Metal-organic frameworks with 1,4-di(1-imidazol-4-yl)benzene and varied carboxylate ligands for selectively sensing Fe() ions and ketone molecules

Four new metal-organic frameworks (MOFs) [Zn(L)(bpdc)]·1.6H 2 O ( 1 ), [Co(L)(bpdc)]·H 2 O ( 2 ), [Ni 3 (L) 2 (bptc) 2 (H 2 O) 10 ]·2H 2 O ( 3 ) and [Cd 2 (L)(Hbptc) 2 ] ( 4 ) were achieved by reactions of the corresponding metal salt with mixed organic ligands of 1,4-di(1 H -imidazol-4-yl)benzene (...

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Published inDalton transactions : an international journal of inorganic chemistry Vol. 46; no. 4; pp. 13943 - 13951
Main Authors Liu, Zhi-Qiang, Zhao, Yue, Zhang, Xiu-Du, Kang, Yan-Shang, Lu, Qing-Yi, Azam, Mohammad, Al-Resayes, Saud I, Sun, Wei-Yin
Format Journal Article
LanguageEnglish
Published England 17.10.2017
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Abstract Four new metal-organic frameworks (MOFs) [Zn(L)(bpdc)]·1.6H 2 O ( 1 ), [Co(L)(bpdc)]·H 2 O ( 2 ), [Ni 3 (L) 2 (bptc) 2 (H 2 O) 10 ]·2H 2 O ( 3 ) and [Cd 2 (L)(Hbptc) 2 ] ( 4 ) were achieved by reactions of the corresponding metal salt with mixed organic ligands of 1,4-di(1 H -imidazol-4-yl)benzene (L) and 4,4′-benzophenonedicarboxylic acid (H 2 bpdc) or biphenyl-2,4′,5-tricarboxylic acid (H 3 bptc). They exhibit varied structures: MOFs 1 and 4 are porous three-dimensional (3D) frameworks, while 2 is an infinite one-dimensional (1D) chain and 3 is a two-dimensional (2D) network. Remarkably, 1 and 4 can act as potential fluorescent materials for sensing Fe( iii ) ions and different ketone molecules with high selectivity and sensitivity. In addition, MOF 1 shows selective adsorption of CO 2 over N 2 . Zn( ii ) and Cd( ii ) frameworks have potential for sensing Fe( iii ) and ketone molecules with high selectivity and sensitivity.
AbstractList Four new metal–organic frameworks (MOFs) [Zn(L)(bpdc)]·1.6H 2 O ( 1 ), [Co(L)(bpdc)]·H 2 O ( 2 ), [Ni 3 (L) 2 (bptc) 2 (H 2 O) 10 ]·2H 2 O ( 3 ) and [Cd 2 (L)(Hbptc) 2 ] ( 4 ) were achieved by reactions of the corresponding metal salt with mixed organic ligands of 1,4-di(1 H -imidazol-4-yl)benzene (L) and 4,4′-benzophenonedicarboxylic acid (H 2 bpdc) or biphenyl-2,4′,5-tricarboxylic acid (H 3 bptc). They exhibit varied structures: MOFs 1 and 4 are porous three-dimensional (3D) frameworks, while 2 is an infinite one-dimensional (1D) chain and 3 is a two-dimensional (2D) network. Remarkably, 1 and 4 can act as potential fluorescent materials for sensing Fe( iii ) ions and different ketone molecules with high selectivity and sensitivity. In addition, MOF 1 shows selective adsorption of CO 2 over N 2 .
Four new metal-organic frameworks (MOFs) [Zn(L)(bpdc)]·1.6H O (1), [Co(L)(bpdc)]·H O (2), [Ni (L) (bptc) (H O) ]·2H O (3) and [Cd (L)(Hbptc) ] (4) were achieved by reactions of the corresponding metal salt with mixed organic ligands of 1,4-di(1H-imidazol-4-yl)benzene (L) and 4,4'-benzophenonedicarboxylic acid (H bpdc) or biphenyl-2,4',5-tricarboxylic acid (H bptc). They exhibit varied structures: MOFs 1 and 4 are porous three-dimensional (3D) frameworks, while 2 is an infinite one-dimensional (1D) chain and 3 is a two-dimensional (2D) network. Remarkably, 1 and 4 can act as potential fluorescent materials for sensing Fe(iii) ions and different ketone molecules with high selectivity and sensitivity. In addition, MOF 1 shows selective adsorption of CO over N .
Four new metal-organic frameworks (MOFs) [Zn(L)(bpdc)]·1.6H2O (1), [Co(L)(bpdc)]·H2O (2), [Ni3(L)2(bptc)2(H2O)10]·2H2O (3) and [Cd2(L)(Hbptc)2] (4) were achieved by reactions of the corresponding metal salt with mixed organic ligands of 1,4-di(1H-imidazol-4-yl)benzene (L) and 4,4'-benzophenonedicarboxylic acid (H2bpdc) or biphenyl-2,4',5-tricarboxylic acid (H3bptc). They exhibit varied structures: MOFs 1 and 4 are porous three-dimensional (3D) frameworks, while 2 is an infinite one-dimensional (1D) chain and 3 is a two-dimensional (2D) network. Remarkably, 1 and 4 can act as potential fluorescent materials for sensing Fe(iii) ions and different ketone molecules with high selectivity and sensitivity. In addition, MOF 1 shows selective adsorption of CO2 over N2.Four new metal-organic frameworks (MOFs) [Zn(L)(bpdc)]·1.6H2O (1), [Co(L)(bpdc)]·H2O (2), [Ni3(L)2(bptc)2(H2O)10]·2H2O (3) and [Cd2(L)(Hbptc)2] (4) were achieved by reactions of the corresponding metal salt with mixed organic ligands of 1,4-di(1H-imidazol-4-yl)benzene (L) and 4,4'-benzophenonedicarboxylic acid (H2bpdc) or biphenyl-2,4',5-tricarboxylic acid (H3bptc). They exhibit varied structures: MOFs 1 and 4 are porous three-dimensional (3D) frameworks, while 2 is an infinite one-dimensional (1D) chain and 3 is a two-dimensional (2D) network. Remarkably, 1 and 4 can act as potential fluorescent materials for sensing Fe(iii) ions and different ketone molecules with high selectivity and sensitivity. In addition, MOF 1 shows selective adsorption of CO2 over N2.
