Polypyrrole-pen ink/polydopamine electrode for flexible all-in-one supercapacitor
Flexible supercapacitors are recently of extensive interest for flexible electronic devices. Cost and ionic diffusion efficiency between interface of electrode and electrolyte are two key factors that affect their practical application. Here, we report an effective polypyrrole-pen ink/polydopamine (...
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| Published in | Ionics Vol. 28; no. 12; pp. 5599 - 5608 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Berlin/Heidelberg
Springer Berlin Heidelberg
01.12.2022
Springer Nature B.V |
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| Abstract | Flexible supercapacitors are recently of extensive interest for flexible electronic devices. Cost and ionic diffusion efficiency between interface of electrode and electrolyte are two key factors that affect their practical application. Here, we report an effective polypyrrole-pen ink/polydopamine (PPy-ink/PDA) film electrode fabricated by in-situ polymerization method. The contribution of diffusion-dominated and surface-dominated processes in charge energy storage process of PPy-ink/PDA film electrode is discussed. Moreover, based on polyvinyl alcohol/polyethylene glycol (PVA/PEG) electrolyte, a flexible all-in-one solid supercapacitor is constructed. Due to the interfacial reaction improved by PDA, the obtained device delivers a high energy density of 12.6 µWh/cm
2
at a power density of 80 µW/cm
2
. In addition, the facile fabrication method of the electrode and low cost of commercial pen ink make it an excellent candidate for flexible electronic devices.
Graphical abstract |
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| AbstractList | Flexible supercapacitors are recently of extensive interest for flexible electronic devices. Cost and ionic diffusion efficiency between interface of electrode and electrolyte are two key factors that affect their practical application. Here, we report an effective polypyrrole-pen ink/polydopamine (PPy-ink/PDA) film electrode fabricated by in-situ polymerization method. The contribution of diffusion-dominated and surface-dominated processes in charge energy storage process of PPy-ink/PDA film electrode is discussed. Moreover, based on polyvinyl alcohol/polyethylene glycol (PVA/PEG) electrolyte, a flexible all-in-one solid supercapacitor is constructed. Due to the interfacial reaction improved by PDA, the obtained device delivers a high energy density of 12.6 µWh/cm
2
at a power density of 80 µW/cm
2
. In addition, the facile fabrication method of the electrode and low cost of commercial pen ink make it an excellent candidate for flexible electronic devices.
Graphical abstract Flexible supercapacitors are recently of extensive interest for flexible electronic devices. Cost and ionic diffusion efficiency between interface of electrode and electrolyte are two key factors that affect their practical application. Here, we report an effective polypyrrole-pen ink/polydopamine (PPy-ink/PDA) film electrode fabricated by in-situ polymerization method. The contribution of diffusion-dominated and surface-dominated processes in charge energy storage process of PPy-ink/PDA film electrode is discussed. Moreover, based on polyvinyl alcohol/polyethylene glycol (PVA/PEG) electrolyte, a flexible all-in-one solid supercapacitor is constructed. Due to the interfacial reaction improved by PDA, the obtained device delivers a high energy density of 12.6 µWh/cm2 at a power density of 80 µW/cm2. In addition, the facile fabrication method of the electrode and low cost of commercial pen ink make it an excellent candidate for flexible electronic devices. |
| Author | Zang, Yue Hu, Danni Yan, Wensheng Lin, Jun Xin, Qing |
| Author_xml | – sequence: 1 givenname: Qing surname: Xin fullname: Xin, Qing email: xinqing@hdu.edu.cn organization: Institute of Carbon Neutrality and New Energy, School of Electronics and Information, Hangzhou Dianzi University – sequence: 2 givenname: Danni surname: Hu fullname: Hu, Danni organization: Institute of Carbon Neutrality and New Energy, School of Electronics and Information, Hangzhou Dianzi University – sequence: 3 givenname: Wensheng surname: Yan fullname: Yan, Wensheng organization: Institute of Carbon Neutrality and New Energy, School of Electronics and Information, Hangzhou Dianzi University – sequence: 4 givenname: Yue surname: Zang fullname: Zang, Yue organization: Institute of Carbon Neutrality and New Energy, School of Electronics and Information, Hangzhou Dianzi University – sequence: 5 givenname: Jun surname: Lin fullname: Lin, Jun organization: Institute of Carbon Neutrality and New Energy, School of Electronics and Information, Hangzhou Dianzi University |
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| Keywords | Polydopamine film Pen ink Flexible supercapacitor |
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| SubjectTerms | Chemistry Chemistry and Materials Science Condensed Matter Physics Electrochemistry Electrodes Electronic devices Energy Storage Interface reactions Ion diffusion Optical and Electronic Materials Original Paper Polyethylene glycol Polypyrroles Polyvinyl alcohol Renewable and Green Energy Supercapacitors |
| Title | Polypyrrole-pen ink/polydopamine electrode for flexible all-in-one supercapacitor |
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