A Platelet Graphitic Nanofiber‐Carbon Nanotube Hybrid for Efficient Oxygen Evolution Reaction
Carbon nanostructures with a high‐density of active sites are needed as catalysts for the oxygen evolution reaction (OER). Here we report a platelet graphitic nanofiber‐carbon nanotube (PGNF‐CNT) hybrid electrocatalyst prepared by chemical vapor deposition. The material is composed of interconnected...
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| Published in | ChemCatChem Vol. 12; no. 1; pp. 360 - 365 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
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Weinheim
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08.01.2020
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| ISSN | 1867-3880 1867-3899 |
| DOI | 10.1002/cctc.201901462 |
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| Abstract | Carbon nanostructures with a high‐density of active sites are needed as catalysts for the oxygen evolution reaction (OER). Here we report a platelet graphitic nanofiber‐carbon nanotube (PGNF‐CNT) hybrid electrocatalyst prepared by chemical vapor deposition. The material is composed of interconnected CNTs and nanofibers consisting of graphitized carbon layers stacked at different angles to the fiber axis with a large number of exposed edges. These unique structural characteristics give the hybrid a high density of active sites, fast electron transfer and a large number of mass transport paths. As a result, the material has an excellent electrocatalytic activity for OER with an overpotential of 0.28 V at a current density of 10 mA cm−2, which is much better than those of Ir/C and previously‐reported carbonaceous catalysts.
OER catalysis: A platelet graphitic nanofiber‐carbon nanotube (PGNF‐CNT) hybrid for OER catalysis, the PGNF composed of stacked carbon flakes with numerous exposed edges provides sufficient active sites, while CNTs function as a pathway permitting fast electron transport. |
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| AbstractList | Carbon nanostructures with a high‐density of active sites are needed as catalysts for the oxygen evolution reaction (OER). Here we report a platelet graphitic nanofiber‐carbon nanotube (PGNF‐CNT) hybrid electrocatalyst prepared by chemical vapor deposition. The material is composed of interconnected CNTs and nanofibers consisting of graphitized carbon layers stacked at different angles to the fiber axis with a large number of exposed edges. These unique structural characteristics give the hybrid a high density of active sites, fast electron transfer and a large number of mass transport paths. As a result, the material has an excellent electrocatalytic activity for OER with an overpotential of 0.28 V at a current density of 10 mA cm
−2
, which is much better than those of Ir/C and previously‐reported carbonaceous catalysts. Carbon nanostructures with a high‐density of active sites are needed as catalysts for the oxygen evolution reaction (OER). Here we report a platelet graphitic nanofiber‐carbon nanotube (PGNF‐CNT) hybrid electrocatalyst prepared by chemical vapor deposition. The material is composed of interconnected CNTs and nanofibers consisting of graphitized carbon layers stacked at different angles to the fiber axis with a large number of exposed edges. These unique structural characteristics give the hybrid a high density of active sites, fast electron transfer and a large number of mass transport paths. As a result, the material has an excellent electrocatalytic activity for OER with an overpotential of 0.28 V at a current density of 10 mA cm−2, which is much better than those of Ir/C and previously‐reported carbonaceous catalysts. Carbon nanostructures with a high‐density of active sites are needed as catalysts for the oxygen evolution reaction (OER). Here we report a platelet graphitic nanofiber‐carbon nanotube (PGNF‐CNT) hybrid electrocatalyst prepared by chemical vapor deposition. The material is composed of interconnected CNTs and nanofibers consisting of graphitized carbon layers stacked at different angles to the fiber axis with a large number of exposed edges. These unique structural characteristics give the hybrid a high density of active sites, fast electron transfer and a large number of mass transport paths. As a result, the material has an excellent electrocatalytic activity for OER with an overpotential of 0.28 V at a current density of 10 mA cm−2, which is much better than those of Ir/C and previously‐reported carbonaceous catalysts. OER catalysis: A platelet graphitic nanofiber‐carbon nanotube (PGNF‐CNT) hybrid for OER catalysis, the PGNF composed of stacked carbon flakes with numerous exposed edges provides sufficient active sites, while CNTs function as a pathway permitting fast electron transport. |
| Author | Majeed, Abdul Mehmood, Mazhar Ahmad, Jamil Hou, Peng‐Xiang Tabassum, Hassina Ali, Zulfiqar Li, Xin Liu, Chang |
| Author_xml | – sequence: 1 givenname: Zulfiqar surname: Ali fullname: Ali, Zulfiqar organization: Pakistan Institute of Engineering and Applied Sciences – sequence: 2 givenname: Mazhar surname: Mehmood fullname: Mehmood, Mazhar organization: Pakistan Institute of Engineering and Applied Sciences – sequence: 3 givenname: Jamil surname: Ahmad fullname: Ahmad, Jamil organization: Pakistan Institute of Engineering and Applied Sciences – sequence: 4 givenname: Xin surname: Li fullname: Li, Xin organization: Chinese Academy of Sciences – sequence: 5 givenname: Abdul surname: Majeed fullname: Majeed, Abdul organization: Chinese Academy of Sciences – sequence: 6 givenname: Hassina surname: Tabassum fullname: Tabassum, Hassina organization: Peking University – sequence: 7 givenname: Peng‐Xiang surname: Hou fullname: Hou, Peng‐Xiang email: pxhou@imr.ac.cn organization: Chinese Academy of Sciences – sequence: 8 givenname: Chang orcidid: 0000-0003-3016-3997 surname: Liu fullname: Liu, Chang email: cliu@imr.ac.cn organization: Chinese Academy of Sciences |
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| Snippet | Carbon nanostructures with a high‐density of active sites are needed as catalysts for the oxygen evolution reaction (OER). Here we report a platelet graphitic... |
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| SubjectTerms | Alcogel electrolysis Carbon Carbon nanaotube Carbon nanotubes Catalysts Chemical vapor deposition CVD Electron transfer Graphitization Nanofibers OER electrocatalysis Organic chemistry Oxygen evolution reactions Platelet graphitic nanofiber |
| Title | A Platelet Graphitic Nanofiber‐Carbon Nanotube Hybrid for Efficient Oxygen Evolution Reaction |
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