Probing of Ultrafast Plasmon Dynamics on Gold Bowtie Nanostructure Using Photoemission Electron Microscopy

We report the direct imaging of plasmon on the tips pulses and probing of ultrafast plasmon dynamics by of nano-prisms in a bowtie structure excited by 7 fs laser combining the pump-probe technology with three-photon photoemission electron microscopy. Different photoemission patterns induced by the...

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Published inChinese physics letters Vol. 32; no. 6; pp. 61 - 65
Main Author 秦将 季博宇 郝作强 林景全
Format Journal Article
LanguageEnglish
Published 01.06.2015
Subjects
Dynamics
Electron microscopy
Excitation
Lasers
Nanostructure
Photoemission
Plasmons
Tips
光电
发射电子显微镜
泵浦-探测
直接成像
等离子体动力学
纳米结构
脉冲等离子体
飞秒激光脉冲
Online AccessGet full text
ISSN0256-307X
1741-3540
DOI10.1088/0256-307X/32/6/064202

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Abstract We report the direct imaging of plasmon on the tips pulses and probing of ultrafast plasmon dynamics by of nano-prisms in a bowtie structure excited by 7 fs laser combining the pump-probe technology with three-photon photoemission electron microscopy. Different photoemission patterns induced by the plasmon effect are observed when the bowties are excited by s- and p-polarized femtosecond laser pulses. A series of images of the evolution of local surface plasmon modes on different tips of the bowtie are obtained by the time-resolved three-photon photoemission electron microscopy, and the result discloses that plasmon excitation is dominated by the interfer- ence of the pump and probe pulses within the first 13 fs of the delay time, and thereafter the individual plasmon starts to oscillate on its own characteristic resonant frequencies.
AbstractList We report the direct imaging of plasmon on the tips of nano-prisms in a bowtie structure excited by 7fs laser pulses and probing of ultrafast plasmon dynamics by combining the pump-probe technology with three-photon photoemission electron microscopy. Different photoemission patterns induced by the plasmon effect are observed when the bowties are excited by s- and p-polarized femtosecond laser pulses. A series of images of the evolution of local surface plasmon modes on different tips of the bowtie are obtained by the time-resolved three-photon photoemission electron microscopy, and the result discloses that plasmon excitation is dominated by the interference of the pump and probe pulses within the first 13 fs of the delay time, and thereafter the individual plasmon starts to oscillate on its own characteristic resonant frequencies.
We report the direct imaging of plasmon on the tips pulses and probing of ultrafast plasmon dynamics by of nano-prisms in a bowtie structure excited by 7 fs laser combining the pump-probe technology with three-photon photoemission electron microscopy. Different photoemission patterns induced by the plasmon effect are observed when the bowties are excited by s- and p-polarized femtosecond laser pulses. A series of images of the evolution of local surface plasmon modes on different tips of the bowtie are obtained by the time-resolved three-photon photoemission electron microscopy, and the result discloses that plasmon excitation is dominated by the interfer- ence of the pump and probe pulses within the first 13 fs of the delay time, and thereafter the individual plasmon starts to oscillate on its own characteristic resonant frequencies.
Author 秦将 季博宇 郝作强 林景全
AuthorAffiliation School of Science, Changchun University of Science and Technology, Changchun 130022 International Research Center for Nano Handling and Manufacturing of China, Changchun 130022
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CitedBy_id crossref_primary_10_12677_APP_2020_101005
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QIN Jiang, JI Bo-Yu, HAO Zuo-Qiang, LIN Jing-Quan（1School of Science, Changchun University of Science and Technology, Changchun 130022 ;2International Research Center for Nano Handling and Manufacturing of China, Changchun 130022）
We report the direct imaging of plasmon on the tips pulses and probing of ultrafast plasmon dynamics by of nano-prisms in a bowtie structure excited by 7 fs laser combining the pump-probe technology with three-photon photoemission electron microscopy. Different photoemission patterns induced by the plasmon effect are observed when the bowties are excited by s- and p-polarized femtosecond laser pulses. A series of images of the evolution of local surface plasmon modes on different tips of the bowtie are obtained by the time-resolved three-photon photoemission electron microscopy, and the result discloses that plasmon excitation is dominated by the interfer- ence of the pump and probe pulses within the first 13 fs of the delay time, and thereafter the individual plasmon starts to oscillate on its own characteristic resonant frequencies.
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Snippet We report the direct imaging of plasmon on the tips pulses and probing of ultrafast plasmon dynamics by of nano-prisms in a bowtie structure excited by 7 fs...
We report the direct imaging of plasmon on the tips of nano-prisms in a bowtie structure excited by 7fs laser pulses and probing of ultrafast plasmon dynamics...
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StartPage 61
SubjectTerms Dynamics
Electron microscopy
Excitation
Lasers
Nanostructure
Photoemission
Plasmons
Tips
光电
发射电子显微镜
泵浦-探测
直接成像
等离子体动力学
纳米结构
脉冲等离子体
飞秒激光脉冲
Title Probing of Ultrafast Plasmon Dynamics on Gold Bowtie Nanostructure Using Photoemission Electron Microscopy
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