Four new metal-organic frameworks (MOFs) [Zn(L)(bpdc)]·1.6H 2 O ( 1 ), [Co(L)(bpdc)]·H 2 O ( 2 ), [Ni 3 (L) 2 (bptc) 2 (H 2 O) 10 ]·2H 2 O ( 3 ) and [Cd 2 (L)(Hbptc) 2 ] ( 4 ) were achieved by reactions of the corresponding metal salt with mixed organic ligands of 1,4-di(1 H -imidazol-4-yl)benzene (L) and 4,4′-benzophenonedicarboxylic acid (H 2 bpdc) or biphenyl-2,4′,5-tricarboxylic acid (H 3 bptc). They exhibit varied structures: MOFs 1 and 4 are porous three-dimensional (3D) frameworks, while 2 is an infinite one-dimensional (1D) chain and 3 is a two-dimensional (2D) network. Remarkably, 1 and 4 can act as potential fluorescent materials for sensing Fe( iii ) ions and different ketone molecules with high selectivity and sensitivity. In addition, MOF 1 shows selective adsorption of CO 2 over N 2 . Zn( ii ) and Cd( ii ) frameworks have potential for sensing Fe( iii ) and ketone molecules with high selectivity and sensitivity.
Author Kang, Yan-Shang
Zhao, Yue
Sun, Wei-Yin
Zhang, Xiu-Du
Azam, Mohammad
Al-Resayes, Saud I
Lu, Qing-Yi
Liu, Zhi-Qiang
AuthorAffiliation Department of Chemistry
State Key Laboratory of Coordination Chemistry
Coordination Chemistry Institute
College of Science
Collaborative Innovation Center of Advanced Microstructures
Nanjing National Laboratory of Microstructures
King Saud University
Nanjing University
School of Chemistry and Chemical Engineering
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  name: Department of Chemistry
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  name: School of Chemistry and Chemical Engineering
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  name: Collaborative Innovation Center of Advanced Microstructures
– sequence: 0
  name: Coordination Chemistry Institute
– sequence: 0
  name: King Saud University
– sequence: 0
  name: State Key Laboratory of Coordination Chemistry
– sequence: 0
  name: Nanjing University
– sequence: 0
  name: College of Science
Author_xml – sequence: 1
  givenname: Zhi-Qiang
  surname: Liu
  fullname: Liu, Zhi-Qiang
– sequence: 2
  givenname: Yue
  surname: Zhao
  fullname: Zhao, Yue
– sequence: 3
  givenname: Xiu-Du
  surname: Zhang
  fullname: Zhang, Xiu-Du
– sequence: 4
  givenname: Yan-Shang
  surname: Kang
  fullname: Kang, Yan-Shang
– sequence: 5
  givenname: Qing-Yi
  surname: Lu
  fullname: Lu, Qing-Yi
– sequence: 6
  givenname: Mohammad
  surname: Azam
  fullname: Azam, Mohammad
– sequence: 7
  givenname: Saud I
  surname: Al-Resayes
  fullname: Al-Resayes, Saud I
– sequence: 8
  givenname: Wei-Yin
  surname: Sun
  fullname: Sun, Wei-Yin
BackLink https://www.ncbi.nlm.nih.gov/pubmed/28972233$$D View this record in MEDLINE/PubMed
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PublicationTitle Dalton transactions : an international journal of inorganic chemistry
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Snippet Four new metal-organic frameworks (MOFs) [Zn(L)(bpdc)]·1.6H 2 O ( 1 ), [Co(L)(bpdc)]·H 2 O ( 2 ), [Ni 3 (L) 2 (bptc) 2 (H 2 O) 10 ]·2H 2 O ( 3 ) and [Cd 2...
Four new metal–organic frameworks (MOFs) [Zn(L)(bpdc)]·1.6H 2 O ( 1 ), [Co(L)(bpdc)]·H 2 O ( 2 ), [Ni 3 (L) 2 (bptc) 2 (H 2 O) 10 ]·2H 2 O ( 3 ) and [Cd 2...
Four new metal-organic frameworks (MOFs) [Zn(L)(bpdc)]·1.6H O (1), [Co(L)(bpdc)]·H O (2), [Ni (L) (bptc) (H O) ]·2H O (3) and [Cd (L)(Hbptc) ] (4) were...
Four new metal-organic frameworks (MOFs) [Zn(L)(bpdc)]·1.6H2O (1), [Co(L)(bpdc)]·H2O (2), [Ni3(L)2(bptc)2(H2O)10]·2H2O (3) and [Cd2(L)(Hbptc)2] (4) were...
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Title Metal-organic frameworks with 1,4-di(1-imidazol-4-yl)benzene and varied carboxylate ligands for selectively sensing Fe() ions and ketone molecules
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