Cyano‐Functionalized Graphitic Carbon Nitride with Adsorption and Photoreduction Isosite Achieving Efficient Uranium Extraction from Seawater
Photocatalytic uranium extraction from seawater is an ideal strategy to obtain uranium resources. Herein, the cyano‐functionalized graphitic carbon nitride (g‐C3N4‐CN) with an isosite structure of adsorption and photoreduction for U(VI) is successfully prepared to achieve efficient photocatalytic ur...
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| Published in | Advanced functional materials Vol. 34; no. 19 |
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| Main Authors | , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
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01.05.2024
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| Abstract | Photocatalytic uranium extraction from seawater is an ideal strategy to obtain uranium resources. Herein, the cyano‐functionalized graphitic carbon nitride (g‐C3N4‐CN) with an isosite structure of adsorption and photoreduction for U(VI) is successfully prepared to achieve efficient photocatalytic uranium extraction from seawater. As the key of the isosite structure, the cyano group not only dramatically promotes the separation of photogenerated charges of g‐C3N4‐CN and enriched electrons around it, but also greatly improves the adsorption capacity and selectivity for U(VI) over g‐C3N4‐CN by complexing with U(VI). Therefore, g‐C3N4‐CN exhibits efficient and stable photocatalytic U(VI) reduction performance, with a saturated uranium extraction capacity of 2644.3 mg g−1, significantly higher than most reported g‐C3N4‐based photocatalysts. Moreover, it also performs well in solar light‐driven uranium extraction from actual seawater. Briefly, this work illustrates the importance of constructing the isosite structure of adsorption and photoreduction for U(VI) in improving the photocatalytic uranium extraction performance.
The cyano‐functionalized graphitic carbon nitride with an isosite structure of adsorption and photoreduction for U(VI) is successfully prepared, which achieves efficient and stable photocatalytic U(VI) reduction performance, with a saturated uranium extraction capacity of 2644.3 mg g−1, significantly higher than most reported g‐C3N4‐based photocatalysts. Moreover, it also performs well in solar light‐driven uranium extraction from actual seawater. |
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| AbstractList | Photocatalytic uranium extraction from seawater is an ideal strategy to obtain uranium resources. Herein, the cyano‐functionalized graphitic carbon nitride (g‐C3N4‐CN) with an isosite structure of adsorption and photoreduction for U(VI) is successfully prepared to achieve efficient photocatalytic uranium extraction from seawater. As the key of the isosite structure, the cyano group not only dramatically promotes the separation of photogenerated charges of g‐C3N4‐CN and enriched electrons around it, but also greatly improves the adsorption capacity and selectivity for U(VI) over g‐C3N4‐CN by complexing with U(VI). Therefore, g‐C3N4‐CN exhibits efficient and stable photocatalytic U(VI) reduction performance, with a saturated uranium extraction capacity of 2644.3 mg g−1, significantly higher than most reported g‐C3N4‐based photocatalysts. Moreover, it also performs well in solar light‐driven uranium extraction from actual seawater. Briefly, this work illustrates the importance of constructing the isosite structure of adsorption and photoreduction for U(VI) in improving the photocatalytic uranium extraction performance. Abstract Photocatalytic uranium extraction from seawater is an ideal strategy to obtain uranium resources. Herein, the cyano‐functionalized graphitic carbon nitride (g‐C 3 N 4 ‐CN) with an isosite structure of adsorption and photoreduction for U(VI) is successfully prepared to achieve efficient photocatalytic uranium extraction from seawater. As the key of the isosite structure, the cyano group not only dramatically promotes the separation of photogenerated charges of g‐C 3 N 4 ‐CN and enriched electrons around it, but also greatly improves the adsorption capacity and selectivity for U(VI) over g‐C 3 N 4 ‐CN by complexing with U(VI). Therefore, g‐C 3 N 4 ‐CN exhibits efficient and stable photocatalytic U(VI) reduction performance, with a saturated uranium extraction capacity of 2644.3 mg g −1 , significantly higher than most reported g‐C 3 N 4 ‐based photocatalysts. Moreover, it also performs well in solar light‐driven uranium extraction from actual seawater. Briefly, this work illustrates the importance of constructing the isosite structure of adsorption and