Molybdate-intercalated NiMn layered double hydroxide nanoarrays supercapacitor electrode with enhanced stability via a differentiated deposition strategy
Nickel-manganese layered double hydroxide (NiMn-LDH) is a promising electrode material for supercapacitor due to its unique two-dimensional (2D) layered structure, adjustable interlayer spacing, tailorable chemical valences, and ion exchange ability. However, NiMn-LDH still suffers from poor conduct...
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| Published in | Journal of power sources Vol. 594; p. 233990 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
28.02.2024
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| Abstract | Nickel-manganese layered double hydroxide (NiMn-LDH) is a promising electrode material for supercapacitor due to its unique two-dimensional (2D) layered structure, adjustable interlayer spacing, tailorable chemical valences, and ion exchange ability. However, NiMn-LDH still suffers from poor conductivity and low cyclic stability during the charge/discharge process. In this work, NiMn-LDH nanoarrays are grown on a carbon cloth substrate using a novel differentiated solvo/hydrothermal deposition strategy, in which molybdate anions act as precipitators during the second-step deposition and also as intercalated anions in the gallery of NiMn-LDH. The molybdate-intercalated NiMn-LDH nanoarray consists of open channels that allow electrolyte access and interconnected nanosheets decorated with tiny nanoflakes, and exhibits a high capacitance of 1712 F g−1 at 1 A g−1 with good cyclic performance, retaining 94.4 % of its capacitance after 8,000 charge/discharge cycles. The as-assembled NiMn-LDH//activated carbon hybrid supercapacitor delivers a high specific capacitance of 148.4 F g−1 at 1 A g−1, and achieves a high energy density of 66.8 Wh kg−1 at a power density of 900 W kg−1 with an excellent cycle stability (96.6 % capacitance maintained after 12,000 cycles).
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•Molybdate as precipitator and intercalated anions for differentiated deposition.•NiMn-LDH nanoarray comprises open channels for effective electrolyte access.•Nanosheets decorated with tiny nanoflakes for enhanced accessible surface area.•Molybdate-intercalated NiMn-LDH shows the capacitance of 1712 F g−1 at 1 A g−1.•All-solid-state asymmetric supercapacitor delivers 66.8 Wh kg−1 at 900 W kg−1. |
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| AbstractList | Nickel-manganese layered double hydroxide (NiMn-LDH) is a promising electrode material for supercapacitor due to its unique two-dimensional (2D) layered structure, adjustable interlayer spacing, tailorable chemical valences, and ion exchange ability. However, NiMn-LDH still suffers from poor conductivity and low cyclic stability during the charge/discharge process. In this work, NiMn-LDH nanoarrays are grown on a carbon cloth substrate using a novel differentiated solvo/hydrothermal deposition strategy, in which molybdate anions act as precipitators during the second-step deposition and also as intercalated anions in the gallery of NiMn-LDH. The molybdate-intercalated NiMn-LDH nanoarray consists of open channels that allow electrolyte access and interconnected nanosheets decorated with tiny nanoflakes, and exhibits a high capacitance of 1712 F g−1 at 1 A g−1 with good cyclic performance, retaining 94.4 % of its capacitance after 8,000 charge/discharge cycles. The as-assembled NiMn-LDH//activated carbon hybrid supercapacitor delivers a high specific capacitance of 148.4 F g−1 at 1 A g−1, and achieves a high energy density of 66.8 Wh kg−1 at a power density of 900 W kg−1 with an excellent cycle stability (96.6 % capacitance maintained after 12,000 cycles).
[Display omitted]
•Molybdate as precipitator and intercalated anions for differentiated deposition.•NiMn-LDH nanoarray comprises open channels for effective electrolyte access.•Nanosheets decorated with tiny nanoflakes for enhanced accessible surface area.•Molybdate-intercalated NiMn-LDH shows the capacitance of 1712 F g−1 at 1 A g−1.•All-solid-state asymmetric supercapacitor delivers 66.8 Wh kg−1 at 900 W kg−1. |
| ArticleNumber | 233990 |
| Author | Tang, Tingfu Liang, Yifan Zeng, Lei Xu, Xuetang Wang, Fan Jiang, Shiwen |
| Author_xml | – sequence: 1 givenname: Lei surname: Zeng fullname: Zeng, Lei – sequence: 2 givenname: Tingfu surname: Tang fullname: Tang, Tingfu – sequence: 3 givenname: Yifan surname: Liang fullname: Liang, Yifan – sequence: 4 givenname: Shiwen surname: Jiang fullname: Jiang, Shiwen – sequence: 5 givenname: Xuetang surname: Xu fullname: Xu, Xuetang email: xxtang@gxu.edu.cn – sequence: 6 givenname: Fan orcidid: 0000-0002-6106-4724 surname: Wang fullname: Wang, Fan email: fanwang@gxu.edu.cn |
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