Aerobic α‐Oxidation of N‐Substituted Tetrahydroisoquinolines to Dihydroisoquinolones via Organo‐photocatalysis
An efficient visible‐light‐induced α‐oxidation of N‐substituted tetrahydroisoquinolines to dihydroisoquinolones has been developed using eosin Y as an organo‐photocatalyst and oxygen as a green oxidant. The reactions were carried out under mild reaction conditions; the desired dihydroisoquinolones w...
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Published in | Advanced synthesis & catalysis Vol. 361; no. 5; pp. 1124 - 1129 |
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Main Authors | , , |
Format | Journal Article |
Language | English |
Published |
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Wiley
05.03.2019
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Abstract | An efficient visible‐light‐induced α‐oxidation of N‐substituted tetrahydroisoquinolines to dihydroisoquinolones has been developed using eosin Y as an organo‐photocatalyst and oxygen as a green oxidant. The reactions were carried out under mild reaction conditions; the desired dihydroisoquinolones were obtained in up to 96% yield at room temperature under oxygen atmosphere. This transformation provides a convenient route to dihydroisoquinolones with a wide range of substrates. |
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AbstractList | An efficient visible‐light‐induced α‐oxidation of N‐substituted tetrahydroisoquinolines to dihydroisoquinolones has been developed using eosin Y as an organo‐photocatalyst and oxygen as a green oxidant. The reactions were carried out under mild reaction conditions; the desired dihydroisoquinolones were obtained in up to 96% yield at room temperature under oxygen atmosphere. This transformation provides a convenient route to dihydroisoquinolones with a wide range of substrates. An efficient visible-light-induced alpha-oxidation of N-substituted tetrahydroisoquinolines to dihydroisoquinolones has been developed using eosin Y as an organo-photocatalyst and oxygen as a green oxidant. The reactions were carried out under mild reaction conditions; the desired dihydroisoquinolones were obtained in up to 96% yield at room temperature under oxygen atmosphere. This transformation provides a convenient route to dihydroisoquinolones with a wide range of substrates. Abstract An efficient visible‐light‐induced α‐oxidation of N ‐substituted tetrahydroisoquinolines to dihydroisoquinolones has been developed using eosin Y as an organo‐photocatalyst and oxygen as a green oxidant. The reactions were carried out under mild reaction conditions; the desired dihydroisoquinolones were obtained in up to 96% yield at room temperature under oxygen atmosphere. This transformation provides a convenient route to dihydroisoquinolones with a wide range of substrates. magnified image |
Author | Lee, Anna Aganda, Kim Christopher C. Hong, Boseok |
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Keywords | SUPPORTED GOLD NANOPARTICLES TERTIARY-AMINES aerobic oxidation C-H FUNCTIONALIZATION dihydroisoquinolones BENZYLIC AMINES lactams VISIBLE-LIGHT SYNTHETIC APPLICATIONS photoredox catalysis BOND ACTIVATION EFFICIENT CYCLIC AMINES MOLECULAR-OXYGEN |
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Snippet | An efficient visible‐light‐induced α‐oxidation of N‐substituted tetrahydroisoquinolines to dihydroisoquinolones has been developed using eosin Y as an... An efficient visible-light-induced alpha-oxidation of N-substituted tetrahydroisoquinolines to dihydroisoquinolones has been developed using eosin Y as an... Abstract An efficient visible‐light‐induced α‐oxidation of N ‐substituted tetrahydroisoquinolines to dihydroisoquinolones has been developed using eosin Y as... |
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SubjectTerms | aerobic oxidation Chemistry Chemistry, Applied Chemistry, Organic dihydroisoquinolones lactams Oxidation Photocatalysis photoredox catalysis Physical Sciences Science & Technology Substitutes Substrates |
Title | Aerobic α‐Oxidation of N‐Substituted Tetrahydroisoquinolines to Dihydroisoquinolones via Organo‐photocatalysis |
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