In Situ Synthesis of β-Na1.5Y1.5F6: Er3+ Crystals in Oxyfluoride Silicate Glass for Temperature Sensors and Their Spectral Conversion and Optical Thermometry Analysis
Transparent oxyfluoride glass-ceramics (GCs) with embedded β-Na1.5Y1.5F6 crystals doped with Er3+ ions were fabricated by a melt-quenching method with subsequent heat-treatment. The structural characterizations and spectroscopic techniques were performed to verify the precipitation of β-Na1.5Y1.5F6...
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Published in | Molecules (Basel, Switzerland) Vol. 26; no. 22; p. 6901 |
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Main Authors | , , , , |
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Abstract | Transparent oxyfluoride glass-ceramics (GCs) with embedded β-Na1.5Y1.5F6 crystals doped with Er3+ ions were fabricated by a melt-quenching method with subsequent heat-treatment. The structural characterizations and spectroscopic techniques were performed to verify the precipitation of β-Na1.5Y1.5F6 crystals and partition of the Er3+ dopant into the crystals. Bright green up-conversion (UC) emission was achieved in Er3+-doped glass-ceramic (Er-GC). Furthermore, the temperature-dependent visible UC behavior based on thermally coupled energy levels (TCLs) and non-thermally coupled energy levels (NTCLs) was also examined in the temperature range 298 k to 823 K with maximum relative sensitivity (Sr) of 1.1% K−1 at 298 K for TCLs in Er-G and Er-GC samples. |
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AbstractList | Transparent oxyfluoride glass-ceramics (GCs) with embedded β-Na1.5Y1.5F6 crystals doped with Er3+ ions were fabricated by a melt-quenching method with subsequent heat-treatment. The structural characterizations and spectroscopic techniques were performed to verify the precipitation of β-Na1.5Y1.5F6 crystals and partition of the Er3+ dopant into the crystals. Bright green up-conversion (UC) emission was achieved in Er3+-doped glass-ceramic (Er-GC). Furthermore, the temperature-dependent visible UC behavior based on thermally coupled energy levels (TCLs) and non-thermally coupled energy levels (NTCLs) was also examined in the temperature range 298 k to 823 K with maximum relative sensitivity (Sr) of 1.1% K-1 at 298 K for TCLs in Er-G and Er-GC samples. Transparent oxyfluoride glass-ceramics (GCs) with embedded β-Na1.5Y1.5F6 crystals doped with Er3+ ions were fabricated by a melt-quenching method with subsequent heat-treatment. The structural characterizations and spectroscopic techniques were performed to verify the precipitation of β-Na1.5Y1.5F6 crystals and partition of the Er3+ dopant into the crystals. Bright green up-conversion (UC) emission was achieved in Er3+-doped glass-ceramic (Er-GC). Furthermore, the temperature-dependent visible UC behavior based on thermally coupled energy levels (TCLs) and non-thermally coupled energy levels (NTCLs) was also examined in the temperature range 298 k to 823 K with maximum relative sensitivity (Sr) of 1.1% K−1 at 298 K for TCLs in Er-G and Er-GC samples. Transparent oxyfluoride glass-ceramics (GCs) with embedded β-Na 1 . 5 Y 1 . 5 F 6 crystals doped with Er 3+ ions were fabricated by a melt-quenching method with subsequent heat-treatment. The structural characterizations and spectroscopic techniques were performed to verify the precipitation of β-Na 1 . 5 Y 1 . 5 F 6 crystals and partition of the Er 3+ dopant into the crystals. Bright green up-conversion (UC) emission was achieved in Er 3+ -doped glass-ceramic (Er-GC). Furthermore, the temperature-dependent visible UC behavior based on thermally coupled energy levels (TCLs) and non-thermally coupled energy levels (NTCLs) was also examined in the temperature range 298 k to 823 K with maximum relative sensitivity ( S r ) of 1.1% K −1 at 298 K for TCLs in Er-G and Er-GC samples. |
Author | Rajavaram, Ramaraghavulu Velázquez, José J Galusek, Dušan Klement, Robert Dagupati, Rajesh |
AuthorAffiliation | 1 FunGlass, Alexander Dubček University of Trenčín, Študentská 2, SK-911 50 Trenčín, Slovakia; jose.velazquez@tnuni.sk (J.J.V.); dusan.galusek@tnuni.sk (D.G.) 3 Joint Glass Centre of the IIC SAS, TnUAD and FChPT STU, Trenčín, Študentská 2, SK-911 50 Trenčín, Slovakia 2 Department of Physics, Annamacharya Institute of Technology & Sciences, Rajampet A.P-516115, India; ramaraghavulu@gmail.com |
AuthorAffiliation_xml | – name: 3 Joint Glass Centre of the IIC SAS, TnUAD and FChPT STU, Trenčín, Študentská 2, SK-911 50 Trenčín, Slovakia – name: 1 FunGlass, Alexander Dubček University of Trenčín, Študentská 2, SK-911 50 Trenčín, Slovakia; jose.velazquez@tnuni.sk (J.J.V.); dusan.galusek@tnuni.sk (D.G.) – name: 2 Department of Physics, Annamacharya Institute of Technology & Sciences, Rajampet A.P-516115, India; ramaraghavulu@gmail.com |
Author_xml | – sequence: 1 givenname: Rajesh surname: Dagupati fullname: Dagupati, Rajesh – sequence: 2 givenname: Robert surname: Klement fullname: Klement, Robert – sequence: 3 givenname: Ramaraghavulu orcidid: 0000-0002-6616-8303 surname: Rajavaram fullname: Rajavaram, Ramaraghavulu – sequence: 4 givenname: José J. orcidid: 0000-0001-7672-0539 surname: Velázquez fullname: Velázquez, José J. – sequence: 5 givenname: Dušan orcidid: 0000-0001-5995-8780 surname: Galusek fullname: Galusek, Dušan |
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CitedBy_id | crossref_primary_10_3390_opt4010006 crossref_primary_10_1016_j_optmat_2023_114301 crossref_primary_10_1016_j_materresbull_2023_112256 crossref_primary_10_1016_j_matpr_2024_04_011 crossref_primary_10_1016_j_jlumin_2024_120627 crossref_primary_10_1111_ijag_16642 crossref_primary_10_1016_j_molliq_2024_125213 |
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Snippet | Transparent oxyfluoride glass-ceramics (GCs) with embedded β-Na1.5Y1.5F6 crystals doped with Er3+ ions were fabricated by a melt-quenching method with... Transparent oxyfluoride glass-ceramics (GCs) with embedded β-Na 1 . 5 Y 1 . 5 F 6 crystals doped with Er 3+ ions were fabricated by a melt-quenching method... |
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SubjectTerms | Ceramics Crystals down-conversion Energy Energy levels Fluorides glass Glass ceramics glass-ceramic Heat treatment optical thermometry Oxyfluorides Sensors Temperature dependence Temperature sensors Thermometry up-conversion |
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Title | In Situ Synthesis of β-Na1.5Y1.5F6: Er3+ Crystals in Oxyfluoride Silicate Glass for Temperature Sensors and Their Spectral Conversion and Optical Thermometry Analysis |
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