Hydrothermally prepared ultra-stable multilayer nanoflake NiO-based electrochromic films
Electrochromic materials cycle between colored and bleached states under various applied voltage and have applications in smart windows and displays. The formation of a micro–nano structure in electrochromic thin films using hydrothermal methods can improve their properties. However, the conventiona...
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| Published in | Electrochimica acta Vol. 441; p. 141812 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
10.02.2023
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| Subjects | |
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| Abstract | Electrochromic materials cycle between colored and bleached states under various applied voltage and have applications in smart windows and displays. The formation of a micro–nano structure in electrochromic thin films using hydrothermal methods can improve their properties. However, the conventional constant-temperature hydrothermal method yields films that easily peel from the conductive substrate during electrochromic cycling, resulting in performance losses. Therefore, we investigated the effect of a gradient-temperature hydrothermal protocol on the electrochromic performance of NiO thin films. First, a layer of small, strongly adhered crystal grains was seeded on an indium tin oxide substrate. Thereafter, NiO nanoflake layers were grown by adjusting the reaction temperature. The prepared film could be operated for 14,000 electrochromic cycles, four-times more than those of the conventionally prepared films, without significant performance loss. Therefore, our proposed method enhances the cyclic stability of micro–nanostructured NiO thin films significantly and will aid the development of high-performance electrochromic thin films having broad applications. |
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| AbstractList | Electrochromic materials cycle between colored and bleached states under various applied voltage and have applications in smart windows and displays. The formation of a micro–nano structure in electrochromic thin films using hydrothermal methods can improve their properties. However, the conventional constant-temperature hydrothermal method yields films that easily peel from the conductive substrate during electrochromic cycling, resulting in performance losses. Therefore, we investigated the effect of a gradient-temperature hydrothermal protocol on the electrochromic performance of NiO thin films. First, a layer of small, strongly adhered crystal grains was seeded on an indium tin oxide substrate. Thereafter, NiO nanoflake layers were grown by adjusting the reaction temperature. The prepared film could be operated for 14,000 electrochromic cycles, four-times more than those of the conventionally prepared films, without significant performance loss. Therefore, our proposed method enhances the cyclic stability of micro–nanostructured NiO thin films significantly and will aid the development of high-performance electrochromic thin films having broad applications. |
| ArticleNumber | 141812 |
| Author | Wang, Long Ge, Chaoqun Liu, Gu Xiong, Shanxin Xu, Kejun Wang, Weichao Wang, Liuying Wang, Bin Chen, Mengzhou |
| Author_xml | – sequence: 1 givenname: Kejun orcidid: 0000-0002-7973-9056 surname: Xu fullname: Xu, Kejun organization: Xi'an Research Institute of High Technology, Xi'an, Shaanxi 710025, China – sequence: 2 givenname: Liuying surname: Wang fullname: Wang, Liuying email: lywangxa@163.com organization: Xi'an Research Institute of High Technology, Xi'an, Shaanxi 710025, China – sequence: 3 givenname: Shanxin orcidid: 0000-0002-6293-3872 surname: Xiong fullname: Xiong, Shanxin email: xiongsx@xust.edu.cn organization: College of Chemistry and Chemical Engineering, Xi‘an University of Science and Technology, Xi'an, 710054, PR China – sequence: 4 givenname: Chaoqun surname: Ge fullname: Ge, Chaoqun organization: Xi'an Research Institute of High Technology, Xi'an, Shaanxi 710025, China – sequence: 5 givenname: Long surname: Wang fullname: Wang, Long organization: Xi'an Research Institute of High Technology, Xi'an, Shaanxi 710025, China – sequence: 6 givenname: Bin surname: Wang fullname: Wang, Bin organization: Xi'an Research Institute of High Technology, Xi'an, Shaanxi 710025, China – sequence: 7 givenname: Weichao surname: Wang fullname: Wang, Weichao organization: Xi'an Research Institute of High Technology, Xi'an, Shaanxi 710025, China – sequence: 8 givenname: Mengzhou surname: Chen fullname: Chen, Mengzhou organization: Xi'an Research Institute of High Technology, Xi'an, Shaanxi 710025, China – sequence: 9 givenname: Gu surname: Liu fullname: Liu, Gu email: liugu5032@163.com organization: Xi'an Research Institute of High Technology, Xi'an, Shaanxi 710025, China |
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| Keywords | Electrochromic film Gradient-temperature hydrothermal protocol Nickel oxide Nano sheet structure adjustment |
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| Snippet | Electrochromic materials cycle between colored and bleached states under various applied voltage and have applications in smart windows and displays. The... |
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| SubjectTerms | Electrochromic film Gradient-temperature hydrothermal protocol Nano sheet structure adjustment Nickel oxide |
| Title | Hydrothermally prepared ultra-stable multilayer nanoflake NiO-based electrochromic films |
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