photoreduction for U(VI) in improving the photocatalytic uranium extraction performance. Photocatalytic uranium extraction from seawater is an ideal strategy to obtain uranium resources. Herein, the cyano‐functionalized graphitic carbon nitride (g‐C3N4‐CN) with an isosite structure of adsorption and photoreduction for U(VI) is successfully prepared to achieve efficient photocatalytic uranium extraction from seawater. As the key of the isosite structure, the cyano group not only dramatically promotes the separation of photogenerated charges of g‐C3N4‐CN and enriched electrons around it, but also greatly improves the adsorption capacity and selectivity for U(VI) over g‐C3N4‐CN by complexing with U(VI). Therefore, g‐C3N4‐CN exhibits efficient and stable photocatalytic U(VI) reduction performance, with a saturated uranium extraction capacity of 2644.3 mg g−1, significantly higher than most reported g‐C3N4‐based photocatalysts. Moreover, it also performs well in solar light‐driven uranium extraction from actual seawater. Briefly, this work illustrates the importance of constructing the isosite structure of adsorption and photoreduction for U(VI) in improving the photocatalytic uranium extraction performance. The cyano‐functionalized graphitic carbon nitride with an isosite structure of adsorption and photoreduction for U(VI) is successfully prepared, which achieves efficient and stable photocatalytic U(VI) reduction performance, with a saturated uranium extraction capacity of 2644.3 mg g−1, significantly higher than most reported g‐C3N4‐based photocatalysts. Moreover, it also performs well in solar light‐driven uranium extraction from actual seawater. |
| Author | Wang, Peng Fan, Xiaofeng Deng, Haibo Gao, Qiong Luo, Xingjian Chen, Xianjie Xu, Shicheng Zhu, Wenkun Zhu, Yongfa Liu, Liping Wu, Guang He, Rong Chen, Qian Wei, Yu Hu, Enmin |
| Author_xml | – sequence: 1 givenname: Enmin surname: Hu fullname: Hu, Enmin organization: Southwest University of Science and Technology – sequence: 2 givenname: Qian surname: Chen fullname: Chen, Qian organization: Southwest University of Science and Technology – sequence: 3 givenname: Qiong surname: Gao fullname: Gao, Qiong organization: Southwest University of Science and Technology – sequence: 4 givenname: Xiaofeng surname: Fan fullname: Fan, Xiaofeng organization: Southwest University of Science and Technology – sequence: 5 givenname: Xingjian surname: Luo fullname: Luo, Xingjian organization: Southwest University of Science and Technology – sequence: 6 givenname: Yu surname: Wei fullname: Wei, Yu organization: Southwest University of Science and Technology – sequence: 7 givenname: Guang surname: Wu fullname: Wu, Guang organization: Southwest University of Science and Technology – sequence: 8 givenname: Haibo surname: Deng fullname: Deng, Haibo organization: Southwest University of Science and Technology – sequence: 9 givenname: Shicheng surname: Xu fullname: Xu, Shicheng organization: Southwest University of Science and Technology – sequence: 10 givenname: Peng surname: Wang fullname: Wang, Peng organization: Southwest University of Science and Technology – sequence: 11 givenname: Liping surname: Liu fullname: Liu, Liping organization: Tsinghua University – sequence: 12 givenname: Rong surname: He fullname: He, Rong organization: Southwest University of Science and Technology – sequence: 13 givenname: Xianjie orcidid: 0000-0001-8206-0557 surname: Chen fullname: Chen, Xianjie email: chenxj823@swust.edu.cn organization: Southwest University of Science and Technology – sequence: 14 givenname: Wenkun surname: Zhu fullname: Zhu, Wenkun email: zhuwenkun@swust.edu.cn organization: Southwest University of Science and Technology – sequence: 15 givenname: Yongfa surname: Zhu fullname: Zhu, Yongfa email: zhuyf@tsinghua.edu.cn organization: Chengdu University |
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| Snippet | Photocatalytic uranium extraction from seawater is an ideal strategy to obtain uranium resources. Herein, the cyano‐functionalized graphitic carbon nitride... Abstract Photocatalytic uranium extraction from seawater is an ideal strategy to obtain uranium resources. Herein, the cyano‐functionalized graphitic carbon... |
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| SubjectTerms | Adsorption adsorption and photoreduction isosite Carbon Carbon nitride cyano group Cyano groups graphitic carbon nitride Photocatalysis Seawater Uranium uranium extraction |
| Title | Cyano‐Functionalized Graphitic Carbon Nitride with Adsorption and Photoreduction Isosite Achieving Efficient Uranium Extraction from Seawater |
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