The entropy-controlled strategy in self-assembling systems

Self-assembly of various building blocks has been considered as a powerful approach to generate novel materials with tailorable structures and optimal properties. Understanding physicochemical interactions and mechanisms related to structural formation and transitions is of essential importance for...

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Published inChemical Society reviews Vol. 52; no. 19; pp. 686 - 6837
Main Authors Zhang, Xuanyu, Dai, Xiaobin, Gao, Lijuan, Xu, Duo, Wan, Haixiao, Wang, Yuming, Yan, Li-Tang
Format Journal Article
LanguageEnglish
Published London Royal Society of Chemistry 02.10.2023
Subjects
Entropy
Self-assembly
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Abstract Self-assembly of various building blocks has been considered as a powerful approach to generate novel materials with tailorable structures and optimal properties. Understanding physicochemical interactions and mechanisms related to structural formation and transitions is of essential importance for this approach. Although it is well-known that diverse forces and energies can significantly contribute to the structures and properties of self-assembling systems, the potential entropic contribution remains less well understood. The past few years have witnessed rapid progress in addressing the entropic effects on the structures, responses, and functions in the self-assembling systems, and many breakthroughs have been achieved. This review provides a framework regarding the entropy-controlled strategy of self-assembly, through which the structures and properties can be tailored by effectively tuning the entropic contribution and its interplay with the enthalpic counterpart. First, we focus on the fundamentals of entropy in thermodynamics and the entropy types that can be explored for self-assembly. Second, we discuss the rules of entropy in regulating the structural organization in self-assembly and delineate the entropic force and superentropic effect. Third, we introduce the basic principles, significance and approaches of the entropy-controlled strategy in self-assembly. Finally, we present the applications where this strategy has been employed in fields like colloids, macromolecular systems and nonequilibrium assembly. This review concludes with a discussion on future directions and future research opportunities for developing and applying the entropy-controlled strategy in complex self-assembling systems. The entropy-controlled strategy of self-assembly offers a conceptually new way to tune the ordering transitions in the development of designer systems and materials with controllable structures and optimal properties.
AbstractList Self-assembly of various building blocks has been considered as a powerful approach to generate novel materials with tailorable structures and optimal properties. Understanding physicochemical interactions and mechanisms related to structural formation and transitions is of essential importance for this approach. Although it is well-known that diverse forces and energies can significantly contribute to the structures and properties of self-assembling systems, the potential entropic contribution remains less well understood. The past few years have witnessed rapid progress in addressing the entropic effects on the structures, responses, and functions in the self-assembling systems, and many breakthroughs have been achieved. This review provides a framework regarding the entropy-controlled strategy of self-assembly, through which the structures and properties can be tailored by effectively tuning the entropic contribution and its interplay with the enthalpic counterpart. First, we focus on the fundamentals of entropy in thermodynamics and the entropy types that can be explored for self-assembly. Second, we discuss the rules of entropy in regulating the structural organization in self-assembly and delineate the entropic force and superentropic effect. Third, we introduce the basic principles, significance and approaches of the entropy-controlled strategy in self-assembly. Finally, we present the applications where this strategy has been employed in fields like colloids, macromolecular systems and nonequilibrium assembly. This review concludes with a discussion on future directions and future research opportunities for developing and applying the entropy-controlled strategy in complex self-assembling systems.Self-assembly of various building blocks has been considered as a powerful approach to generate novel materials with tailorable structures and optimal properties. Understanding physicochemical interactions and mechanisms related to structural formation and transitions is of essential importance for this approach. Although it is well-known that diverse forces and energies can significantly contribute to the structures and properties of self-assembling systems, the potential entropic contribution remains less well understood. The past few years have witnessed rapid progress in addressing the entropic effects on the structures, responses, and functions in the self-assembling systems, and many breakthroughs have been achieved. This review provides a framework regarding the entropy-controlled strategy of self-assembly, through which the structures and properties can be tailored by effectively tuning the entropic contribution and its interplay with the enthalpic counterpart. First, we focus on the fundamentals of entropy in thermodynamics and the entropy types that can be explored for self-assembly. Second, we discuss the rules of entropy in regulating the structural organization in self-assembly and delineate the entropic force and superentropic effect. Third, we introduce the basic principles, significance and approaches of the entropy-controlled strategy in self-assembly. Finally, we present the applications where this strategy has been employed in fields like colloids, macromolecular systems and nonequilibrium assembly. This review concludes with a discussion on future directions and future research opportunities for developing and applying the entropy-controlled strategy in complex self-assembling systems.
Self-assembly of various building blocks has been considered as a powerful approach to generate novel materials with tailorable structures and optimal properties. Understanding physicochemical interactions and mechanisms related to structural formation and transitions is of essential importance for this approach. Although it is well-known that diverse forces and energies can significantly contribute to the structures and properties of self-assembling systems, the potential entropic contribution remains less well understood. The past few years have witnessed rapid progress in addressing the entropic effects on the structures, responses, and functions in the self-assembling systems, and many breakthroughs have been achieved. This review provides a framework regarding the entropy-controlled strategy of self-assembly, through which the structures and properties can be tailored by effectively tuning the entropic contribution and its interplay with the enthalpic counterpart. First, we focus on the fundamentals of entropy in thermodynamics and the entropy types that can be explored for self-assembly. Second, we discuss the rules of entropy in regulating the structural organization in self-assembly and delineate the entropic force and superentropic effect. Third, we introduce the basic principles, significance and approaches of the entropy-controlled strategy in self-assembly. Finally, we present the applications where this strategy has been employed in fields like colloids, macromolecular systems and nonequilibrium assembly. This review concludes with a discussion on future directions and future research opportunities for developing and applying the entropy-controlled strategy in complex self-assembling systems.
