Photoelectron marginalization effect in ZnO/WO3/graphene-like composites: Study of alternating strong-low photocatalytic hydrogen production performance and mechanism
ZnO/WO3/graphene-like composite photocatalysts are prepared by in-situ deposition and successfully utilized for alternating strong-low light catalytic decomposition of water to produce hydrogen. Additionally, the study details the microscopic morphology and optoelectronic properties of the ZnO/WO3/g...
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| Published in | Journal of alloys and compounds Vol. 1009; p. 176824 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
25.12.2024
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| Abstract | ZnO/WO3/graphene-like composite photocatalysts are prepared by in-situ deposition and successfully utilized for alternating strong-low light catalytic decomposition of water to produce hydrogen. Additionally, the study details the microscopic morphology and optoelectronic properties of the ZnO/WO3/graphene-like composite. The results indicate that an internal electric field is generated between the ZnO/WO3 heterostructure and the graphene-like material. This induced electric field leads to a large amount of ordered electron transfer from ZnO/WO3 to the graphene-like material, resulting in the electron marginalization effect, which ensures the prerequisite for alternating strong-low photocatalytic splitting of water into hydrogen. When the mass fraction of the graphene-like material in the WO3/ZnO/graphene-like composite photocatalyst is 30 %, the photocatalytic hydrogen production rate reaches the maximum value of 820 times that of intrinsic ZnO. Therefore, this work provides a new perspective for alternating strong-low light catalytic water splitting to produce hydrogen.
•WO3/ZnO graphene-like composite is successfully prepared.•WO3/ZnO graphene-like hydrogen rate is 1025 μmol·h−1·g−1 with strong-low light.•Mechanism of hydrogen production under strong-low light irradiation is analyzed.•Conducting photogenerated electrons in graphene like materials is analyzed. |
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| AbstractList | ZnO/WO3/graphene-like composite photocatalysts are prepared by in-situ deposition and successfully utilized for alternating strong-low light catalytic decomposition of water to produce hydrogen. Additionally, the study details the microscopic morphology and optoelectronic properties of the ZnO/WO3/graphene-like composite. The results indicate that an internal electric field is generated between the ZnO/WO3 heterostructure and the graphene-like material. This induced electric field leads to a large amount of ordered electron transfer from ZnO/WO3 to the graphene-like material, resulting in the electron marginalization effect, which ensures the prerequisite for alternating strong-low photocatalytic splitting of water into hydrogen. When the mass fraction of the graphene-like material in the WO3/ZnO/graphene-like composite photocatalyst is 30 %, the photocatalytic hydrogen production rate reaches the maximum value of 820 times that of intrinsic ZnO. Therefore, this work provides a new perspective for alternating strong-low light catalytic water splitting to produce hydrogen.
•WO3/ZnO graphene-like composite is successfully prepared.•WO3/ZnO graphene-like hydrogen rate is 1025 μmol·h−1·g−1 with strong-low light.•Mechanism of hydrogen production under strong-low light irradiation is analyzed.•Conducting photogenerated electrons in graphene like materials is analyzed. |
| ArticleNumber | 176824 |
| Author | Yunlong, Zhou Haifeng, Zhang Meng, Sun |
| Author_xml | – sequence: 1 givenname: Sun surname: Meng fullname: Meng, Sun – sequence: 2 givenname: Zhang surname: Haifeng fullname: Haifeng, Zhang email: 2636004507@qq.com – sequence: 3 givenname: Zhou surname: Yunlong fullname: Yunlong, Zhou |
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| Keywords | Strong-low light alternating catalysis Graphene-like materials WO3/ZnO-graphene-like composite materials Hydrogen production |
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| Snippet | ZnO/WO3/graphene-like composite photocatalysts are prepared by in-situ deposition and successfully utilized for alternating strong-low light catalytic... |
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| StartPage | 176824 |
| SubjectTerms | Graphene-like materials Hydrogen production Strong-low light alternating catalysis WO3/ZnO-graphene-like composite materials |
| Title | Photoelectron marginalization effect in ZnO/WO3/graphene-like composites: Study of alternating strong-low photocatalytic hydrogen production performance and mechanism |
| URI | https://dx.doi.org/10.1016/j.jallcom.2024.176824 |
| Volume | 1009 |
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