Magnetism and hydrogen absorption in UNiZn
UNiZn is the first Zn containing UTX ternary with the ZrNiAl structure type. Zn is smaller than other p-metals (Al, Ga, Sn, In) forming this type of structure. This compound can be seen as analogous to UNiAl and UNiGa, but the small X ligand leads to a non-magnetic ground state with moderately enhan...
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| Published in | Journal of alloys and compounds Vol. 646; pp. 885 - 892 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
15.10.2015
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| Abstract | UNiZn is the first Zn containing UTX ternary with the ZrNiAl structure type. Zn is smaller than other p-metals (Al, Ga, Sn, In) forming this type of structure. This compound can be seen as analogous to UNiAl and UNiGa, but the small X ligand leads to a non-magnetic ground state with moderately enhanced Sommerfeld coefficient γ = 100 mJ/mol K2. H absorption leads to analogous effects (amount of hydrogen absorbed, crystal structure changed) as in UNiAlH2.3, in which the ordering temperature increases. UNiZnH2.3 exhibits antiferromagnetic order below the Néel temperature TN = 55 K.
•New hexagonal Zn-compound with 111 stoichiometry was found.•UNiZn does not show any magnetic order down to 2 K.•Hydrogen absorption in UNiZn is very sensitive to the temperature.•High-T absorption leads to the reversible decomposition of the compound.•Low-T hydride exhibits antiferromagnetic order below TN = 55 K. |
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| AbstractList | UNiZn is the first Zn containing UTX ternary with the ZrNiAl structure type. Zn is smaller than other p-metals (Al, Ga, Sn, In) forming this type of structure. This compound can be seen as analogous to UNiAl and UNiGa, but the small X ligand leads to a non-magnetic ground state with moderately enhanced Sommerfeld coefficient γ = 100 mJ/mol K2. H absorption leads to analogous effects (amount of hydrogen absorbed, crystal structure changed) as in UNiAlH2.3, in which the ordering temperature increases. UNiZnH2.3 exhibits antiferromagnetic order below the Néel temperature TN = 55 K.
•New hexagonal Zn-compound with 111 stoichiometry was found.•UNiZn does not show any magnetic order down to 2 K.•Hydrogen absorption in UNiZn is very sensitive to the temperature.•High-T absorption leads to the reversible decomposition of the compound.•Low-T hydride exhibits antiferromagnetic order below TN = 55 K. |
| Author | Kolomiets, A.V. Mašková, S. Daniš, S. Miliyanchuk, K. Stelmakhovych, O. Vondráčková, B. Havela, L. |
| Author_xml | – sequence: 1 givenname: S. surname: Mašková fullname: Mašková, S. email: maskova@mag.mff.cuni.cz organization: Department of Condensed Matter Physics, Faculty of Mathematics and Physics, Charles University, Prague 2, Czech Republic – sequence: 2 givenname: S. surname: Daniš fullname: Daniš, S. organization: Department of Condensed Matter Physics, Faculty of Mathematics and Physics, Charles University, Prague 2, Czech Republic – sequence: 3 givenname: K. surname: Miliyanchuk fullname: Miliyanchuk, K. organization: Department of Inorganic Chemistry, Faculty of Chemistry, Ivan Franko National University of Lviv, 79005 Lviv, Ukraine – sequence: 4 givenname: O. surname: Stelmakhovych fullname: Stelmakhovych, O. organization: Department of Life Safety, Ivan Franko National University of Lviv, 79005 Lviv, Ukraine – sequence: 5 givenname: B. surname: Vondráčková fullname: Vondráčková, B. organization: Department of Condensed Matter Physics, Faculty of Mathematics and Physics, Charles University, Prague 2, Czech Republic – sequence: 6 givenname: A.V. surname: Kolomiets fullname: Kolomiets, A.V. organization: Department of Condensed Matter Physics, Faculty of Mathematics and Physics, Charles University, Prague 2, Czech Republic – sequence: 7 givenname: L. surname: Havela fullname: Havela, L. organization: Department of Condensed Matter Physics, Faculty of Mathematics and Physics, Charles University, Prague 2, Czech Republic |
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| CitedBy_id | crossref_primary_10_1016_j_jallcom_2017_07_038 crossref_primary_10_1016_j_jallcom_2021_162721 crossref_primary_10_1016_j_jallcom_2020_155606 crossref_primary_10_1088_1361_6633_acbe50 |
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