Ferroelectric polarization promoted electrocatalytic hydrogen evolution on Bi2Fe4O9 nanoplates

Unconventional ferroelectricity exhibited by Bi-based nanosheets presents potential opportunities in catalytic fields, whereas the polarization characteristic remains controversial in electrocatalysis. Herein, we report a novel ferroelectric catalyst of polarized Bi2Fe4O9 nanoplates through the coro...

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Published inScripta materialia Vol. 232; p. 115509
Main Authors Xu, Guang-Rui, Wang, Jing, Zhang, Ning, Zhang, Qiong, Dong, Zemeng, Zhang, Wen, Wu, Zexing, Xie, Cong-xia, Wang, Lei
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 15.07.2023
Subjects
Electrochemistry
Ferroelectric materials
Ferroelectric polarization
Hydrogen evolution reaction
Nanoplate
Electrochemistry
Hydrogen evolution reaction
Nanoplate
Ferroelectric materials
Ferroelectric polarization
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Abstract Unconventional ferroelectricity exhibited by Bi-based nanosheets presents potential opportunities in catalytic fields, whereas the polarization characteristic remains controversial in electrocatalysis. Herein, we report a novel ferroelectric catalyst of polarized Bi2Fe4O9 nanoplates through the corona poling method after hydrothermal and calcination processes, exhibiting super catalytic activity for water splitting controlled by ferroelectric switching and special two-dimensional (2D) structure. The ferroelectric polarization depending on high voltage greatly enhances the activity of polarized Bi2Fe4O9 nanoplates for hydrogen evolution reaction (HER) with a 98 mV positive shift of overpotential compared to the unpolarized Bi2Fe4O9 nanoplates in alkaline conditions. And after long-term stability tests, the polarized Bi2Fe4O9 nanoplates exhibit excellent durability for hydrogen production. Our results show that the effect of ferroelectric polarization of Bi2Fe4O9 nanoplates enhances the electrocatalytic hydrogen evolution, which provide a new strategy for broad the application of ferroelectric materials. The polarized Bi2Fe4O9 nanoplates boost the hydrogen evolution reaction (HER) with a 98 mV positive shift of overpotential compared to the unpolarized Bi2Fe4O9 nanoplates ascribed to the adjusted d-band center and special two-dimensional (2D) structure. [Display omitted]
AbstractList Unconventional ferroelectricity exhibited by Bi-based nanosheets presents potential opportunities in catalytic fields, whereas the polarization characteristic remains controversial in electrocatalysis. Herein, we report a novel ferroelectric catalyst of polarized Bi2Fe4O9 nanoplates through the corona poling method after hydrothermal and calcination processes, exhibiting super catalytic activity for water splitting controlled by ferroelectric switching and special two-dimensional (2D) structure. The ferroelectric polarization depending on high voltage greatly enhances the activity of polarized Bi2Fe4O9 nanoplates for hydrogen evolution reaction (HER) with a 98 mV positive shift of overpotential compared to the unpolarized Bi2Fe4O9 nanoplates in alkaline conditions. And after long-term stability tests, the polarized Bi2Fe4O9 nanoplates exhibit excellent durability for hydrogen production. Our results show that the effect of ferroelectric polarization of Bi2Fe4O9 nanoplates enhances the electrocatalytic hydrogen evolution, which provide a new strategy for broad the application of ferroelectric materials. The polarized Bi2Fe4O9 nanoplates boost the hydrogen evolution reaction (HER) with a 98 mV positive shift of overpotential compared to the unpolarized Bi2Fe4O9 nanoplates ascribed to the adjusted d-band center and special two-dimensional (2D) structure. [Display omitted]
ArticleNumber 115509
Author Zhang, Qiong
Wu, Zexing
Dong, Zemeng
Xie, Cong-xia
Wang, Lei
Xu, Guang-Rui
Wang, Jing
Zhang, Wen
Zhang, Ning
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  fullname: Zhang, Wen
  organization: Key Laboratory of Eco-chemical Engineering, Key Laboratory of Optic-electric Sensing and Analytical Chemistry of Life Science, Taishan Scholar Advantage and Characteristic Discipline Team of Eco Chemical Process and Technology, School of Materials Science and Engineering, Qingdao University of Science and Technology, Qingdao 266042, PR China
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  email: inorchemwl@126.com
  organization: Key Laboratory of Eco-chemical Engineering, Key Laboratory of Optic-electric Sensing and Analytical Chemistry of Life Science, Taishan Scholar Advantage and Characteristic Discipline Team of Eco Chemical Process and Technology, School of Materials Science and Engineering, Qingdao University of Science and Technology, Qingdao 266042, PR China
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Snippet Unconventional ferroelectricity exhibited by Bi-based nanosheets presents potential opportunities in catalytic fields, whereas the polarization characteristic...
SourceID crossref
elsevier
SourceType Aggregation Database
Publisher
StartPage 115509
SubjectTerms Electrochemistry
Ferroelectric materials
Ferroelectric polarization
Hydrogen evolution reaction
Nanoplate
Title Ferroelectric polarization promoted electrocatalytic hydrogen evolution on Bi2Fe4O9 nanoplates
URI https://dx.doi.org/10.1016/j.scriptamat.2023.115509
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