Steam reforming of methane over nickel-aluminum spinel-derived catalyst
Despite steam reforming of methane (SRM) has been the dominant way to produce hydrogen in industrial owing to its large hydrogen production capacity, easy accessibility of feedstocks and relative low cost, the development of high-efficient catalysts is still of great significance. In this work, we r...
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| Published in | International journal of hydrogen energy Vol. 51; pp. 1256 - 1266 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
02.01.2024
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| Abstract | Despite steam reforming of methane (SRM) has been the dominant way to produce hydrogen in industrial owing to its large hydrogen production capacity, easy accessibility of feedstocks and relative low cost, the development of high-efficient catalysts is still of great significance. In this work, we report the synthesis, characterizations and evaluation of Nickel-aluminum spinel (NiAl2O4) catalyst in SRM reaction. Compared with Ni/γ-Al2O3 catalyst prepared by impregnation, NiAl2O4 presents higher methane conversion. Virous of characterizations exhibit NiAl2O4 possesses higher distribution of Ni and smaller Ni nanoparticle size, which is one of advantages for its high activity. Another vital reason is the generation of oxygen vacancies in spinel during the reduction, which is beneficial for the activation of water. Moreover, NiAl2O4 catalyst shows extremely stability without obvious deactivation in 160 h. This study illustrates that the construction of catalyst with high activity and stability via NiAl2O4 spinel and reals its high activity origination.
•NiAl2O4 spinel shows excellent activity and stability in methane steam reforming.•NiAl2O4 spinel catalyst presents better distribution of Ni comparing with Ni/Al2O3.•The abundant oxygen vacancies in NiAl2O4 play a vital role on activating water. |
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| AbstractList | Despite steam reforming of methane (SRM) has been the dominant way to produce hydrogen in industrial owing to its large hydrogen production capacity, easy accessibility of feedstocks and relative low cost, the development of high-efficient catalysts is still of great significance. In this work, we report the synthesis, characterizations and evaluation of Nickel-aluminum spinel (NiAl2O4) catalyst in SRM reaction. Compared with Ni/γ-Al2O3 catalyst prepared by impregnation, NiAl2O4 presents higher methane conversion. Virous of characterizations exhibit NiAl2O4 possesses higher distribution of Ni and smaller Ni nanoparticle size, which is one of advantages for its high activity. Another vital reason is the generation of oxygen vacancies in spinel during the reduction, which is beneficial for the activation of water. Moreover, NiAl2O4 catalyst shows extremely stability without obvious deactivation in 160 h. This study illustrates that the construction of catalyst with high activity and stability via NiAl2O4 spinel and reals its high activity origination.
•NiAl2O4 spinel shows excellent activity and stability in methane steam reforming.•NiAl2O4 spinel catalyst presents better distribution of Ni comparing with Ni/Al2O3.•The abundant oxygen vacancies in NiAl2O4 play a vital role on activating water. |
| Author | Ding, Xi Yang, Yunfeng Wang, Yanqin Li, Bing Liu, Xiaohui Guo, Yong |
| Author_xml | – sequence: 1 givenname: Xi surname: Ding fullname: Ding, Xi organization: State Key Laboratory of Green Chemical Engineering and Industrial Catalysis, School of Chemistry and Molecular Engineering, East China University of Science and Technology, Shanghai 200237, PR China – sequence: 2 givenname: Bing surname: Li fullname: Li, Bing organization: Shanghai Institute of Quality Inspection and Technical Research, No.381, Cangwu Rd, Shanghai 200233, PR China – sequence: 3 givenname: Yunfeng surname: Yang fullname: Yang, Yunfeng organization: State Key Laboratory of Green Chemical Engineering and Industrial Catalysis, School of Chemistry and Molecular Engineering, East China University of Science and Technology, Shanghai 200237, PR China – sequence: 4 givenname: Xiaohui surname: Liu fullname: Liu, Xiaohui organization: State Key Laboratory of Green Chemical Engineering and Industrial Catalysis, School of Chemistry and Molecular Engineering, East China University of Science and Technology, Shanghai 200237, PR China – sequence: 5 givenname: Yong orcidid: 0000-0002-5104-2732 surname: Guo fullname: Guo, Yong email: guoyong@ecust.edu.cn organization: State Key Laboratory of Green Chemical Engineering and Industrial Catalysis, School of Chemistry and Molecular Engineering, East China University of Science and Technology, Shanghai 200237, PR China – sequence: 6 givenname: Yanqin surname: Wang fullname: Wang, Yanqin organization: State Key Laboratory of Green Chemical Engineering and Industrial Catalysis, School of Chemistry and Molecular Engineering, East China University of Science and Technology, Shanghai 200237, PR China |
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| Keywords | NiAl2O4 spinel Steam reforming of methane Hydrogen production Oxygen vacancy |
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