Superhydrophobic PDMS@PEI-cCNTs wood with Joule heat and demulsification capability for oil-water emulsion separation

Superhydrophobic materials possess prospective applications of oily wastewater treatment due to their high efficiency and easy operation. Nevertheless, most superhydrophobic materials are difficult to separate oil-water emulsion, especially for highly viscous water-in-crude oil emulsion. Herein, a s...

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Published inProgress in organic coatings Vol. 185; p. 107960
Main Authors Chen, Zhuohan, Su, Xiaojing, Li, Kunquan, Chen, Rongxuan, Lai, Zhixuan, Li, Xuanjun, Chen, Shengye, Wu, Wenjian
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.12.2023
Subjects
Compressibility
Demulsification
Joule heat
Superhydrophobic wood
Water-in-crude oil emulsion separation
Water-in-crude oil emulsion separation
Superhydrophobic wood
Joule heat
Compressibility
Demulsification
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Abstract Superhydrophobic materials possess prospective applications of oily wastewater treatment due to their high efficiency and easy operation. Nevertheless, most superhydrophobic materials are difficult to separate oil-water emulsion, especially for highly viscous water-in-crude oil emulsion. Herein, a superhydrophobic wood with excellent Joule heat and demulsification was proposed by chemically treating the natural wood and subsequent coating of the carboxyl-modified carbon nanotubes (cCNTs) for providing conductive pathways, polyethylenimide (PEI) for supporting demulsification and polydimethylsiloxane (PDMS) for hydrophobic modification. The fabricated superhydrophobic PDMS@PEI-cCNTs wood displayed a water contact angle of 155o and great compression property with a nearly undamaged structure at a strain of 40 % after 50 compression tests, which could separate and recover oil from the oil-water mixture via absorption-extrusion process. Besides, due to the filtration and electrostatic interaction of the PDMS@PEI-cCNTs wood, the water-in-oil emulsion was demulsified quickly with a separation efficiency greater than 99.7 %. Meanwhile, the PDMS@PEI-cCNTs wood showed a good Joule heat capability, and the surface temperature reached 160 °C at 35 V of voltage within 120 s, which largely reduced the viscosity of water-in-crude oil emulsion. Thus, the PDMS@PEI-cCNTs wood was successful in separating the water-in-crude oil emulsion via Joule heat capability with a separation rate of 4.33 × 104 kg·m−3·h−1 and a separation efficiency of 93.4 %. The material developed in this study has wide range of applications in treating the stable crude oil-water emulsion with high viscosity. [Display omitted] •A new strategy for fabricating superhydrophobic wood for various oil-water emulsions separation is proposed.•The wood presents stable superhydrophobicity and good electrical conductivity.•The wood shows excellent demulsification capability via charge action, absorption and gathering.•The wood exhibits great Joule heat to promote separating viscous water-in-crude oil emulsion.
AbstractList Superhydrophobic materials possess prospective applications of oily wastewater treatment due to their high efficiency and easy operation. Nevertheless, most superhydrophobic materials are difficult to separate oil-water emulsion, especially for highly viscous water-in-crude oil emulsion. Herein, a superhydrophobic wood with excellent Joule heat and demulsification was proposed by chemically treating the natural wood and subsequent coating of the carboxyl-modified carbon nanotubes (cCNTs) for providing conductive pathways, polyethylenimide (PEI) for supporting demulsification and polydimethylsiloxane (PDMS) for hydrophobic modification. The fabricated superhydrophobic PDMS@PEI-cCNTs wood displayed a water contact angle of 155o and great compression property with a nearly undamaged structure at a strain of 40 % after 50 compression tests, which could separate and recover oil from the oil-water mixture via absorption-extrusion process. Besides, due to the filtration and electrostatic interaction of the PDMS@PEI-cCNTs wood, the water-in-oil emulsion was demulsified quickly with a separation efficiency greater than 99.7 %. Meanwhile, the PDMS@PEI-cCNTs wood showed a good Joule heat capability, and the surface temperature reached 160 °C at 35 V of voltage within 120 s, which largely reduced the viscosity of water-in-crude oil emulsion. Thus, the PDMS@PEI-cCNTs wood was successful in separating the water-in-crude oil emulsion via Joule heat capability with a separation rate of 4.33 × 104 kg·m−3·h−1 and a separation efficiency of 93.4 %. The material developed in this study has wide range of applications in treating the stable crude oil-water emulsion with high viscosity. [Display omitted] •A new strategy for fabricating superhydrophobic wood for various oil-water emulsions separation is proposed.•The wood presents stable superhydrophobicity and good electrical conductivity.•The wood shows excellent demulsification capability via charge action, absorption and gathering.•The wood exhibits great Joule heat to promote separating viscous water-in-crude oil emulsion.
ArticleNumber 107960
Author Wu, Wenjian
Chen, Shengye
Su, Xiaojing
Lai, Zhixuan
Chen, Rongxuan
Li, Xuanjun
Chen, Zhuohan
Li, Kunquan
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Keywords Water-in-crude oil emulsion separation
Superhydrophobic wood
Joule heat
Compressibility
Demulsification
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– volume: 26
  start-page: 101424
  year: 2021
  ident: 10.1016/j.porgcoat.2023.107960_bb0175
  article-title: The three-line synergistic icephobicity of conductive CNTs/PDMS nanocomposite with bio-inspired hierarchical surface
  publication-title: Surf. Interfaces
  doi: 10.1016/j.surfin.2021.101424
  contributor:
    fullname: Wang
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Snippet Superhydrophobic materials possess prospective applications of oily wastewater treatment due to their high efficiency and easy operation. Nevertheless, most...
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StartPage 107960
SubjectTerms Compressibility
Demulsification
Joule heat
Superhydrophobic wood
Water-in-crude oil emulsion separation
Title Superhydrophobic PDMS@PEI-cCNTs wood with Joule heat and demulsification capability for oil-water emulsion separation
URI https://dx.doi.org/10.1016/j.porgcoat.2023.107960
Volume 185
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