanoparticles and PVB side chain. The AC conductivity and dielectric constant of PVB/CeO 2 polymer nanodielectrics are also decreased for 1.0 wt% of CeO 2 nanoparticle loading. The reduced free volume restricts the ionic mobility of CeO 2 nanoparticles and impedes dipoles mobility.
AbstractList To produce a polymer nanodielectric material with low dielectric constant for high speed communication network cables, polymer nanodielectrics of Polyvinyl butyral (PVB) with (0.2, 0.4, 0.6, 0.8, and 1 wt%) of CeO 2 nanoparticles are prepared. Cerium dioxide (CeO 2 ) nanoparticles were synthesized by hydrothermal technique. The average size of CeO 2 nanoparticles determined by Dynamic Light Scattering studies is 60 nm. The dependence of free volume and crystallinity on dielectric properties of PVB/CeO 2 polymer nanodielectrics is explored. The positron lifetime parameters viz., o-Ps lifetime ( τ 3 ) and free volume size ( V f ) show minimum value for 1.0 wt% of CeO 2 nanoparticles loading. The reduced free volume is attributed to the increased chemical interaction between CeO 2 nanoparticles and PVB side chain. The AC conductivity and dielectric constant of PVB/CeO 2 polymer nanodielectrics are also decreased for 1.0 wt% of CeO 2 nanoparticle loading. The reduced free volume restricts the ionic mobility of CeO 2 nanoparticles and impedes dipoles mobility.
To produce a polymer nanodielectric material with low dielectric constant for high speed communication network cables, polymer nanodielectrics of Polyvinyl butyral (PVB) with (0.2, 0.4, 0.6, 0.8, and 1 wt%) of CeO2 nanoparticles are prepared. Cerium dioxide (CeO2) nanoparticles were synthesized by hydrothermal technique. The average size of CeO2 nanoparticles determined by Dynamic Light Scattering studies is 60 nm. The dependence of free volume and crystallinity on dielectric properties of PVB/CeO2 polymer nanodielectrics is explored. The positron lifetime parameters viz., o-Ps lifetime (τ3) and free volume size (Vf) show minimum value for 1.0 wt% of CeO2 nanoparticles loading. The reduced free volume is attributed to the increased chemical interaction between CeO2 nanoparticles and PVB side chain. The AC conductivity and dielectric constant of PVB/CeO2 polymer nanodielectrics are also decreased for 1.0 wt% of CeO2 nanoparticle loading. The reduced free volume restricts the ionic mobility of CeO2 nanoparticles and impedes dipoles mobility.
Author Raghavendra, M.
Srikantaswamy, S.
Jagadish, K.
Gnana Prakash, A. P.
Pradeep, T. M.
Ravikumar, H. B.
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  organization: Department of Studies in Physics, University of Mysore
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Snippet To produce a polymer nanodielectric material with low dielectric constant for high speed communication network cables, polymer nanodielectrics of Polyvinyl...
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SubjectTerms Cables
Cerium oxides
Characterization and Evaluation of Materials
Chemistry and Materials Science
Dielectric properties
Dipoles
Ionic mobility
Materials Science
Nanoparticles
Optical and Electronic Materials
Permittivity
Photon correlation spectroscopy
Polymers
Polystyrene resins
Polyvinyl acetal resins
Polyvinyl butyral
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Title Effect of CeO2 nanoparticles on dielectric properties of PVB/CeO2 polymer nanodielectrics: a positron lifetime study
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