Liquid phase catalytic exchange column of water detritiation system: Steady-state modeling, simulation, and optimization
This paper presents a steady-state modeling, simulations, and optimization for an LPCE column of water detritiation system. It introduces a three-fluid model that integrates isotopic exchange, equilibrium-stage, and hydrodynamic models, considering energy balance and multiple feeds with adaptable fe...
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| Published in | Fusion engineering and design Vol. 200; p. 114222 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.03.2024
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| Subjects | |
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| Abstract | This paper presents a steady-state modeling, simulations, and optimization for an LPCE column of water detritiation system. It introduces a three-fluid model that integrates isotopic exchange, equilibrium-stage, and hydrodynamic models, considering energy balance and multiple feeds with adaptable feed location. The models were implemented in Pyomo, an equation-oriented, Python-based optimization modeling framework. Parametric studies are presented to analyze the effects on the detritiation factor and deuterium concentration resulting from changes in the gas to liquid feed mole ratio, gas feed composition, heat duty distribution, and gas feed location. Using the three most commonly employed catalysts, a design study investigates the minimal number of hypothetical stages required to meet the defined annual tritium discharge levels.
•A steady-state modeling for an LPCE column of water detritiation system.•Parametric studies on detritiation factor and deuterium concentration.•Design study to find minimal hypothetical stages for tritium discharge compliance. |
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| AbstractList | This paper presents a steady-state modeling, simulations, and optimization for an LPCE column of water detritiation system. It introduces a three-fluid model that integrates isotopic exchange, equilibrium-stage, and hydrodynamic models, considering energy balance and multiple feeds with adaptable feed location. The models were implemented in Pyomo, an equation-oriented, Python-based optimization modeling framework. Parametric studies are presented to analyze the effects on the detritiation factor and deuterium concentration resulting from changes in the gas to liquid feed mole ratio, gas feed composition, heat duty distribution, and gas feed location. Using the three most commonly employed catalysts, a design study investigates the minimal number of hypothetical stages required to meet the defined annual tritium discharge levels.
•A steady-state modeling for an LPCE column of water detritiation system.•Parametric studies on detritiation factor and deuterium concentration.•Design study to find minimal hypothetical stages for tritium discharge compliance. |
| ArticleNumber | 114222 |
| Author | Lee, Jae-Uk Chang, Min Ho Son, Yeong Woo Kwon, Gwanghyeon Lee, Jong Min Urm, Jae Jung |
| Author_xml | – sequence: 1 givenname: Yeong Woo orcidid: 0009-0007-6091-5703 surname: Son fullname: Son, Yeong Woo organization: School of Chemical and Biological Engineering, Seoul National University, 1 Gwanak-ro, Gwanak-gu, Seoul 08826, Republic of Korea – sequence: 2 givenname: Jae Jung orcidid: 0000-0002-3867-3206 surname: Urm fullname: Urm, Jae Jung organization: School of Chemical and Biological Engineering, Seoul National University, 1 Gwanak-ro, Gwanak-gu, Seoul 08826, Republic of Korea – sequence: 3 givenname: Gwanghyeon orcidid: 0009-0003-6805-9842 surname: Kwon fullname: Kwon, Gwanghyeon organization: School of Chemical and Biological Engineering, Seoul National University, 1 Gwanak-ro, Gwanak-gu, Seoul 08826, Republic of Korea – sequence: 4 givenname: Jae-Uk orcidid: 0000-0001-9386-8009 surname: Lee fullname: Lee, Jae-Uk organization: Korea Institute of Fusion Energy, 69-148 Gwahak-ro, Yuseong-gu, Daejeon 34133, Republic of Korea – sequence: 5 givenname: Min Ho orcidid: 0009-0006-1184-9466 surname: Chang fullname: Chang, Min Ho organization: Korea Institute of Fusion Energy, 69-148 Gwahak-ro, Yuseong-gu, Daejeon 34133, Republic of Korea – sequence: 6 givenname: Jong Min orcidid: 0000-0001-5395-0067 surname: Lee fullname: Lee, Jong Min email: jongmin@snu.ac.kr organization: School of Chemical and Biological Engineering, Seoul National University, 1 Gwanak-ro, Gwanak-gu, Seoul 08826, Republic of Korea |
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| Keywords | LPCE column Water detritiation system Steady-state simulation |
