Polyepitaxial grain matching to study the oxidation of uranium dioxide

Although the principal physical behaviour of a material is inherently connected to its fundamental crystal structure, the behaviours observed in the real-world are often driven by the microstructure, which for many polycrystalline materials, equates to the size and shape of the constituent crystal g...

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Published inNpj Materials degradation Vol. 8; no. 1; pp. 68 - 6
Main Authors Wasik, Jacek, Sutcliffe, Joseph, Podor, Renaud, Lewis, Jarrod, Darnbrough, James Edward, Rennie, Sophie, Akbar Hussain, Syed, Bell, Christopher, Chaney, Daniel Alexander, Griffiths, Gareth, Harding, Lottie Mae, Legg, Florence, Lawrence Bright, Eleanor, Nicholls, Rebecca, Sasikumar, Yadukrishnan, Siberry, Angus, Smith, Philip, Springell, Ross
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 11.07.2024
Nature Publishing Group
Nature Portfolio
Subjects
639/301/119/544
639/301/299/892
639/925/357/1018
639/925/357/551
Chemistry and Materials Science
Corrosion and Coatings
Crystal structure
Electrochemistry
Grain size
High temperature
Investigations
Laboratories
Materials Science
Nuclear fission
Nuclear fuels
Oxidation
Phase transitions
Structural Materials
Synthesis
Thin films
Tribology
Uranium
Uranium dioxide
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Abstract Although the principal physical behaviour of a material is inherently connected to its fundamental crystal structure, the behaviours observed in the real-world are often driven by the microstructure, which for many polycrystalline materials, equates to the size and shape of the constituent crystal grains. Here we highlight a cutting edge synthesis route to the controlled engineering of grain structures in thin films and the simplification of associated 3-dimensional problems to less complex 2D ones. This has been applied to the actinide ceramic, uranium dioxide, to replicate structures typical in nuclear fission fuel pellets, in order to investigate the oxidation and subsequent transformation of cubic UO 2 to orthorhombic U 3 O 8 . This article shows how this synthesis approach could be utilised to investigate a range of phenomena, affected by grain morphology, and highlights some unusual results in the oxidation behaviour of UO 2 , regarding the phase transition to U 3 O 8 .
AbstractList Although the principal physical behaviour of a material is inherently connected to its fundamental crystal structure, the behaviours observed in the real-world are often driven by the microstructure, which for many polycrystalline materials, equates to the size and shape of the constituent crystal grains. Here we highlight a cutting edge synthesis route to the controlled engineering of grain structures in thin films and the simplification of associated 3-dimensional problems to less complex 2D ones. This has been applied to the actinide ceramic, uranium dioxide, to replicate structures typical in nuclear fission fuel pellets, in order to investigate the oxidation and subsequent transformation of cubic UO 2 to orthorhombic U 3 O 8 . This article shows how this synthesis approach could be utilised to investigate a range of phenomena, affected by grain morphology, and highlights some unusual results in the oxidation behaviour of UO 2 , regarding the phase transition to U 3 O 8 .
Abstract Although the principal physical behaviour of a material is inherently connected to its fundamental crystal structure, the behaviours observed in the real-world are often driven by the microstructure, which for many polycrystalline materials, equates to the size and shape of the constituent crystal grains. Here we highlight a cutting edge synthesis route to the controlled engineering of grain structures in thin films and the simplification of associated 3-dimensional problems to less complex 2D ones. This has been applied to the actinide ceramic, uranium dioxide, to replicate structures typical in nuclear fission fuel pellets, in order to investigate the oxidation and subsequent transformation of cubic UO 2 to orthorhombic U 3 O 8 . This article shows how this synthesis approach could be utilised to investigate a range of phenomena, affected by grain morphology, and highlights some unusual results in the oxidation behaviour of UO 2 , regarding the phase transition to U 3 O 8 .
Although the principal physical behaviour of a material is inherently connected to its fundamental crystal structure, the behaviours observed in the real-world are often driven by the microstructure, which for many polycrystalline materials, equates to the size and shape of the constituent crystal grains. Here we highlight a cutting edge synthesis route to the controlled engineering of grain structures in thin films and the simplification of associated 3-dimensional problems to less complex 2D ones. This has been applied to the actinide ceramic, uranium dioxide, to replicate structures typical in nuclear fission fuel pellets, in order to investigate the oxidation and subsequent transformation of cubic UO2 to orthorhombic U3O8. This article shows how this synthesis approach could be utilised to investigate a range of phenomena, affected by grain morphology, and highlights some unusual results in the oxidation behaviour of UO2, regarding the phase transition to U3O8.
Abstract Although the principal physical behaviour of a material is inherently connected to its fundamental crystal structure, the behaviours observed in the real-world are often driven by the microstructure, which for many polycrystalline materials, equates to the size and shape of the constituent crystal grains. Here we highlight a cutting edge synthesis route to the controlled engineering of grain structures in thin films and the simplification of associated 3-dimensional problems to less complex 2D ones. This has been applied to the actinide ceramic, uranium dioxide, to replicate structures typical in nuclear fission fuel pellets, in order to investigate the oxidation and subsequent transformation of cubic UO2 to orthorhombic U3O8. This article shows how this synthesis approach could be utilised to investigate a range of phenomena, affected by grain morphology, and highlights some unusual results in the oxidation behaviour of UO2, regarding the phase transition to U3O8.
ArticleNumber 68
Author Lawrence Bright, Eleanor
Legg, Florence
Bell, Christopher
Akbar Hussain, Syed
Darnbrough, James Edward
Griffiths, Gareth
Nicholls, Rebecca
Chaney, Daniel Alexander
Harding, Lottie Mae
Rennie, Sophie
Smith, Philip
Wasik, Jacek
Siberry, Angus
Springell, Ross
Podor, Renaud
Sutcliffe, Joseph
Lewis, Jarrod
Sasikumar, Yadukrishnan
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Snippet Although the principal physical behaviour of a material is inherently connected to its fundamental crystal structure, the behaviours observed in the real-world...
Abstract Although the principal physical behaviour of a material is inherently connected to its fundamental crystal structure, the behaviours observed in the...
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SubjectTerms 639/301/119/544
639/301/299/892
639/925/357/1018
639/925/357/551
Chemistry and Materials Science
Corrosion and Coatings
Crystal structure
Electrochemistry
Grain size
High temperature
Investigations
Laboratories
Materials Science
Nuclear fission
Nuclear fuels
Oxidation
Phase transitions
Structural Materials
Synthesis
Thin films
Tribology
Uranium
Uranium dioxide
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Title Polyepitaxial grain matching to study the oxidation of uranium dioxide
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