Molten-salt growth of Bi5FeTi3O15-based composite to dramatically boost photocatalytic performance
[Display omitted] •Bi5FeTi3O15-based composite were successfully synthesized via a molten-salt growth path.•The BFTO-M exhibited dramatically enhanced photocatalytic activity relative to BFTO-H and BFTO-S.•The photocatalytic mechanism for BFTO-M system was elucidated. Bi5FeTi3O15-based composite was...
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| Published in | Journal of photochemistry and photobiology. A, Chemistry. Vol. 415; p. 113306 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
15.06.2021
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| Subjects | |
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| Abstract | [Display omitted]
•Bi5FeTi3O15-based composite were successfully synthesized via a molten-salt growth path.•The BFTO-M exhibited dramatically enhanced photocatalytic activity relative to BFTO-H and BFTO-S.•The photocatalytic mechanism for BFTO-M system was elucidated.
Bi5FeTi3O15-based composite was successfully synthesized via a molten-salt growth path, and the Bi5FeTi3O15-based composite synthesized by molten salt method (BFTO-M) was involved in photocatalytic system for the first time. For comparison, the Bi5FeTi3O15 samples synthesized by hydrothermal process and solid state reaction method (BFTO-H and BFTO-S) were prepared. The BFTO-M exhibited a typical morphology of nanosheets, and possessed higher carrier separation efficiency relative to BFTO-H and BFTO-S. XRD results indicated that the as-obtained BFTO-M sample was a composite composed of BiOCl, Bi5FeTi3O15 and Bi2O2.75. RhB could hardly be degraded in BFTO-H or BFTO-S reaction system, while RhB was dramatically degraded in BFTO-M reaction system with the degradation efficiency of 95.8 %. A possible visible-light driven catalytic mechanism was exposed. |
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| AbstractList | [Display omitted]
•Bi5FeTi3O15-based composite were successfully synthesized via a molten-salt growth path.•The BFTO-M exhibited dramatically enhanced photocatalytic activity relative to BFTO-H and BFTO-S.•The photocatalytic mechanism for BFTO-M system was elucidated.
Bi5FeTi3O15-based composite was successfully synthesized via a molten-salt growth path, and the Bi5FeTi3O15-based composite synthesized by molten salt method (BFTO-M) was involved in photocatalytic system for the first time. For comparison, the Bi5FeTi3O15 samples synthesized by hydrothermal process and solid state reaction method (BFTO-H and BFTO-S) were prepared. The BFTO-M exhibited a typical morphology of nanosheets, and possessed higher carrier separation efficiency relative to BFTO-H and BFTO-S. XRD results indicated that the as-obtained BFTO-M sample was a composite composed of BiOCl, Bi5FeTi3O15 and Bi2O2.75. RhB could hardly be degraded in BFTO-H or BFTO-S reaction system, while RhB was dramatically degraded in BFTO-M reaction system with the degradation efficiency of 95.8 %. A possible visible-light driven catalytic mechanism was exposed. |
| ArticleNumber | 113306 |
| Author | Liu, Yutang Shao, Luhua Yang, Zhenfei Xia, Xinnian Li, Sijian |
| Author_xml | – sequence: 1 givenname: Luhua surname: Shao fullname: Shao, Luhua organization: College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, PR China – sequence: 2 givenname: Zhenfei surname: Yang fullname: Yang, Zhenfei organization: College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, PR China – sequence: 3 givenname: Sijian surname: Li fullname: Li, Sijian organization: College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, PR China – sequence: 4 givenname: Xinnian surname: Xia fullname: Xia, Xinnian email: xnxia@hnu.edu.cn organization: College of Chemistry and Chemical Engineering, Hunan University, Changsha, 410082, PR China – sequence: 5 givenname: Yutang surname: Liu fullname: Liu, Yutang organization: College of Environmental Science and Engineering, Hunan University, Changsha, 410082, PR China |
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| Cites_doi | 10.1016/j.jallcom.2018.10.229 10.1002/adma.201903491 10.1016/j.seppur.2020.117328 10.1016/j.jhazmat.2020.123236 10.1016/j.cej.2020.125807 10.1016/j.jcis.2018.09.054 10.1021/acssuschemeng.9b01516 10.1016/j.apcatb.2020.119403 10.1007/s10854-015-4044-6 10.1016/j.cej.2020.127028 10.1016/j.seppur.2020.117444 10.1016/j.apcatb.2017.06.012 10.1016/j.apsusc.2019.143895 10.1016/j.jmst.2020.03.039 10.1016/j.jphotochem.2019.111972 10.1016/j.nanoen.2018.05.001 10.1039/C9TA13724F 10.1039/C7TA06618J 10.1021/am505767c 10.1016/j.ceramint.2019.06.154 10.1016/j.ceramint.2017.06.103 10.1039/C9CY02513H 10.1016/j.apcatb.2019.04.044 10.1016/j.envres.2021.111056 10.1016/j.apcatb.2020.119401 10.1002/adma.201907702 10.1016/j.ceramint.2018.09.144 10.1021/acsami.9b05074 10.1021/jp807379c 10.1016/j.apcatb.2020.119377 |
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| Keywords | Perovskite Molten-salt growth Bi5FeTi3O15 Photocatalysis |
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•Bi5FeTi3O15-based composite were successfully synthesized via a molten-salt growth path.•The BFTO-M exhibited dramatically enhanced... |
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| SubjectTerms | Bi5FeTi3O15 Molten-salt growth Perovskite Photocatalysis |
| Title | Molten-salt growth of Bi5FeTi3O15-based composite to dramatically boost photocatalytic performance |
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