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| References | Spagnolo, Everatt, Seto, Chuang (b1) 1988; 14 de Koeijer, Rivero (b22) 2003; 58 Carillo, Martín, Roselló (b18) 2000; 23 Ovcharov, Rozenkevich, Perevezentsev (b3) 2009; 56 Bigeleisen (b10) 1961; 34 Palibroda (b2) 1966; 21 Van Hook (b11) 1968; 72 Bornea, Zamfirache, Ana, Stefan, Balteanu, Bucur (b5) 2020; 76 Bron, Chang, Wolfsberg (b12) 1973; 28 Boniface, Gnanapragasam, Ryland, Suppiah, Perevezentsev (b20) 2017; 71 Rabbani, Busigin, Mao, Halsey, La Barbera (b21) 2023 Busigin (b4) 2017; 71 Wächter, Biegler (b9) 2006; 106 Brad, Bilegan, Ana, Lazar, Vijulie (b19) 2014; 17 Tkachenko, Ovcharov, Rozenkevich (b7) 2017; 71 Wolf, Lehner, Hoffmann (b16) 2015 Urm, Park, Lee, Chang, Lee (b24) 2021; 172 Cristescu, Tamm, Cristescu, Glugla, Caldwell-Nichols (b14) 2002; 61 Hart, Laird, Watson, Woodruff, Hackebeil, Nicholson, Siirola (b8) 2017 Billet, Schultes (b6) 1999; 77 Ovcharov (b15) 2017; 71 Raghunathan, Diaz, Biegler (b17) 2004; 28 Sauar, Siragusa, Andresen (b23) 2001; 105 Butler, Rolston, Stevens (b13) 1978 Spagnolo (10.1016/j.fusengdes.2024.114222_b1) 1988; 14 Ovcharov (10.1016/j.fusengdes.2024.114222_b15) 2017; 71 Carillo (10.1016/j.fusengdes.2024.114222_b18) 2000; 23 de Koeijer (10.1016/j.fusengdes.2024.114222_b22) 2003; 58 Urm (10.1016/j.fusengdes.2024.114222_b24) 2021; 172 Wächter (10.1016/j.fusengdes.2024.114222_b9) 2006; 106 Boniface (10.1016/j.fusengdes.2024.114222_b20) 2017; 71 Bigeleisen (10.1016/j.fusengdes.2024.114222_b10) 1961; 34 Rabbani (10.1016/j.fusengdes.2024.114222_b21) 2023 Ovcharov (10.1016/j.fusengdes.2024.114222_b3) 2009; 56 Bornea (10.1016/j.fusengdes.2024.114222_b5) 2020; 76 Tkachenko (10.1016/j.fusengdes.2024.114222_b7) 2017; 71 Raghunathan (10.1016/j.fusengdes.2024.114222_b17) 2004; 28 Busigin (10.1016/j.fusengdes.2024.114222_b4) 2017; 71 Billet (10.1016/j.fusengdes.2024.114222_b6) 1999; 77 Bron (10.1016/j.fusengdes.2024.114222_b12) 1973; 28 Butler (10.1016/j.fusengdes.2024.114222_b13) 1978 Wolf (10.1016/j.fusengdes.2024.114222_b16) 2015 Van Hook (10.1016/j.fusengdes.2024.114222_b11) 1968; 72 Brad (10.1016/j.fusengdes.2024.114222_b19) 2014; 17 Hart (10.1016/j.fusengdes.2024.114222_b8) 2017 Palibroda (10.1016/j.fusengdes.2024.114222_b2) 1966; 21 Sauar (10.1016/j.fusengdes.2024.114222_b23) 2001; 105 Cristescu (10.1016/j.fusengdes.2024.114222_b14) 2002; 61 |
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Eng. doi: 10.1016/j.compchemeng.2004.03.015 contributor: fullname: Raghunathan – volume: 17 start-page: 65 issue: 1 year: 2014 ident: 10.1016/j.fusengdes.2024.114222_b19 article-title: Design and analysis method of the WDS tritiated water holding tanks publication-title: Smart Energy Sustain. Environ. contributor: fullname: Brad – volume: 172 year: 2021 ident: 10.1016/j.fusengdes.2024.114222_b24 article-title: Design study of a cryogenic distillation column for hydrogen isotope separation system publication-title: Fusion Eng. Des. doi: 10.1016/j.fusengdes.2021.112736 contributor: fullname: Urm – volume: 23 start-page: 425 issue: 5 year: 2000 ident: 10.1016/j.fusengdes.2024.114222_b18 article-title: A shortcut method for the estimation of structured packings HEPT in distillation publication-title: Chem. Eng. Technol.: Ind. Chem.-Plant Equip.-Process Eng.-Biotechnol. doi: 10.1002/(SICI)1521-4125(200005)23:5<425::AID-CEAT425>3.0.CO;2-8 contributor: fullname: Carillo – volume: 105 start-page: 2312 issue: 11 year: 2001 ident: 10.1016/j.fusengdes.2024.114222_b23 article-title: Equal thermodynamic distance and equipartition of forces principles applied to binary distillation publication-title: J. Phys. Chem. A doi: 10.1021/jp003555p contributor: fullname: Sauar – year: 2017 ident: 10.1016/j.fusengdes.2024.114222_b8 contributor: fullname: Hart – volume: 34 start-page: 1485 issue: 5 year: 1961 ident: 10.1016/j.fusengdes.2024.114222_b10 article-title: Statistical mechanics of isotope effects on the thermodynamic properties of condensed systems publication-title: J. Chem. Phys. doi: 10.1063/1.1701033 contributor: fullname: Bigeleisen – volume: 28 start-page: 129 issue: 2 year: 1973 ident: 10.1016/j.fusengdes.2024.114222_b12 article-title: Isotopic partition function ratios involving H2, H2O, H2S, H2Se, and NH3 publication-title: Z. Nat.forsch. A contributor: fullname: Bron – start-page: 93 year: 1978 ident: 10.1016/j.fusengdes.2024.114222_b13 article-title: Novel catalysts for isotopic exchange between hydrogen and liquid water contributor: fullname: Butler |
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| Title | Liquid phase catalytic exchange column of water detritiation system: Steady-state modeling, simulation, and optimization |
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