Efficient microwave absorption achieved through in situ construction of core-shell CoFe2O4@mesoporous carbon hollow spheres
Cobalt ferrite (CoFe 2 O 4 ), with good chemical stability and magnetic loss, can be used to prepare composites with a unique structure and high absorption. In this study, CoFe 2 O 4 @mesoporous carbon hollow spheres (MCHS) with a core-shell structure were prepared by introducing CoFe 2 O 4 magnetic...
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| Published in | International journal of minerals, metallurgy and materials Vol. 30; no. 3; pp. 504 - 514 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Beijing
University of Science and Technology Beijing
01.03.2023
Springer Nature B.V |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Cobalt ferrite (CoFe
2
O
4
), with good chemical stability and magnetic loss, can be used to prepare composites with a unique structure and high absorption. In this study, CoFe
2
O
4
@mesoporous carbon hollow spheres (MCHS) with a core-shell structure were prepared by introducing CoFe
2
O
4
magnetic particles into hollow mesoporous carbon through a simple
in situ
method. Then, the microwave absorption performance of the CoFe
2
O
4
@MCHS composites was investigated. Magnetic and dielectric losses can be effectively coordinated by constructing the porous structure and adjusting the ratio of MCHS and CoFe
2
O
4
. Results show that the impedance matching and absorption properties of the CoFe
2
O
4
@MCHS composites can be altered by tweaking the mass ratio of MCHS and CoFe
2
O
4
. The minimum reflection loss of the CoFe
2
O
4
@MCHS composites reaches -29.7 dB at 5.8 GHz. In addition, the effective absorption bandwidth is 3.7 GHz, with the thickness being 2.5 mm. The boosted microwave absorption can be ascribed to the porous core-shell structure and introduction of magnetic particles. The coordination between the microporous morphology and the core-shell structure is conducive to improving the attenuation coefficient and achieving good impedance matching. The porous core-shell structure provides large solid-void and CoFe
2
O
4
−C interfaces to induce interfacial polarization and extend the electromagnetic waves’ multiple scattering and reflection. Furthermore, natural resonance, exchange resonance, and eddy current loss work together for the magnetic loss. This method provides a practical solution to prepare core-shell structure microwave absorbents. |
|---|---|
| AbstractList | Cobalt ferrite (CoFe
2
O
4
), with good chemical stability and magnetic loss, can be used to prepare composites with a unique structure and high absorption. In this study, CoFe
2
O
4
@mesoporous carbon hollow spheres (MCHS) with a core-shell structure were prepared by introducing CoFe
2
O
4
magnetic particles into hollow mesoporous carbon through a simple
in situ
method. Then, the microwave absorption performance of the CoFe
2
O
4
@MCHS composites was investigated. Magnetic and dielectric losses can be effectively coordinated by constructing the porous structure and adjusting the ratio of MCHS and CoFe
2
O
4
. Results show that the impedance matching and absorption properties of the CoFe
2
O
4
@MCHS composites can be altered by tweaking the mass ratio of MCHS and CoFe
2
O
4
. The minimum reflection loss of the CoFe
2
O
4
@MCHS composites reaches -29.7 dB at 5.8 GHz. In addition, the effective absorption bandwidth is 3.7 GHz, with the thickness being 2.5 mm. The boosted microwave absorption can be ascribed to the porous core-shell structure and introduction of magnetic particles. The coordination between the microporous morphology and the core-shell structure is conducive to improving the attenuation coefficient and achieving good impedance matching. The porous core-shell structure provides large solid-void and CoFe
2
O
4
−C interfaces to induce interfacial polarization and extend the electromagnetic waves’ multiple scattering and reflection. Furthermore, natural resonance, exchange resonance, and eddy current loss work together for the magnetic loss. This method provides a practical solution to prepare core-shell structure microwave absorbents. Cobalt ferrite (CoFe2O4), with good chemical stability and magnetic loss, can be used to prepare composites with a unique structure and high absorption. In this study, CoFe2O4@mesoporous carbon hollow spheres (MCHS) with a core-shell structure were prepared by introducing CoFe2O4 magnetic particles into hollow mesoporous carbon through a simple in situ method. Then, the microwave absorption performance of the CoFe2O4@MCHS composites was investigated. Magnetic and dielectric losses can be effectively coordinated by constructing the porous structure and adjusting the ratio of MCHS and CoFe2O4. Results show that the impedance matching and absorption properties of the CoFe2O4@MCHS composites can be altered by tweaking the mass ratio of MCHS and CoFe2O4. The minimum reflection loss of the CoFe2O4@MCHS composites reaches -29.7 dB at 5.8 GHz. In addition, the effective absorption bandwidth is 3.7 GHz, with the thickness being 2.5 mm. The boosted microwave absorption can be ascribed to the porous core-shell structure and introduction of magnetic particles. The coordination between the microporous morphology and the core-shell structure is conducive to improving the attenuation coefficient and achieving good impedance matching. The porous core-shell structure provides large solid-void and CoFe2O4−C interfaces to induce interfacial polarization and extend the electromagnetic waves’ multiple scattering and reflection. Furthermore, natural resonance, exchange resonance, and eddy current loss work together for the magnetic loss. This method provides a practical solution to prepare core-shell structure microwave absorbents. |
| Author | Zhang, Xin Ren, Lianggui Wang, Yiqun Wu, Guanglei He, Qinchuan |
| Author_xml | – sequence: 1 givenname: Lianggui surname: Ren fullname: Ren, Lianggui organization: College of Materials and Chemistry & Chemical Engineering, Chengdu University of Technology, Institute of Materials for Energy and Environment, State Key Laboratory of Bio-fibers and Eco-textiles, College of Materials Science and Engineering, Qingdao University – sequence: 2 givenname: Yiqun surname: Wang fullname: Wang, Yiqun email: wangyiqun17@cdut.edu.cn organization: College of Materials and Chemistry & Chemical Engineering, Chengdu University of Technology – sequence: 3 givenname: Xin surname: Zhang fullname: Zhang, Xin organization: College of Materials and Chemistry & Chemical Engineering, Chengdu University of Technology – sequence: 4 givenname: Qinchuan surname: He fullname: He, Qinchuan organization: College of Materials and Chemistry & Chemical Engineering, Chengdu University of Technology – sequence: 5 givenname: Guanglei surname: Wu fullname: Wu, Guanglei email: wuguanglei@qdu.edu.cn, wuguanglei@mail.xjtu.edu.cn organization: Institute of Materials for Energy and Environment, State Key Laboratory of Bio-fibers and Eco-textiles, College of Materials Science and Engineering, Qingdao University |
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), with good chemical stability and magnetic loss, can be used to prepare composites with a unique structure and high absorption. In... Cobalt ferrite (CoFe2O4), with good chemical stability and magnetic loss, can be used to prepare composites with a unique structure and high absorption. In... |
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| Title | Efficient microwave absorption achieved through in situ construction of core-shell CoFe2O4@mesoporous carbon hollow spheres |
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