Photoelectric properties of monolayer WS2-MoS2 lateral heterojunction from first principles
•The photocurrent of monolayer WS2-MoS2 lateral heterojunction is investigated by using the first principle method.•CPGE is generally similar LPGE for monolayer WS2-MoS2 lateral heterojunction.•The peaks of photoresponse occur at photon energies of 2.0 eV and 2.3 eV for both LPGE and CPGE. The first...
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| Published in | Physics letters. A Vol. 420; p. 127771 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
30.12.2021
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0375-9601 1873-2429 |
| DOI | 10.1016/j.physleta.2021.127771 |
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| Abstract | •The photocurrent of monolayer WS2-MoS2 lateral heterojunction is investigated by using the first principle method.•CPGE is generally similar LPGE for monolayer WS2-MoS2 lateral heterojunction.•The peaks of photoresponse occur at photon energies of 2.0 eV and 2.3 eV for both LPGE and CPGE.
The first-principles calculation is applied to investigate the photocurrents elicited by the circular photogalvanic effect (CPGE) and linear photogalvanic effect (LPGE) of monolayer WS2-MoS2 lateral heterojunction. Our results demonstrate that the band alignment of the WS2-MoS2 lateral heterojunction belongs to type-II, which can effectually isolate electron-hole pairs and augment the photocurrent conversion rate of the heterojunction. Furthermore, the photocurrent generated by LPGE and CPGE both have peaks around the photon energy of 2.0 eV and 2.3 eV, which can be subject to explain by DOS via Fermi's Golden Rule. More importantly, the monolayer WS2-MoS2 lateral heterojunction exhibits an obvious photocurrent effect, which also attest the existence of the PN junction. These results will contribute some theoretical guidance for the application of the WS2-MoS2 lateral heterojunction in the area of optoelectronics. |
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| AbstractList | •The photocurrent of monolayer WS2-MoS2 lateral heterojunction is investigated by using the first principle method.•CPGE is generally similar LPGE for monolayer WS2-MoS2 lateral heterojunction.•The peaks of photoresponse occur at photon energies of 2.0 eV and 2.3 eV for both LPGE and CPGE.
The first-principles calculation is applied to investigate the photocurrents elicited by the circular photogalvanic effect (CPGE) and linear photogalvanic effect (LPGE) of monolayer WS2-MoS2 lateral heterojunction. Our results demonstrate that the band alignment of the WS2-MoS2 lateral heterojunction belongs to type-II, which can effectually isolate electron-hole pairs and augment the photocurrent conversion rate of the heterojunction. Furthermore, the photocurrent generated by LPGE and CPGE both have peaks around the photon energy of 2.0 eV and 2.3 eV, which can be subject to explain by DOS via Fermi's Golden Rule. More importantly, the monolayer WS2-MoS2 lateral heterojunction exhibits an obvious photocurrent effect, which also attest the existence of the PN junction. These results will contribute some theoretical guidance for the application of the WS2-MoS2 lateral heterojunction in the area of optoelectronics. |
| ArticleNumber | 127771 |
| Author | Liu, Ping-Ping Luo, Wen-Ming Shao, Zhi-Gang Yang, Mou Li, Han-Bing |
| Author_xml | – sequence: 1 givenname: Ping-Ping surname: Liu fullname: Liu, Ping-Ping organization: Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials, Guangdong Engineering Technology Research Center of Efficient Green Energy and Environment Protection Materials, SPTE, South China Normal University, Guangzhou 510006, China – sequence: 2 givenname: Zhi-Gang orcidid: 0000-0002-1639-7597 surname: Shao fullname: Shao, Zhi-Gang email: zgshao@scnu.edu.cn organization: Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials, Guangdong Engineering Technology Research Center of Efficient Green Energy and Environment Protection Materials, SPTE, South China Normal University, Guangzhou 510006, China – sequence: 3 givenname: Wen-Ming surname: Luo fullname: Luo, Wen-Ming organization: Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials, Guangdong Engineering Technology Research Center of Efficient Green Energy and Environment Protection Materials, SPTE, South China Normal University, Guangzhou 510006, China – sequence: 4 givenname: Han-Bing surname: Li fullname: Li, Han-Bing organization: Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials, Guangdong Engineering Technology Research Center of Efficient Green Energy and Environment Protection Materials, SPTE, South China Normal University, Guangzhou 510006, China – sequence: 5 givenname: Mou surname: Yang fullname: Yang, Mou organization: Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials, Guangdong Engineering Technology Research Center of Efficient Green Energy and Environment Protection Materials, SPTE, South China Normal University, Guangzhou 510006, China |
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