Rational Design of Nanostructured MnO2 Cathode for High-performance Aqueous Zinc Ion Batteries

Aqueous Zn-MnO 2 batteries hold a promising potential for grid-scale energy storage applications due to their intrinsic safety, low fabrication cost, environmental friendliness and high theoretical energy densities. Developing novel nanostructured cathode materials with high discharge voltage, large...

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Published in	Chemical research in Chinese universities Vol. 39; no. 4; pp. 599 - 611
Main Authors	Li, Qi, Zhao, Yajun, Wang, Yueyang, Khasraw, Abdalla Kovan, Zhao, Yi, Sun, Xiaoming
Format	Journal Article
Language	English
Published	Changchun Jilin University and The Editorial Department of Chemical Research in Chinese Universities 01.08.2023 Springer Nature B.V
Subjects	Analytical Chemistry Cathodes Chemical reactions Chemistry Chemistry and Materials Science Chemistry/Food Science Design defects Electrode materials Energy storage Inorganic Chemistry Manganese dioxide Nanostructure Organic Chemistry Physical Chemistry Production costs Rechargeable batteries Review Structural stability Energy storage mechanism cathode Aqueous Zn battery Nanostructured MnO Material design strategy
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Abstract	Aqueous Zn-MnO 2 batteries hold a promising potential for grid-scale energy storage applications due to their intrinsic safety, low fabrication cost, environmental friendliness and high theoretical energy densities. Developing novel nanostructured cathode materials with high discharge voltage, large capacity and excellent structural stability is one of the critical ways to achieve the high-performance aqueous Zn batteries. Enlighten by that, comprehending principles of materials design and identifying the challenges faced by the state-of-the-art MnO 2 hosts are vital preconditions. Rather than a simple comparison, this review mainly focuses on design strategies regarding to MnO 2 -based materials, including defect engineering, interfacial engineering, and pre-intercalation engineering. In addition, the energy storage mechanisms of MnO 2 -based cathodes are discussed to clarify the complicated chemical reactions during battery cycling. Challenges and perspectives are outlined to guide the further development of advanced Zn-MnO 2 batteries.
AbstractList	Aqueous Zn-MnO 2 batteries hold a promising potential for grid-scale energy storage applications due to their intrinsic safety, low fabrication cost, environmental friendliness and high theoretical energy densities. Developing novel nanostructured cathode materials with high discharge voltage, large capacity and excellent structural stability is one of the critical ways to achieve the high-performance aqueous Zn batteries. Enlighten by that, comprehending principles of materials design and identifying the challenges faced by the state-of-the-art MnO 2 hosts are vital preconditions. Rather than a simple comparison, this review mainly focuses on design strategies regarding to MnO 2 -based materials, including defect engineering, interfacial engineering, and pre-intercalation engineering. In addition, the energy storage mechanisms of MnO 2 -based cathodes are discussed to clarify the complicated chemical reactions during battery cycling. Challenges and perspectives are outlined to guide the further development of advanced Zn-MnO 2 batteries. Aqueous Zn-MnO2 batteries hold a promising potential for grid-scale energy storage applications due to their intrinsic safety, low fabrication cost, environmental friendliness and high theoretical energy densities. Developing novel nanostructured cathode materials with high discharge voltage, large capacity and excellent structural stability is one of the critical ways to achieve the high-performance aqueous Zn batteries. Enlighten by that, comprehending principles of materials design and identifying the challenges faced by the state-of-the-art MnO2 hosts are vital preconditions. Rather than a simple comparison, this review mainly focuses on design strategies regarding to MnO2-based materials, including defect engineering, interfacial engineering, and pre-intercalation engineering. In addition, the energy storage mechanisms of MnO2-based cathodes are discussed to clarify the complicated chemical reactions during battery cycling. Challenges and perspectives are outlined to guide the further development of advanced Zn-MnO2 batteries.
Author	Zhao, Yi Wang, Yueyang Khasraw, Abdalla Kovan Sun, Xiaoming Li, Qi Zhao, Yajun
Author_xml	– sequence: 1 givenname: Qi surname: Li fullname: Li, Qi organization: State Key Laboratory of Chemical Resource Engineering, College of Chemistry, Beijing University of Chemical Technology – sequence: 2 givenname: Yajun surname: Zhao fullname: Zhao, Yajun organization: State Key Laboratory of Chemical Resource Engineering, College of Chemistry, Beijing University of Chemical Technology – sequence: 3 givenname: Yueyang surname: Wang fullname: Wang, Yueyang organization: State Key Laboratory of Chemical Resource Engineering, College of Chemistry, Beijing University of Chemical Technology – sequence: 4 givenname: Abdalla Kovan surname: Khasraw fullname: Khasraw, Abdalla Kovan organization: State Key Laboratory of Chemical Resource Engineering, College of Chemistry, Beijing University of Chemical Technology – sequence: 5 givenname: Yi surname: Zhao fullname: Zhao, Yi email: zybattery@buct.edu.cn organization: State Key Laboratory of Chemical Resource Engineering, College of Chemistry, Beijing University of Chemical Technology, Advanced Technology Research Institute, Beijing Institute of Technology – sequence: 6 givenname: Xiaoming surname: Sun fullname: Sun, Xiaoming email: sunxm@mail.buct.edu.cn organization: State Key Laboratory of Chemical Resource Engineering, College of Chemistry, Beijing University of Chemical Technology
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Snippet	Aqueous Zn-MnO 2 batteries hold a promising potential for grid-scale energy storage applications due to their intrinsic safety, low fabrication cost,... Aqueous Zn-MnO2 batteries hold a promising potential for grid-scale energy storage applications due to their intrinsic safety, low fabrication cost,...
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SubjectTerms	Analytical Chemistry Cathodes Chemical reactions Chemistry Chemistry and Materials Science Chemistry/Food Science Design defects Electrode materials Energy storage Inorganic Chemistry Manganese dioxide Nanostructure Organic Chemistry Physical Chemistry Production costs Rechargeable batteries Review Structural stability
Title	Rational Design of Nanostructured MnO2 Cathode for High-performance Aqueous Zinc Ion Batteries
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