Petroleum pitch derived hard carbon via NaCl-template as anode materials with high rate performance for sodium ion battery
Sodium-ion batteries (SIBs) have garnered significant interest in energy storage due to their similar working mechanism to lithium ion batteries and abundant reserves of sodium resource. Exploring facile synthesis of a carbon-based anode materials with capable electrochemical performance is key to p...
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| Published in | Frontiers of chemical science and engineering Vol. 18; no. 7 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Beijing
Higher Education Press
01.07.2024
Springer Nature B.V |
| Subjects | |
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| Abstract | Sodium-ion batteries (SIBs) have garnered significant interest in energy storage due to their similar working mechanism to lithium ion batteries and abundant reserves of sodium resource. Exploring facile synthesis of a carbon-based anode materials with capable electrochemical performance is key to promoting the practical application of SIBs. In this work, a combination of petroleum pitch and recyclable sodium chloride is selected as the carbon source and template to obtain hard carbon (HC) anode for SIBs. Carbonization times and temperatures are optimized by assessing the sodium ion storage behavior of different HC materials. The optimized HC exhibits a remarkable capacity of over 430 mA·hg
−1
after undergoing full activation through 500 cycles at a density of current of 0.1 A·g
−1
. Furthermore, it demonstrates an initial discharge capacity of 276 mAh·g
−1
at a density of current of 0.5 A·g
−1
. Meanwhile, the optimized HC shows a good capacity retention (170 mAh·g
−1
after 750 cycles) and a remarkable rate ability (166 mAh·g
−1
at 2 A·g
−1
). The enhanced capacity is attributed to the suitable degree of graphitization and surface area, which improve the sodium ion transport and storage. |
|---|---|
| AbstractList | Sodium-ion batteries (SIBs) have garnered significant interest in energy storage due to their similar working mechanism to lithium ion batteries and abundant reserves of sodium resource. Exploring facile synthesis of a carbon-based anode materials with capable electrochemical performance is key to promoting the practical application of SIBs. In this work, a combination of petroleum pitch and recyclable sodium chloride is selected as the carbon source and template to obtain hard carbon (HC) anode for SIBs. Carbonization times and temperatures are optimized by assessing the sodium ion storage behavior of different HC materials. The optimized HC exhibits a remarkable capacity of over 430 mA·hg−1 after undergoing full activation through 500 cycles at a density of current of 0.1 A·g−1. Furthermore, it demonstrates an initial discharge capacity of 276 mAh·g−1 at a density of current of 0.5 A·g−1. Meanwhile, the optimized HC shows a good capacity retention (170 mAh·g−1 after 750 cycles) and a remarkable rate ability (166 mAh·g−1 at 2 A·g−1). The enhanced capacity is attributed to the suitable degree of graphitization and surface area, which improve the sodium ion transport and storage. Sodium-ion batteries (SIBs) have garnered significant interest in energy storage due to their similar working mechanism to lithium ion batteries and abundant reserves of sodium resource. Exploring facile synthesis of a carbon-based anode materials with capable electrochemical performance is key to promoting the practical application of SIBs. In this work, a combination of petroleum pitch and recyclable sodium chloride is selected as the carbon source and template to obtain hard carbon (HC) anode for SIBs. Carbonization times and temperatures are optimized by assessing the sodium ion storage behavior of different HC materials. The optimized HC exhibits a remarkable capacity of over 430 mA·hg −1 after undergoing full activation through 500 cycles at a density of current of 0.1 A·g −1 . Furthermore, it demonstrates an initial discharge capacity of 276 mAh·g −1 at a density of current of 0.5 A·g −1 . Meanwhile, the optimized HC shows a good capacity retention (170 mAh·g −1 after 750 cycles) and a remarkable rate ability (166 mAh·g −1 at 2 A·g −1 ). The enhanced capacity is attributed to the suitable degree of graphitization and surface area, which improve the sodium ion transport and storage. |
| ArticleNumber | 73 |
| Author | Li, Xiaoxue Wu, Baoyu Gao, Yinyi Bao, Tianzeng Cao, Dianxue Zhu, Kai Sun, Hao Wu, Hongbin |
| Author_xml | – sequence: 1 givenname: Baoyu surname: Wu fullname: Wu, Baoyu organization: Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education, College of Materials Science and Chemical Engineering, Harbin Engineering University – sequence: 2 givenname: Hao surname: Sun fullname: Sun, Hao organization: Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education, College of Materials Science and Chemical Engineering, Harbin Engineering University – sequence: 3 givenname: Xiaoxue surname: Li fullname: Li, Xiaoxue organization: Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education, College of Materials Science and Chemical Engineering, Harbin Engineering University – sequence: 4 givenname: Yinyi surname: Gao fullname: Gao, Yinyi organization: Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education, College of Materials Science and Chemical Engineering, Harbin Engineering University – sequence: 5 givenname: Tianzeng surname: Bao fullname: Bao, Tianzeng organization: Hunan Hongshan New Energy Technology Co., Ltd – sequence: 6 givenname: Hongbin surname: Wu fullname: Wu, Hongbin organization: Hunan Hongshan New Energy Technology Co., Ltd – sequence: 7 givenname: Kai surname: Zhu fullname: Zhu, Kai email: kzhu@hrbeu.edu.cn organization: Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education, College of Materials Science and Chemical Engineering, Harbin Engineering University – sequence: 8 givenname: Dianxue surname: Cao fullname: Cao, Dianxue email: caodianxue@hrbeu.edu.cn organization: Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education, College of Materials Science and Chemical Engineering, Harbin Engineering University |
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| Snippet | Sodium-ion batteries (SIBs) have garnered significant interest in energy storage due to their similar working mechanism to lithium ion batteries and abundant... |
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| SubjectTerms | Anodes Carbon Chemical synthesis Chemistry Chemistry and Materials Science Density Electrochemical analysis Electrode materials Graphitization Industrial Chemistry/Chemical Engineering Ion storage Ion transport Lithium-ion batteries Nanotechnology Research Article Sodium Sodium chloride Sodium-ion batteries |
| Title | Petroleum pitch derived hard carbon via NaCl-template as anode materials with high rate performance for sodium ion battery |
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