Working Principles of Lithium Metal Anode in Pouch Cells

Lithium metal battery has been considered as one of the potential candidates for next‐generation energy storage systems. However, the dendrite growth issue in Li anodes results in low practical energy density, short lifespan, and poor safety performance. The strategies in suppressing Li dendrite gro...

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Published inAdvanced energy materials Vol. 12; no. 47
Main Authors Liu, He, Sun, Xin, Cheng, Xin‐Bing, Guo, Cong, Yu, Feng, Bao, Weizhai, Wang, Tao, Li, Jingfa, Zhang, Qiang
Format Journal Article
LanguageEnglish
Published Weinheim Wiley Subscription Services, Inc 01.12.2022
Subjects
Anodes
dendrites
Dendritic structure
Electrochemical analysis
Energy storage
Failure mechanisms
Life span
Lithium batteries
lithium metal anodes
pouch cells
pressure
solid electrolyte interphase
Storage systems
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Abstract Lithium metal battery has been considered as one of the potential candidates for next‐generation energy storage systems. However, the dendrite growth issue in Li anodes results in low practical energy density, short lifespan, and poor safety performance. The strategies in suppressing Li dendrite growth are mostly conducted in materials‐level coin cells, while their validity in device‐level pouch cells is still under debate. It is imperative to address dendrite issues in pouch cells to realize the practical application of Li metal batteries. This review presents a comprehensive overview of the failure mechanism and regulation strategies of Li metal anodes in practical pouch cells. First, the gaps between the scientific findings in materials‐level coin cells and device‐level pouch cells are underscored. Specific attention is paid to the mechanistic understanding and quantitative discussion on the failure mechanisms of pouch‐type Li metal batteries. Subsequently, recently proposed strategies are reviewed to suppress dendrite growth in pouch cells. The state‐of‐the‐art electrochemical performance of pouch cells, especially the cell‐level energy density and lifespan, is critically concerned. The review concludes with an attempt to summarize the scientific and engineering understandings of pouch‐type Li metal anodes and propose some novel insights for the practical applications of Li metal batteries. This review presents a comprehensive overview of the gaps between the materials‐level coin cells and device‐level pouch cells, mechanistic understanding and quantitative discussion for failure mechanisms of pouch‐type Li metal anodes, and the recently proposed strategies to suppress dendrite growth in pouch cells.
AbstractList Lithium metal battery has been considered as one of the potential candidates for next‐generation energy storage systems. However, the dendrite growth issue in Li anodes results in low practical energy density, short lifespan, and poor safety performance. The strategies in suppressing Li dendrite growth are mostly conducted in materials‐level coin cells, while their validity in device‐level pouch cells is still under debate. It is imperative to address dendrite issues in pouch cells to realize the practical application of Li metal batteries. This review presents a comprehensive overview of the failure mechanism and regulation strategies of Li metal anodes in practical pouch cells. First, the gaps between the scientific findings in materials‐level coin cells and device‐level pouch cells are underscored. Specific attention is paid to the mechanistic understanding and quantitative discussion on the failure mechanisms of pouch‐type Li metal batteries. Subsequently, recently proposed strategies are reviewed to suppress dendrite growth in pouch cells. The state‐of‐the‐art electrochemical performance of pouch cells, especially the cell‐level energy density and lifespan, is critically concerned. The review concludes with an attempt to summarize the scientific and engineering understandings of pouch‐type Li metal anodes and propose some novel insights for the practical applications of Li metal batteries.
Lithium metal battery has been considered as one of the potential candidates for next‐generation energy storage systems. However, the dendrite growth issue in Li anodes results in low practical energy density, short lifespan, and poor safety performance. The strategies in suppressing Li dendrite growth are mostly conducted in materials‐level coin cells, while their validity in device‐level pouch cells is still under debate. It is imperative to address dendrite issues in pouch cells to realize the practical application of Li metal batteries. This review presents a comprehensive overview of the failure mechanism and regulation strategies of Li metal anodes in practical pouch cells. First, the gaps between the scientific findings in materials‐level coin cells and device‐level pouch cells are underscored. Specific attention is paid to the mechanistic understanding and quantitative discussion on the failure mechanisms of pouch‐type Li metal batteries. Subsequently, recently proposed strategies are reviewed to suppress dendrite growth in pouch cells. The state‐of‐the‐art electrochemical performance of pouch cells, especially the cell‐level energy density and lifespan, is critically concerned. The review concludes with an attempt to summarize the scientific and engineering understandings of pouch‐type Li metal anodes and propose some novel insights for the practical applications of Li metal batteries. This review presents a comprehensive overview of the gaps between the materials‐level coin cells and device‐level pouch cells, mechanistic understanding and quantitative discussion for failure mechanisms of pouch‐type Li metal anodes, and the recently proposed strategies to suppress dendrite growth in pouch cells.
Author Bao, Weizhai
Liu, He
Yu, Feng
Sun, Xin
Zhang, Qiang
Li, Jingfa
Cheng, Xin‐Bing
Guo, Cong
Wang, Tao
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  organization: Tsinghua University
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2021; 2021
2022; 169
2019; 7
2019; 9
2019; 4
2019; 3
2019; 31
2022; 93
2019; 2
2019; 37
2020; 39
2020; 33
2021; 143
2020; 32
2021; 57
2016; 1
2021; 56
2015; 60
2020; 30
2022; 4
2022; 5
2022; 7
2019; 45
2022; 8
2022; 9
2018; 115
2017; 56
2022; 12
2022; 13
2020; 26
2022; 14
2022; 15
2022; 96
2022; 10
2022; 1
2021; 496
2022; 2
2021; 60
2018; 10
2016; 9
2022; 17
2022; 18
2018; 13
2019; 572
2017; 6
2021; 24
2017; 8
2021; 21
2021; 20
2022; 72
2020; 120
2022; 69
2020; 59
2022; 66
2020; 8
2020; 7
2020; 6
2020; 5
2020; 4
2021; 31
2020; 3
2021; 33
2020; 53
2020; 49
2020; 48
2021; 40
2021; 9
2021; 8
2021; 7
2021; 6
2015; 6
2015; 5
2021; 509
2021; 4
2018; 140
2019; MA2019‐01
2022; 45
2022; 48
2022; 41
2020; 463
2020; 77
2021; 1
2022; 49
2021; 14
2022; 144
2021; 13
2021; 16
2021; 11
2022; 61
2021; 17
2009; 8
2013; 135
2020; 475
2018; 50
2018; 57
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Snippet Lithium metal battery has been considered as one of the potential candidates for next‐generation energy storage systems. However, the dendrite growth issue in...
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SubjectTerms Anodes
dendrites
Dendritic structure
Electrochemical analysis
Energy storage
Failure mechanisms
Life span
Lithium batteries
lithium metal anodes
pouch cells
pressure
solid electrolyte interphase
Storage systems
Title Working Principles of Lithium Metal Anode in Pouch Cells
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Faenm.202202518
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Volume 12
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