2D Nanomaterial Supported Single‐Metal Atoms for Heterogeneous Photo/Electrocatalysis

Single‐atom catalysts (SACs) attract intensive attention owing to their unmatched catalytic activities and high atom utilization. Besides metal species themselves, the substrates play a key role for the improvement of their catalytic performance by optimizing metal–support interactions and coordinat...

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Published inAdvanced functional materials Vol. 33; no. 5
Main Authors Yan, Cheng, Liu, Yi‐Lin, Zeng, Qingyi, Wang, Gui‐Gen, Han, Jie‐Cai
Format Journal Article
LanguageEnglish
Published Hoboken Wiley Subscription Services, Inc 01.01.2023
Subjects
2D nanomaterials
Carbon dioxide
Chemical reduction
electrocatalyses
Electrocatalysis
Energy conversion
Energy technology
Hydrogen evolution reactions
Materials science
Nanomaterials
operando characterizations
Oxygen evolution reactions
Oxygen reduction reactions
photocatalyses
Reaction mechanisms
single‐atom catalysts
Substrates
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Abstract Single‐atom catalysts (SACs) attract intensive attention owing to their unmatched catalytic activities and high atom utilization. Besides metal species themselves, the substrates play a key role for the improvement of their catalytic performance by optimizing metal–support interactions and coordination structures. In the past years, various 2D nanomaterials have been employed to anchor single metal atoms for renewable energy technologies and other important industrial processes. Tremendous progress has been achieved in the development of 2D supported SACs for advanced energy conversion reactions. This article provides a comprehensive and critical review of up‐to‐date advances in the field of 2D supported SACs. The state‐of‐the‐art characterizations including ex/in situ microscopic and spectroscopic techniques are summarized with the emphasis on their specific superiorities in identifying the reactive sites and reaction mechanisms, combined with theoretical calculations and experimental results. A brief overview of various reactions including hydrogen evolution reaction (HER), oxygen evolution reaction (OER), two‐electron oxygen reduction reaction (2e‐ORR), carbon dioxide reduction (CO2RR), and nitrogen reduction reaction (NRR) under the framework of electrocatalysis and photocatalysis, is presented on basis of versatile 2D nanomaterial supports. Last, the key challenges and opportunities in this rising field are highlighted. This review article presents advances in 2D nanomaterial supported single metal atom catalysts (SACs) toward photo/electrocatalysis, with the special emphasis on the superiorities of 2D nanosheets as host materials. Advanced ex/in situ microscopic and spectroscopic approaches as well as rational design strategies of 2D‐SACs, are comprehensively summarized. The future challenges and opportunities on the 2D nanosheets‐supported SACs for photo/electrocatalysis are highlighted.
AbstractList Single‐atom catalysts (SACs) attract intensive attention owing to their unmatched catalytic activities and high atom utilization. Besides metal species themselves, the substrates play a key role for the improvement of their catalytic performance by optimizing metal–support interactions and coordination structures. In the past years, various 2D nanomaterials have been employed to anchor single metal atoms for renewable energy technologies and other important industrial processes. Tremendous progress has been achieved in the development of 2D supported SACs for advanced energy conversion reactions. This article provides a comprehensive and critical review of up‐to‐date advances in the field of 2D supported SACs. The state‐of‐the‐art characterizations including ex/in situ microscopic and spectroscopic techniques are summarized with the emphasis on their specific superiorities in identifying the reactive sites and reaction mechanisms, combined with theoretical calculations and experimental results. A brief overview of various reactions including hydrogen evolution reaction (HER), oxygen evolution reaction (OER), two‐electron oxygen reduction reaction (2e‐ORR), carbon dioxide reduction (CO2RR), and nitrogen reduction reaction (NRR) under the framework of electrocatalysis and photocatalysis, is presented on basis of versatile 2D nanomaterial supports. Last, the key challenges and opportunities in this rising field are highlighted.
