Temperature Dependence of Emission Properties of Self-Assembled InGaN Quantum Dots
Emission properties of self-assembled green-emitting InGaN quantum dots (QDs) grown on sapphire substrates by using metal organic chemical vapor deposition are studied by temperature-dependent photoluminescence (PL) measurements. As temperature increases (15-300K), the PL peak energy shows an anomal...
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Published in | Chinese physics letters Vol. 31; no. 11; pp. 70 - 73 |
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Language | English |
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01.11.2014
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Abstract | Emission properties of self-assembled green-emitting InGaN quantum dots (QDs) grown on sapphire substrates by using metal organic chemical vapor deposition are studied by temperature-dependent photoluminescence (PL) measurements. As temperature increases (15-300K), the PL peak energy shows an anomalous V-shaped (redshift blueshift) variation instead of an S-shaped (redshift-blueshift-redshift) variation, as observed typically in green-emitting InGaN/GaN multi-quantum wells (MOWs). The PL full width at half maximum (FWHM) also shows a V-shaped (decrease-increase) variation. The temperature dependence of the PL peak energy and FWHM of QDs are well explained by a model similar to MOWs, in which carriers transferring in localized states play an important role, while the confinement energy of localized states in the QDs is significantly larger than that in MOWs. By analyzing the integrated PL intensity, the larger confinement energy of localized states in the QDs is estimated to be 105.9meV, which is well explained by taking into account the band-gap shrinkage and carrier thermalization with temperature. It is also found that the nonradiative combination centers in QD samples are much less than those in QW samples with the same In content. |
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AbstractList | Emission properties of self-assembled green-emitting InGaN quantum dots (QDs) grown on sapphire substrates by using metal organic chemical vapor deposition are studied by temperature-dependent photoluminescence (PL) measurements. As temperature increases (15-300K), the PL peak energy shows an anomalous V-shaped (redshift-blueshift) variation instead of an S-shaped (redshift-blueshift-redshift) variation, as observed typically in green-emitting InGaN/GaN multi-quantum wells (MQWs). The PL full width at half maximum (FWHM) also shows a V-shaped (decrease-increase) variation. The temperature dependence of the PL peak energy and FWHM of QDs are well explained by a model similar to MQWs, in which carriers transferring in localized states play an important role, while the confinement energy of localized states in the QDs is significantly larger than that in MQWs. By analyzing the integrated PL intensity, the larger confinement energy of localized states in the QDs is estimated to be 105.9 meV, which is well explained by taking into account the band-gap shrinkage and carrier thermalization with temperature. It is also found that the nonradiative combination centers in QD samples are much less than those in QW samples with the same In content. Emission properties of self-assembled green-emitting InGaN quantum dots (QDs) grown on sapphire substrates by using metal organic chemical vapor deposition are studied by temperature-dependent photoluminescence (PL) measurements. As temperature increases (15-300K), the PL peak energy shows an anomalous V-shaped (redshift blueshift) variation instead of an S-shaped (redshift-blueshift-redshift) variation, as observed typically in green-emitting InGaN/GaN multi-quantum wells (MOWs). The PL full width at half maximum (FWHM) also shows a V-shaped (decrease-increase) variation. The temperature dependence of the PL peak energy and FWHM of QDs are well explained by a model similar to MOWs, in which carriers transferring in localized states play an important role, while the confinement energy of localized states in the QDs is significantly larger than that in MOWs. By analyzing the integrated PL intensity, the larger confinement energy of localized states in the QDs is estimated to be 105.9meV, which is well explained by taking into account the band-gap shrinkage and carrier thermalization with temperature. It is also found that the nonradiative combination centers in QD samples are much less than those in QW samples with the same In content. |
Author | 赵婉茹 翁国恩 梁明明 李增成 刘建平 张江勇 张保平 |
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Cites_doi | 10.1016/j.jcrysgro.2004.05.027 10.1063/1.2785135 10.1063/1.2800290 10.1063/1.3266520 10.1002/pssa.200674834 10.1038/35022529 10.1063/1.3596436 10.1088/0256-307X/31/7/076101 10.1063/1.122164 10.1116/1.590149 10.7567/APEX.7.025203 10.1143/JJAP.38.3976 10.1007/BF03353673 10.1063/1.3460921 10.1088/0256-307X/30/8/087101 10.1103/PhysRevB.32.8191 10.1063/1.1531837 10.1117/12.2007025 10.1063/1.4820935 10.1088/1674-1056/23/5/054211 10.1063/1.1381102 10.1016/j.jcrysgro.2008.06.077 10.1063/1.125444 10.1063/1.4754533 10.1063/1.1607521 10.1109/JQE.2013.2281062 10.1016/j.physe.2013.10.033 |
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Notes | 11-1959/O4 Emission properties of self-assembled green-emitting InGaN quantum dots (QDs) grown on sapphire substrates by using metal organic chemical vapor deposition are studied by temperature-dependent photoluminescence (PL) measurements. As temperature increases (15-300K), the PL peak energy shows an anomalous V-shaped (redshift blueshift) variation instead of an S-shaped (redshift-blueshift-redshift) variation, as observed typically in green-emitting InGaN/GaN multi-quantum wells (MOWs). The PL full width at half maximum (FWHM) also shows a V-shaped (decrease-increase) variation. The temperature dependence of the PL peak energy and FWHM of QDs are well explained by a model similar to MOWs, in which carriers transferring in localized states play an important role, while the confinement energy of localized states in the QDs is significantly larger than that in MOWs. By analyzing the integrated PL intensity, the larger confinement energy of localized states in the QDs is estimated to be 105.9meV, which is well explained by taking into account the band-gap shrinkage and carrier thermalization with temperature. It is also found that the nonradiative combination centers in QD samples are much less than those in QW samples with the same In content. ZHAO Wan-Ru, WENG Guo-En, LIANG Ming-Ming, LI Zeng-Cheng, LIU Jian-Ping, ZHANG Jiang-Yong,ZHANG Bao-Ping(1. Optoelectronics Engineering Research Center, Department of Electronic Engineering, Xiamen University, Xiamen 361005; 2.Department of Physics, Xiamen University, Xiamen 361005; 3.Suzhou Institute of Nano-tech and Nano-bionics, Chinese Academy of Sciences, Suzhou 215123) ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
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References | 22 23 25 26 27 Lv W B (18) 2014; 7 Mukai T (3) 1999; 38 Liang M M (21) 2014; 23 10 11 12 Ding L Z (24) 2014; 31 13 14 15 16 17 19 Zhang N (1) 2013; 30 2 4 5 6 7 8 9 20 |
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Snippet | Emission properties of self-assembled green-emitting InGaN quantum dots (QDs) grown on sapphire substrates by using metal organic chemical vapor deposition are... Emission properties of self-assembled green-emitting InGaN quantum dots (QDs) grown on sapphire substrates by using metal organic chemical vapor deposition are... |
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SubjectTerms | Carriers Confinement Emission Emission analysis Energy gaps (solid state) InGaN Photoluminescence Quantum dots Temperature dependence 发射性能 峰值能量 温度依赖性 绿色发光 自组装 量子点 金属有机化学气相沉积 |
Title | Temperature Dependence of Emission Properties of Self-Assembled InGaN Quantum Dots |
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