Increased residual lithium compounds guided design for green recycling of spent lithium-ion cathodes
Recycling of spent lithium-ion batteries has recently become a critical issue based on environmental concerns and a desire to reutilize resources. Among the existing recycling strategies, direct regeneration is largely encouraged from an economic and environmental perspective. However, current proce...
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| Published in | Energy & environmental science Vol. 14; no. 3; pp. 1461 - 1468 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Cambridge
Royal Society of Chemistry
23.03.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Recycling of spent lithium-ion batteries has recently become a critical issue based on environmental concerns and a desire to reutilize resources. Among the existing recycling strategies, direct regeneration is largely encouraged from an economic and environmental perspective. However, current procedures used to separate the active cathode materials from the aluminum foil have some limitations for direct regeneration because they either destroy the structure of the cathode or use too many toxic and expensive reagents. Hence, we conducted comprehensive research on the microstructural evolution of the LiNi
1−
x
−
y
Co
x
Mn
y
O
2
degraded electrode and then proposed a targeted method to recycle the spent cathode materials based on the increased residual lithium compounds. This separation process involves no other reagents but water, and toxic organic solvents, complicated processes, and waste treatments are unnecessary compared with the existing pretreatment strategies. Moreover, the separated cathodes are suitable for direct regeneration. Satisfactory capacity recovery of the cathode was achieved
via
simple sintering. Such a recycling process enables a sustainable closed-loop for the spent cathodes and provides new inspiration for the design of LIB recycling.
Based on the increased residual lithium compounds of the degraded cathode, a green water-based strategy is designed for achieving closed-loop recycling of spent lithium-ion batteries. |
|---|---|
| AbstractList | Recycling of spent lithium-ion batteries has recently become a critical issue based on environmental concerns and a desire to reutilize resources. Among the existing recycling strategies, direct regeneration is largely encouraged from an economic and environmental perspective. However, current procedures used to separate the active cathode materials from the aluminum foil have some limitations for direct regeneration because they either destroy the structure of the cathode or use too many toxic and expensive reagents. Hence, we conducted comprehensive research on the microstructural evolution of the LiNi1−x−yCoxMnyO2 degraded electrode and then proposed a targeted method to recycle the spent cathode materials based on the increased residual lithium compounds. This separation process involves no other reagents but water, and toxic organic solvents, complicated processes, and waste treatments are unnecessary compared with the existing pretreatment strategies. Moreover, the separated cathodes are suitable for direct regeneration. Satisfactory capacity recovery of the cathode was achieved via simple sintering. Such a recycling process enables a sustainable closed-loop for the spent cathodes and provides new inspiration for the design of LIB recycling. Recycling of spent lithium-ion batteries has recently become a critical issue based on environmental concerns and a desire to reutilize resources. Among the existing recycling strategies, direct regeneration is largely encouraged from an economic and environmental perspective. However, current procedures used to separate the active cathode materials from the aluminum foil have some limitations for direct regeneration because they either destroy the structure of the cathode or use too many toxic and expensive reagents. Hence, we conducted comprehensive research on the microstructural evolution of the LiNi 1− x − y Co x Mn y O 2 degraded electrode and then proposed a targeted method to recycle the spent cathode materials based on the increased residual lithium compounds. This separation process involves no other reagents but water, and toxic organic solvents, complicated processes, and waste treatments are unnecessary compared with the existing pretreatment strategies. Moreover, the separated cathodes are suitable for direct regeneration. Satisfactory capacity recovery of the cathode was achieved via simple sintering. Such a recycling process enables a sustainable closed-loop for the spent cathodes and provides new inspiration for the design of LIB recycling. Based on the increased residual lithium compounds of the degraded cathode, a green water-based strategy is designed for achieving closed-loop recycling of spent lithium-ion batteries. Recycling of spent lithium-ion batteries has recently become a critical issue based on environmental concerns and a desire to reutilize resources. Among the existing recycling strategies, direct regeneration is largely encouraged from an economic and environmental perspective. However, current procedures used to separate the active cathode materials from the aluminum foil have some limitations for direct regeneration because they either destroy the structure of the cathode or use too many toxic and expensive reagents. Hence, we conducted comprehensive research on the microstructural evolution of the LiNi 1−x−y Co x Mn y O 2 degraded electrode and then proposed a targeted method to recycle the spent cathode materials based on the increased residual lithium compounds. This separation process involves no other reagents but water, and toxic organic solvents, complicated processes, and waste treatments are unnecessary compared with the existing pretreatment strategies. Moreover, the separated cathodes are suitable for direct regeneration. Satisfactory capacity recovery of the cathode was achieved via simple sintering. Such a recycling process enables a sustainable closed-loop for the spent cathodes and provides new inspiration for the design of LIB recycling. |
| Author | Chang, Xin Guo, Yu-Jie Fan, Min Meng, Qinghai Wan, Li-Jun Yang, Xinan Chen, Wan-Ping Yin, Ya-Xia Guo, Yu-Guo |
| AuthorAffiliation | Beijing National Laboratory for Condensed Matter Physics Chinese Academy of Sciences Institute of Chemistry Chinese Academy of Sciences (CAS) School of Chemical Sciences Institute of Physics CAS Research/Education Center for Excellence in Molecular Sciences CAS Key Laboratory of Molecular Nanostructure and Nanotechnology Beijing National Laboratory for Molecular Sciences (BNLMS) University of Chinese Academy of Sciences |
| AuthorAffiliation_xml | – name: Institute of Chemistry – name: CAS Key Laboratory of Molecular Nanostructure and Nanotechnology – name: Beijing National Laboratory for Molecular Sciences (BNLMS) – name: Chinese Academy of Sciences – name: Chinese Academy of Sciences (CAS) – name: School of Chemical Sciences – name: University of Chinese Academy of Sciences – name: CAS Research/Education Center for Excellence in Molecular Sciences – name: Beijing National Laboratory for Condensed Matter Physics – name: Institute of Physics |
| Author_xml | – sequence: 1 givenname: Min surname: Fan fullname: Fan, Min – sequence: 2 givenname: Xin surname: Chang fullname: Chang, Xin – sequence: 3 givenname: Yu-Jie surname: Guo fullname: Guo, Yu-Jie – sequence: 4 givenname: Wan-Ping surname: Chen fullname: Chen, Wan-Ping – sequence: 5 givenname: Ya-Xia surname: Yin fullname: Yin, Ya-Xia – sequence: 6 givenname: Xinan surname: Yang fullname: Yang, Xinan – sequence: 7 givenname: Qinghai surname: Meng fullname: Meng, Qinghai – sequence: 8 givenname: Li-Jun surname: Wan fullname: Wan, Li-Jun – sequence: 9 givenname: Yu-Guo surname: Guo fullname: Guo, Yu-Guo |
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| SubjectTerms | Aluminum Cathodes Design for recycling Electrode materials Lithium Lithium compounds Lithium-ion batteries Metal foils Organic solvents Pretreatment Reagents Rechargeable batteries Recycling Regeneration Waste treatment |
| Title | Increased residual lithium compounds guided design for green recycling of spent lithium-ion cathodes |
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