Single‐atom catalysts (SACs) attract intensive attention owing to their unmatched catalytic activities and high atom utilization. Besides metal species themselves, the substrates play a key role for the improvement of their catalytic performance by optimizing metal–support interactions and coordination structures. In the past years, various 2D nanomaterials have been employed to anchor single metal atoms for renewable energy technologies and other important industrial processes. Tremendous progress has been achieved in the development of 2D supported SACs for advanced energy conversion reactions. This article provides a comprehensive and critical review of up‐to‐date advances in the field of 2D supported SACs. The state‐of‐the‐art characterizations including ex/in situ microscopic and spectroscopic techniques are summarized with the emphasis on their specific superiorities in identifying the reactive sites and reaction mechanisms, combined with theoretical calculations and experimental results. A brief overview of various reactions including hydrogen evolution reaction (HER), oxygen evolution reaction (OER), two‐electron oxygen reduction reaction (2e‐ORR), carbon dioxide reduction (CO2RR), and nitrogen reduction reaction (NRR) under the framework of electrocatalysis and photocatalysis, is presented on basis of versatile 2D nanomaterial supports. Last, the key challenges and opportunities in this rising field are highlighted. This review article presents advances in 2D nanomaterial supported single metal atom catalysts (SACs) toward photo/electrocatalysis, with the special emphasis on the superiorities of 2D nanosheets as host materials. Advanced ex/in situ microscopic and spectroscopic approaches as well as rational design strategies of 2D‐SACs, are comprehensively summarized. The future challenges and opportunities on the 2D nanosheets‐supported SACs for photo/electrocatalysis are highlighted.
Single‐atom catalysts (SACs) attract intensive attention owing to their unmatched catalytic activities and high atom utilization. Besides metal species themselves, the substrates play a key role for the improvement of their catalytic performance by optimizing metal–support interactions and coordination structures. In the past years, various 2D nanomaterials have been employed to anchor single metal atoms for renewable energy technologies and other important industrial processes. Tremendous progress has been achieved in the development of 2D supported SACs for advanced energy conversion reactions. This article provides a comprehensive and critical review of up‐to‐date advances in the field of 2D supported SACs. The state‐of‐the‐art characterizations including ex/in situ microscopic and spectroscopic techniques are summarized with the emphasis on their specific superiorities in identifying the reactive sites and reaction mechanisms, combined with theoretical calculations and experimental results. A brief overview of various reactions including hydrogen evolution reaction (HER), oxygen evolution reaction (OER), two‐electron oxygen reduction reaction (2e‐ORR), carbon dioxide reduction (CO 2 RR), and nitrogen reduction reaction (NRR) under the framework of electrocatalysis and photocatalysis, is presented on basis of versatile 2D nanomaterial supports. Last, the key challenges and opportunities in this rising field are highlighted.
Author Yan, Cheng
Wang, Gui‐Gen
Han, Jie‐Cai
Liu, Yi‐Lin
Zeng, Qingyi
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  fullname: Zeng, Qingyi
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  givenname: Gui‐Gen
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  organization: Harbin Institute of Technology (Shenzhen)
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  givenname: Jie‐Cai
  surname: Han
  fullname: Han, Jie‐Cai
  organization: Harbin Institute of Technology
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Snippet Single‐atom catalysts (SACs) attract intensive attention owing to their unmatched catalytic activities and high atom utilization. Besides metal species...
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SubjectTerms 2D nanomaterials
Carbon dioxide
Chemical reduction
electrocatalyses
Electrocatalysis
Energy conversion
Energy technology
Hydrogen evolution reactions
Materials science
Nanomaterials
operando characterizations
Oxygen evolution reactions
Oxygen reduction reactions
photocatalyses
Reaction mechanisms
single‐atom catalysts
Substrates
Title 2D Nanomaterial Supported Single‐Metal Atoms for Heterogeneous Photo/Electrocatalysis
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadfm.202210837
https://www.proquest.com/docview/2769882395
Volume 33
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