Living supramolecular polymerization
Greater control is achieved over the chain growth and properties of dynamic materials Most polymers that we encounter, like those used in grocery bags and soda bottles, are formed from small molecules (monomers) held together by strong covalent bonds. In supramolecular polymerization, monomers bond...
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| Published in | Science (American Association for the Advancement of Science) Vol. 349; no. 6245; pp. 241 - 242 |
|---|---|
| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Washington
The American Association for the Advancement of Science
17.07.2015
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Greater control is achieved over the chain growth and properties of dynamic materials
Most polymers that we encounter, like those used in grocery bags and soda bottles, are formed from small molecules (monomers) held together by strong covalent bonds. In supramolecular polymerization, monomers bond through weaker reversible interactions, such as hydrogen bonds (H-bonds). Supramolecular polymerization usually proceeds through step-growth mechanisms (
1
), where both ends of each monomer are reactive and many smaller oligomers form before long polymers appear. To overcome this problem, a method developed for covalent polymers known as living polymerization has been adopted for supramolecular polymers to achieve better control and uniformity of chain growth and dispersity. |
|---|---|
| AbstractList | Most polymers that we encounter, like those used in grocery bags and soda bottles, are formed from small molecules (monomers) held together by strong covalent bonds. In supramolecular polymerization, monomers bond through weaker reversible interactions, such as hydrogen bonds (H-bonds). Supramolecular polymerization usually proceeds through step-growth mechanisms (1), where both ends of each monomer are reactive and many smaller oligomers form before long polymers appear. To overcome this problem, a method developed for covalent polymers known as living polymerization has been adopted for supramolecular polymers to achieve better control and uniformity of chain growth and dispersity. Greater control is achieved over the chain growth and properties of dynamic materials Most polymers that we encounter, like those used in grocery bags and soda bottles, are formed from small molecules (monomers) held together by strong covalent bonds. In supramolecular polymerization, monomers bond through weaker reversible interactions, such as hydrogen bonds (H-bonds). Supramolecular polymerization usually proceeds through step-growth mechanisms ( 1 ), where both ends of each monomer are reactive and many smaller oligomers form before long polymers appear. To overcome this problem, a method developed for covalent polymers known as living polymerization has been adopted for supramolecular polymers to achieve better control and uniformity of chain growth and dispersity. Most polymers that we encounter, like those used in grocery bags and soda bottles, are formed from small molecules (monomers) held together by strong covalent bonds. In supramolecular polymerization, monomers bond through weaker reversible interactions, such as hydrogen bonds (H-bonds). Supramolecular polymerization usually proceeds through step-growth mechanisms , where both ends of each monomer are reactive and many smaller oligomers form before long polymers appear. To overcome this problem, a method developed for covalent polymers known as living polymerization has been adopted for supramolecular polymers to achieve better control and uniformity of chain growth and dispersity. |
| Author | Mukhopadhyay, Rahul Dev Ajayaghosh, Ayyappanpillai |
| Author_xml | – sequence: 1 givenname: Rahul Dev surname: Mukhopadhyay fullname: Mukhopadhyay, Rahul Dev organization: Chemical Sciences and Technology Division, CSIR–National Institute for Interdisciplinary Science and Technology (CSIRNIIST), Trivandrum 695019, India., Academy of Scientific and Innovative Research (AcSIR), CSIR-NIIST, Trivandrum 695019, India – sequence: 2 givenname: Ayyappanpillai surname: Ajayaghosh fullname: Ajayaghosh, Ayyappanpillai organization: Chemical Sciences and Technology Division, CSIR–National Institute for Interdisciplinary Science and Technology (CSIRNIIST), Trivandrum 695019, India., Academy of Scientific and Innovative Research (AcSIR), CSIR-NIIST, Trivandrum 695019, India |
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| Cites_doi | 10.1126/science.251.4996.887 10.1021/ja505941b 10.1038/nchem.1332 10.1038/453171a 10.1038/ncomms5372 10.1038/nchem.2038 10.1126/science.1261816 10.1038/nchem.1849 10.1126/science.1141382 10.1021/ja511952c 10.1126/science.aaa4249 |
| ContentType | Journal Article |
| Copyright | Copyright © 2015, American Association for the Advancement of Science |
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| DOI | 10.1126/science.aac7422 |
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| Snippet | Greater control is achieved over the chain growth and properties of dynamic materials
Most polymers that we encounter, like those used in grocery bags and soda... Most polymers that we encounter, like those used in grocery bags and soda bottles, are formed from small molecules (monomers) held together by strong covalent... |
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| SubjectTerms | Bags bottles Covalence Covalent bonds hydrogen bonding Hydrogen bonds Molecular chemistry Monomers Polymerization Polymers Variability |
| Title | Living supramolecular polymerization |
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