Evaluation of the photocurrent value for poly(2,5-dicyano-p-phenylene-vinylene)-co-(p-phenylene-vinylene) (DCN-PPV/PPV)

A method to obtain poly(2,5-dicyano- p -phenylene-vinylene)-co-( p -phenylene-vinylene) (DCN-PPV/PPV) block copolymer was developed. The structural characteristics of the copolymer and its capability to generate a photocurrent were evaluated. IR spectra indicate the complete conversion of precursor...

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Published inJournal of solid state electrochemistry Vol. 20; no. 9; pp. 2551 - 2557
Main Authors Santos, Fábio Santana dos, Bertuzzi, Diego L., Pedroso, Alex V., Voinarovicz, Marco A., Klider, Karine C. C. W. dos S., Péres, Laura O., Garcia, Jarem R.
Format Journal Article
LanguageEnglish
Published Berlin/Heidelberg Springer Berlin Heidelberg 01.09.2016
Springer Nature B.V
Subjects
Analytical Chemistry
Block copolymers
Characterization and Evaluation of Materials
Chemistry
Chemistry and Materials Science
Condensed Matter Physics
Cyano groups
Electrochemistry
Energy levels
Energy Storage
Evaluation
Infrared spectroscopy
Low pressure
Molecular orbitals
Original Paper
Photoelectric effect
Photoelectric emission
Physical Chemistry
Polyphenylene vinylene
Stability analysis
Thermal analysis
Conjugated polymers
Photocurrent
Cyano group
PPV-type copolymer
Photovoltaic devices
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Abstract A method to obtain poly(2,5-dicyano- p -phenylene-vinylene)-co-( p -phenylene-vinylene) (DCN-PPV/PPV) block copolymer was developed. The structural characteristics of the copolymer and its capability to generate a photocurrent were evaluated. IR spectra indicate the complete conversion of precursor copolymer into DCN-PPV/PPV at 250 °C under low-pressure conditions. The DCN-PPV/PPV polymer optical band gap was determined based on the observed UV-Vis spectral data by using Tauc’s equation. The two linear regions in the Tauc curve (E g  = 2.63 eV and 2.02) revealed the formation of a block copolymer. Thermal analysis showed that DCN-PPV/PPV has a higher stability than PPV and starts to degrade at 317 °C in air. The electronic parameters of DCN-PPV/PPV (IP = 5.25 eV, EA = 3.30 eV, and E g  = 1.95 eV) indicate that the cyano groups reduce the LUMO energy level without affecting the HOMO energy by much. DCN-PPV/PPV photoactivity measurements show higher photocurrent values compared to those for PPV.
AbstractList A method to obtain poly(2,5-dicyano-p-phenylene-vinylene)-co-(p-phenylene-vinylene) (DCN-PPV/PPV) block copolymer was developed. The structural characteristics of the copolymer and its capability to generate a photocurrent were evaluated. IR spectra indicate the complete conversion of precursor copolymer into DCN-PPV/PPV at 250 °C under low-pressure conditions. The DCN-PPV/PPV polymer optical band gap was determined based on the observed UV-Vis spectral data by using Tauc’s equation. The two linear regions in the Tauc curve (Eg = 2.63 eV and 2.02) revealed the formation of a block copolymer. Thermal analysis showed that DCN-PPV/PPV has a higher stability than PPV and starts to degrade at 317 °C in air. The electronic parameters of DCN-PPV/PPV (IP = 5.25 eV, EA = 3.30 eV, and Eg = 1.95 eV) indicate that the cyano groups reduce the LUMO energy level without affecting the HOMO energy by much. DCN-PPV/PPV photoactivity measurements show higher photocurrent values compared to those for PPV.
A method to obtain poly(2,5-dicyano- p -phenylene-vinylene)-co-( p -phenylene-vinylene) (DCN-PPV/PPV) block copolymer was developed. The structural characteristics of the copolymer and its capability to generate a photocurrent were evaluated. IR spectra indicate the complete conversion of precursor copolymer into DCN-PPV/PPV at 250 °C under low-pressure conditions. The DCN-PPV/PPV polymer optical band gap was determined based on the observed UV-Vis spectral data by using Tauc’s equation. The two linear regions in the Tauc curve (E g  = 2.63 eV and 2.02) revealed the formation of a block copolymer. Thermal analysis showed that DCN-PPV/PPV has a higher stability than PPV and starts to degrade at 317 °C in air. The electronic parameters of DCN-PPV/PPV (IP = 5.25 eV, EA = 3.30 eV, and E g  = 1.95 eV) indicate that the cyano groups reduce the LUMO energy level without affecting the HOMO energy by much. DCN-PPV/PPV photoactivity measurements show higher photocurrent values compared to those for PPV.
Author Voinarovicz, Marco A.
Pedroso, Alex V.
Klider, Karine C. C. W. dos S.
Garcia, Jarem R.
Péres, Laura O.
Santos, Fábio Santana dos
Bertuzzi, Diego L.
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CitedBy_id crossref_primary_10_1515_polyeng_2022_0104
crossref_primary_10_1002_slct_202103460
crossref_primary_10_1021_acscatal_6b03064
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Keywords Conjugated polymers
Photocurrent
Cyano group
PPV-type copolymer
Photovoltaic devices
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Snippet A method to obtain poly(2,5-dicyano- p -phenylene-vinylene)-co-( p -phenylene-vinylene) (DCN-PPV/PPV) block copolymer was developed. The structural...
A method to obtain poly(2,5-dicyano-p-phenylene-vinylene)-co-(p-phenylene-vinylene) (DCN-PPV/PPV) block copolymer was developed. The structural characteristics...
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SubjectTerms Analytical Chemistry
Block copolymers
Characterization and Evaluation of Materials
Chemistry
Chemistry and Materials Science
Condensed Matter Physics
Cyano groups
Electrochemistry
Energy levels
Energy Storage
Evaluation
Infrared spectroscopy
Low pressure
Molecular orbitals
Original Paper
Photoelectric effect
Photoelectric emission
Physical Chemistry
Polyphenylene vinylene
Stability analysis
Thermal analysis
Title Evaluation of the photocurrent value for poly(2,5-dicyano-p-phenylene-vinylene)-co-(p-phenylene-vinylene) (DCN-PPV/PPV)
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