Metal‐Halide Perovskite Crystallization Kinetics: A Review of Experimental and Theoretical Studies

Metal‐halide perovskites (MHPs) are regarded as ideal photovoltaic materials because of their variable crystal material composition and superb optoelectronic performance. However, this compositional variability results in a complicated crystallization process during MHP film fabrication, leading to...

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Published inAdvanced energy materials Vol. 11; no. 24
Main Authors Xie, Yue‐Min, Xue, Qifan, Yip, Hin‐Lap
Format Journal Article
LanguageEnglish
Published Weinheim Wiley Subscription Services, Inc 01.06.2021
Subjects
Crystallization
crystallization kinetics
crystallization modulation
crystallization properties
Kinetics
metal‐halide perovskites
Optoelectronics
Perovskites
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Abstract Metal‐halide perovskites (MHPs) are regarded as ideal photovoltaic materials because of their variable crystal material composition and superb optoelectronic performance. However, this compositional variability results in a complicated crystallization process during MHP film fabrication, leading to reduced MHP film crystallinity and decreased performance of devices containing such films. The crystallization kinetics of MHPs have therefore been extensively explored in efforts to determine the effect of crystallization properties on MHP film properties and figure out the corresponding modulating strategies. Here, the first comprehensive review of reported studies on the crystallization properties of 3D MHPs is presented. The experimental and theoretical research on 3D MHP crystallization kinetics is systematically surveyed, and the methods that are used for modulating MHP crystallization are summarized, namely, solution engineering, compositional engineering, interfacial engineering, and additive passivation. Meanwhile, the prospects and current challenges in revealing perovskite crystallization kinetics are suggested. The vast literature on experimental and theoretical research on the nucleation and growth of metal‐halide perovskite films, as well as the relationships between film properties and crystallization modulating methods including solution engineering, composition engineering, interface engineering, and additive passivation are systematically reviewed. This work consolidates the research on metal‐halide perovskite crystallization kinetics, and highlights new and promising areas of study.
AbstractList Metal‐halide perovskites (MHPs) are regarded as ideal photovoltaic materials because of their variable crystal material composition and superb optoelectronic performance. However, this compositional variability results in a complicated crystallization process during MHP film fabrication, leading to reduced MHP film crystallinity and decreased performance of devices containing such films. The crystallization kinetics of MHPs have therefore been extensively explored in efforts to determine the effect of crystallization properties on MHP film properties and figure out the corresponding modulating strategies. Here, the first comprehensive review of reported studies on the crystallization properties of 3D MHPs is presented. The experimental and theoretical research on 3D MHP crystallization kinetics is systematically surveyed, and the methods that are used for modulating MHP crystallization are summarized, namely, solution engineering, compositional engineering, interfacial engineering, and additive passivation. Meanwhile, the prospects and current challenges in revealing perovskite crystallization kinetics are suggested.
Metal‐halide perovskites (MHPs) are regarded as ideal photovoltaic materials because of their variable crystal material composition and superb optoelectronic performance. However, this compositional variability results in a complicated crystallization process during MHP film fabrication, leading to reduced MHP film crystallinity and decreased performance of devices containing such films. The crystallization kinetics of MHPs have therefore been extensively explored in efforts to determine the effect of crystallization properties on MHP film properties and figure out the corresponding modulating strategies. Here, the first comprehensive review of reported studies on the crystallization properties of 3D MHPs is presented. The experimental and theoretical research on 3D MHP crystallization kinetics is systematically surveyed, and the methods that are used for modulating MHP crystallization are summarized, namely, solution engineering, compositional engineering, interfacial engineering, and additive passivation. Meanwhile, the prospects and current challenges in revealing perovskite crystallization kinetics are suggested. The vast literature on experimental and theoretical research on the nucleation and growth of metal‐halide perovskite films, as well as the relationships between film properties and crystallization modulating methods including solution engineering, composition engineering, interface engineering, and additive passivation are systematically reviewed. This work consolidates the research on metal‐halide perovskite crystallization kinetics, and highlights new and promising areas of study.
Author Yip, Hin‐Lap
Xie, Yue‐Min
Xue, Qifan
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2019; 571
2017; 5
2018; 122
2017; 7
2017; 8
2017; 1
2017; 2
2013; 25
2018; 360
2017; 3
2019; 58
2020; 367
2015; 348
2019; 364
2017; 9
2019; 365
2020; 8
2020; 7
2020; 6
2015; 48
2011; 169
2020; 5
2014; 5
2020; 4
2020; 3
2020; 2
2021; 33
2019; 64
2019; 63
2015; 40
2017; 39
2013; 13
2017; 35
2020; 370
2008; 69
2016; 354
2017; 360
2008; 63
2017; 121
2014; 8
2014; 7
2014; 6
2012; 338
2017; 247
2014; 53
2015; 6
2015; 17
2021; 4
2015; 5
2015; 3
2015; 18
2020; 580
2017; 27
2011; 40
2015; 10
2018; 63
2017; 29
2009; 131
2019; 141
2015; 8
2015; 7
2016; 120
2015; 23
2015; 25
2015; 27
2021
2020; 73
2017; 17
2020
2018; 399
2017; 11
2017; 10
2013; 499
2020; 68
2020; 67
2014; 345
2016; 371
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Snippet Metal‐halide perovskites (MHPs) are regarded as ideal photovoltaic materials because of their variable crystal material composition and superb optoelectronic...
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SubjectTerms Crystallization
crystallization kinetics
crystallization modulation
crystallization properties
Kinetics
metal‐halide perovskites
Optoelectronics
Perovskites
Title Metal‐Halide Perovskite Crystallization Kinetics: A Review of Experimental and Theoretical Studies
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Faenm.202100784
https://www.proquest.com/docview/2544384734
Volume 11
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