Direct Synthesis of Indolines via Cyclization of Tertiary Aryl Amines with Iodonium Ylides under Sole Visible Light Irradiation
Herein we reported a direct synthesis series of indolines through cyclization of tertiary aryl amines with iodonium ylides. This cyclization reaction occurred under sole visible‐light irradiation at room temperature without the addition of any photocatalysts and additives. Preliminary mechanism stud...
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| Published in | Advanced synthesis & catalysis Vol. 365; no. 1; pp. 110 - 115 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
WEINHEIM
Wiley
10.01.2023
Wiley Subscription Services, Inc |
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| Abstract | Herein we reported a direct synthesis series of indolines through cyclization of tertiary aryl amines with iodonium ylides. This cyclization reaction occurred under sole visible‐light irradiation at room temperature without the addition of any photocatalysts and additives. Preliminary mechanism studies revealed that an electron donor‐acceptor (EDA) complex between iodonium ylides and tertiary aryl amines should be formed during the reaction. |
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| AbstractList | Herein we reported a direct synthesis series of indolines through cyclization of tertiary aryl amines with iodonium ylides. This cyclization reaction occurred under sole visible‐light irradiation at room temperature without the addition of any photocatalysts and additives. Preliminary mechanism studies revealed that an electron donor‐acceptor (EDA) complex between iodonium ylides and tertiary aryl amines should be formed during the reaction. Herein we reported a direct synthesis series of indolines through cyclization of tertiary aryl amines with iodonium ylides. This cyclization reaction occurred under sole visible‐light irradiation at room temperature without the addition of any photocatalysts and additives. Preliminary mechanism studies revealed that an electron donor‐acceptor (EDA) complex between iodonium ylides and tertiary aryl amines should be formed during the reaction. magnified image |
| Author | Xuan, Jun Li, Lei Zhao, Yan‐Rui |
| Author_xml | – sequence: 1 givenname: Yan‐Rui surname: Zhao fullname: Zhao, Yan‐Rui organization: Anhui University – sequence: 2 givenname: Lei surname: Li fullname: Li, Lei email: llee2005@163.com organization: Anhui University – sequence: 3 givenname: Jun orcidid: 0000-0003-0578-9330 surname: Xuan fullname: Xuan, Jun email: xuanjun@ahu.edu.cn organization: Anhui University) |
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| CitedBy_id | crossref_primary_10_1002_ejoc_202300713 crossref_primary_10_1002_ejoc_202401438 crossref_primary_10_1021_acs_orglett_3c02009 crossref_primary_10_1039_D3QO00039G crossref_primary_10_1039_D4CC02046D crossref_primary_10_3762_bjoc_19_86 crossref_primary_10_6023_cjoc202406050 crossref_primary_10_1021_acs_joc_3c00380 crossref_primary_10_1021_acs_chemrev_4c00303 crossref_primary_10_1002_chem_202404442 |
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| Keywords | EDA complex Iodonium ylides CYCLOPROPANATION Visible light TRANSYLIDATION CATALYST Indolines Photochemistry ALKALOIDS |
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| Snippet | Herein we reported a direct synthesis series of indolines through cyclization of tertiary aryl amines with iodonium ylides. This cyclization reaction occurred... |
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| SubjectTerms | Additives Amines Aromatic compounds Chemistry Chemistry, Applied Chemistry, Organic EDA complex Heterocyclic compounds Indolines Iodonium ylides Light irradiation Photochemistry Physical Sciences Room temperature Science & Technology Synthesis Visible light |
| Title | Direct Synthesis of Indolines via Cyclization of Tertiary Aryl Amines with Iodonium Ylides under Sole Visible Light Irradiation |
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