Self-assembly of various building blocks has been considered as a powerful approach to generate novel materials with tailorable structures and optimal properties. Understanding physicochemical interactions and mechanisms related to structural formation and transitions is of essential importance for this approach. Although it is well-known that diverse forces and energies can significantly contribute to the structures and properties of self-assembling systems, the potential entropic contribution remains less well understood. The past few years have witnessed rapid progress in addressing the entropic effects on the structures, responses, and functions in the self-assembling systems, and many breakthroughs have been achieved. This review provides a framework regarding the entropy-controlled strategy of self-assembly, through which the structures and properties can be tailored by effectively tuning the entropic contribution and its interplay with the enthalpic counterpart. First, we focus on the fundamentals of entropy in thermodynamics and the entropy types that can be explored for self-assembly. Second, we discuss the rules of entropy in regulating the structural organization in self-assembly and delineate the entropic force and superentropic effect. Third, we introduce the basic principles, significance and approaches of the entropy-controlled strategy in self-assembly. Finally, we present the applications where this strategy has been employed in fields like colloids, macromolecular systems and nonequilibrium assembly. This review concludes with a discussion on future directions and future research opportunities for developing and applying the entropy-controlled strategy in complex self-assembling systems. The entropy-controlled strategy of self-assembly offers a conceptually new way to tune the ordering transitions in the development of designer systems and materials with controllable structures and optimal properties.
Author Dai, Xiaobin
Wan, Haixiao
Wang, Yuming
Yan, Li-Tang
Zhang, Xuanyu
Xu, Duo
Gao, Lijuan
AuthorAffiliation Department of Chemical Engineering
Tsinghua University
State Key Laboratory of Chemical Engineering
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Notes Xiaobin Dai is currently a fifth year PHD student at the Department of Chemical Engineering at Tsinghua University, working under Professor Li-Tang Yan. His research interests include diffusion and transport processes of nano-objects in macromolecular networks, self-assembly in polymer nanocomposites, and theoretical and computational biophysics.
Lijuan Gao received her BS in chemical engineering from Tsinghua University in 2020 and is currently a PhD student under the guidance of Prof. Li-Tang Yan at Tsinghua University in China. Her research focuses on the simulation and theoretical study of the self-assembly of colloidal particles under confinement.
Haixiao Wan received her BS degree in materials science and engineering from Zhengzhou University in 2016, and her PhD degree in materials science and engineering from Beijing University of Chemical Technology in 2021. She is currently working as a postdoc under the guidance of Prof. Li-Tang Yan at Tsinghua University. Her main research interests are focused on simulations and theoretical studies of polymer nanocomposites and nanoparticle cellular interactions.
Prof. Li-Tang Yan obtained his PhD in polymer physics and chemistry from Tsinghua University in 2007. Then he went to Bayreuth University in Germany with a Humboldt Research Fellowship. In 2010, he joined Prof. Anna Balazs' group at the University of Pittsburgh in USA as a postdoctoral research fellow. He returned to Tsinghua University as a faculty in the Department of Chemical Engineering in May 2011. In 2020, he obtained the "NSFC Award" for outstanding young scholar. His research interests focus on computational and theoretical aspects of soft matter systems, including nanoparticle cellular interactions and nano-engineer materials that are self-assembling and self-regulating.
Xuanyu Zhang received her BS in chemical engineering from Tianjin University in 2019 and is currently a fourth year PhD student under the guidance of Prof. Li-Tang Yan at Tsinghua University in China. Her research focuses on rod-like particle diffusion in macromolecular networks and nanoparticle diffusion in DNA dynamical networks.
Yuming Wang received his BS degree in Chemical Engineering from Tsinghua University in 2021 and is currently a PhD student under the guidance of Prof. Li-Tang Yan at Tsinghua University in China. His research focuses on the crystallization of hard spheres.
Duo Xu received her BS and PhD degrees from the College of Chemistry, Jilin University in 2015 and 2021. From 2014 to 2015, she studied at the University of California, Los Angles, as an exchange student for a year. She is currently working as a postdoc under the guidance of Prof. Li-Tang Yan at Tsinghua University. Her research interests are focused on simulations and theoretical studies of polymer and biomacromolecule systems in non-equilibrium states.
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PublicationDateYYYYMMDD 2023-10-02
PublicationDate_xml – month: 10
  year: 2023
  text: 2023-10-02
  day: 02
PublicationDecade 2020
PublicationPlace London
PublicationPlace_xml – name: London
PublicationTitle Chemical Society reviews
PublicationYear 2023
Publisher Royal Society of Chemistry
Publisher_xml – name: Royal Society of Chemistry
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Snippet Self-assembly of various building blocks has been considered as a powerful approach to generate novel materials with tailorable structures and optimal...
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SubjectTerms Entropy
Self-assembly
Title The entropy-controlled strategy in self-assembling systems
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