A Li3Bi/LiF interfacial layer enabling highly stable lithium metal anode
Lithium metal anode is considered the alternative to graphite anode due to its ultra-high theoretical capacity of 3860 mAh·g −1 . However, serious Li dendrite growth and drastic electrolyte side reactions restrain the commercial application of Li metal anode. In this work, a Li 3 Bi/LiF interfacial...
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| Published in | Rare metals Vol. 42; no. 12; pp. 4081 - 4090 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Beijing
Nonferrous Metals Society of China
01.12.2023
Springer Nature B.V |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Lithium metal anode is considered the alternative to graphite anode due to its ultra-high theoretical capacity of 3860 mAh·g
−1
. However, serious Li dendrite growth and drastic electrolyte side reactions restrain the commercial application of Li metal anode. In this work, a Li
3
Bi/LiF interfacial layer is constructed on the surface of the Li metal anode by a spontaneous substitution reaction. The composite interfacial layer possesses excellent ionic conductivity, high mechanical strength, and great electrolyte wettability, which ensures fast Li-ion transfer and uniform Li deposition of the Li
3
Bi/LiF@Li anode. Impressively, the Li
3
Bi/LiF@Li symmetric cell provides a cycle life of more than 400 h with only 73 mV voltage polarization at 10 mA·cm
−2
. By pairing with commercial NCM622 cathode, the Li
3
Bi/LiF@Li full cell exhibits a long cycle at a rate of 2 C.
Graphical Abstract |
|---|---|
| AbstractList | Lithium metal anode is considered the alternative to graphite anode due to its ultra-high theoretical capacity of 3860 mAh·g
−1
. However, serious Li dendrite growth and drastic electrolyte side reactions restrain the commercial application of Li metal anode. In this work, a Li
3
Bi/LiF interfacial layer is constructed on the surface of the Li metal anode by a spontaneous substitution reaction. The composite interfacial layer possesses excellent ionic conductivity, high mechanical strength, and great electrolyte wettability, which ensures fast Li-ion transfer and uniform Li deposition of the Li
3
Bi/LiF@Li anode. Impressively, the Li
3
Bi/LiF@Li symmetric cell provides a cycle life of more than 400 h with only 73 mV voltage polarization at 10 mA·cm
−2
. By pairing with commercial NCM622 cathode, the Li
3
Bi/LiF@Li full cell exhibits a long cycle at a rate of 2 C.
Graphical Abstract Lithium metal anode is considered the alternative to graphite anode due to its ultra-high theoretical capacity of 3860 mAh·g−1. However, serious Li dendrite growth and drastic electrolyte side reactions restrain the commercial application of Li metal anode. In this work, a Li3Bi/LiF interfacial layer is constructed on the surface of the Li metal anode by a spontaneous substitution reaction. The composite interfacial layer possesses excellent ionic conductivity, high mechanical strength, and great electrolyte wettability, which ensures fast Li-ion transfer and uniform Li deposition of the Li3Bi/LiF@Li anode. Impressively, the Li3Bi/LiF@Li symmetric cell provides a cycle life of more than 400 h with only 73 mV voltage polarization at 10 mA·cm−2. By pairing with commercial NCM622 cathode, the Li3Bi/LiF@Li full cell exhibits a long cycle at a rate of 2 C. |
| Author | Chen, Peng Zou, Kang-Yu Nie, Yan-Mei Li, Ling-Jun Chen, Qiao-Yun Tan, Lei Huang, Xing |
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| ContentType | Journal Article |
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| Copyright_xml | – notice: Youke Publishing Co.,Ltd 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
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| Keywords | LiF interfacial layer High current density Li Lithium metal anode Dendrite-free Bi |
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| Snippet | Lithium metal anode is considered the alternative to graphite anode due to its ultra-high theoretical capacity of 3860 mAh·g
−1
. However, serious Li dendrite... Lithium metal anode is considered the alternative to graphite anode due to its ultra-high theoretical capacity of 3860 mAh·g−1. However, serious Li dendrite... |
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| SubjectTerms | Biomaterials Chemistry and Materials Science Electrode polarization Energy Ion currents Lithium fluoride Lithium ions Materials Engineering Materials Science Metallic Materials Nanoscale Science and Technology Original Article Physical Chemistry Substitution reactions Wettability |
| Title | A Li3Bi/LiF interfacial layer enabling highly stable lithium metal anode |
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