Recent advances in plasmon-enhanced Raman spectroscopy for catalytic reactions on bifunctional metallic nanostructures

Metallic nanostructures exhibit superior catalytic performance for diverse chemical reactions and the in-depth understanding of reaction mechanisms requires versatile characterization methods. Plasmon-enhanced Raman spectroscopy (PERS), including surface-enhanced Raman spectroscopy (SERS), shell-iso...

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Published inNanoscale Vol. 13; no. 33; pp. 13962 - 13975
Main Authors Su, Hai-Sheng, Feng, Hui-Shu, Wu, Xiang, Sun, Juan-Juan, Ren, Bin
Format Journal Article
LanguageEnglish
Published Cambridge Royal Society of Chemistry 07.09.2021
Subjects
Chemical reactions
Nanoparticles
Nanostructure
Raman spectroscopy
Reaction mechanisms
Spatial resolution
Spectrum analysis
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Abstract Metallic nanostructures exhibit superior catalytic performance for diverse chemical reactions and the in-depth understanding of reaction mechanisms requires versatile characterization methods. Plasmon-enhanced Raman spectroscopy (PERS), including surface-enhanced Raman spectroscopy (SERS), shell-isolated nanoparticle-enhanced Raman spectroscopy (SHINERS), and tip-enhanced Raman spectroscopy (TERS), appears as a powerful technique to characterize the Raman fingerprint information of surface species with high chemical sensitivity and spatial resolution. To expand the range of catalytic reactions studied by PERS, catalytically active metals are integrated with plasmonic metals to produce bifunctional metallic nanostructures. In this minireview, we discuss the recent advances in PERS techniques to probe the chemical reactions catalysed by bifunctional metallic nanostructures. First, we introduce different architectures of these dual-functionality nanostructures. We then highlight the recent works using PERS to investigate important catalytic reactions as well as the electronic and catalytic properties of these nanostructures. Finally, we provide some perspectives for future PERS studies in this field. This minireview provides a comprehensive discussion on recent advances in plasmon-enhanced Raman spectroscopy for catalytic reactions on bifunctional metallic nanostructures.
AbstractList Metallic nanostructures exhibit superior catalytic performance for diverse chemical reactions and the in-depth understanding of reaction mechanisms requires versatile characterization methods. Plasmon-enhanced Raman spectroscopy (PERS), including surface-enhanced Raman spectroscopy (SERS), shell-isolated nanoparticle-enhanced Raman spectroscopy (SHINERS), and tip-enhanced Raman spectroscopy (TERS), appears as a powerful technique to characterize the Raman fingerprint information of surface species with high chemical sensitivity and spatial resolution. To expand the range of catalytic reactions studied by PERS, catalytically active metals are integrated with plasmonic metals to produce bifunctional metallic nanostructures. In this minireview, we discuss the recent advances in PERS techniques to probe the chemical reactions catalysed by bifunctional metallic nanostructures. First, we introduce different architectures of these dual-functionality nanostructures. We then highlight the recent works using PERS to investigate important catalytic reactions as well as the electronic and catalytic properties of these nanostructures. Finally, we provide some perspectives for future PERS studies in this field.
Metallic nanostructures exhibit superior catalytic performance for diverse chemical reactions and the in-depth understanding of reaction mechanisms requires versatile characterization methods. Plasmon-enhanced Raman spectroscopy (PERS), including surface-enhanced Raman spectroscopy (SERS), shell-isolated nanoparticle-enhanced Raman spectroscopy (SHINERS), and tip-enhanced Raman spectroscopy (TERS), appears as a powerful technique to characterize the Raman fingerprint information of surface species with high chemical sensitivity and spatial resolution. To expand the range of catalytic reactions studied by PERS, catalytically active metals are integrated with plasmonic metals to produce bifunctional metallic nanostructures. In this minireview, we discuss the recent advances in PERS techniques to probe the chemical reactions catalysed by bifunctional metallic nanostructures. First, we introduce different architectures of these dual-functionality nanostructures. We then highlight the recent works using PERS to investigate important catalytic reactions as well as the electronic and catalytic properties of these nanostructures. Finally, we provide some perspectives for future PERS studies in this field. This minireview provides a comprehensive discussion on recent advances in plasmon-enhanced Raman spectroscopy for catalytic reactions on bifunctional metallic nanostructures.
Author Sun, Juan-Juan
Su, Hai-Sheng
Feng, Hui-Shu
Wu, Xiang
Ren, Bin
AuthorAffiliation State Key Laboratory of Physical Chemistry of Solid Surfaces
Xiamen University
Collaborative Innovation Center of Chemistry for Energy Materials (iChEM)
College of Chemistry and Chemical Engineering
AuthorAffiliation_xml – name: College of Chemistry and Chemical Engineering
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  givenname: Xiang
  surname: Wu
  fullname: Wu, Xiang
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  givenname: Juan-Juan
  surname: Sun
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  fullname: Ren, Bin
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Snippet Metallic nanostructures exhibit superior catalytic performance for diverse chemical reactions and the in-depth understanding of reaction mechanisms requires...
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SubjectTerms Chemical reactions
Nanoparticles
Nanostructure
Raman spectroscopy
Reaction mechanisms
Spatial resolution
Spectrum analysis
Title Recent advances in plasmon-enhanced Raman spectroscopy for catalytic reactions on bifunctional metallic nanostructures
URI https://www.proquest.com/docview/2564503618
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