Preparation of anode by MOF pyrolysis enabled long-life rechargeable zinc nickel batteries
Water-induced parasitic reaction and zinc dendrite growth caused by uneven electric field distribution on the surface of the zinc anode are the most controversial problems in the practical application of zinc-nickel rechargeable batteries in large-scale energy storage. Herein, Bi2O3/In2O3 doped ZnO@...
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| Published in | Journal of alloys and compounds Vol. 949; p. 169870 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
15.07.2023
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0925-8388 1873-4669 |
| DOI | 10.1016/j.jallcom.2023.169870 |
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| Abstract | Water-induced parasitic reaction and zinc dendrite growth caused by uneven electric field distribution on the surface of the zinc anode are the most controversial problems in the practical application of zinc-nickel rechargeable batteries in large-scale energy storage. Herein, Bi2O3/In2O3 doped ZnO@C synthesized by MOF pyrolysis with good cycle stability. The ability to inhibit hydrogen evolution and achieve uniform deposition of zinc is characterized by CV, Tafel, and scanning electron microscopy (SEM). Benefiting from the high hydrogen evolution overpotential and high electrical conductivity, Bi2O3 doped ZnO@C (BCZ) and In2O3 doped ZnO@C (ICZ) electrodes deliver high capacity of 640 mA h g−1 and 580 mA h g−1 at 10 C after 1200 and 3400 cycles, respectively, and reveals long-term cyclic stability with capacity retention over 90%. This work provides new ideas for the anode synthesis of aqueous rechargeable zinc metal batteries and other batteries.
•Bi2O3/In2O3 doped ZnO@C are synthesized in one step by a simple MOF-5 pyrolysis route.•Bi2O3/In2O3 doped ZnO@C anode achieves ultra-long cycle stability at a high rate.•The dual regulation mechanism of MOF and Bi2O3/In2O3 inhibit the growth of dendrites and the occurrence of HER. |
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| AbstractList | Water-induced parasitic reaction and zinc dendrite growth caused by uneven electric field distribution on the surface of the zinc anode are the most controversial problems in the practical application of zinc-nickel rechargeable batteries in large-scale energy storage. Herein, Bi2O3/In2O3 doped ZnO@C synthesized by MOF pyrolysis with good cycle stability. The ability to inhibit hydrogen evolution and achieve uniform deposition of zinc is characterized by CV, Tafel, and scanning electron microscopy (SEM). Benefiting from the high hydrogen evolution overpotential and high electrical conductivity, Bi2O3 doped ZnO@C (BCZ) and In2O3 doped ZnO@C (ICZ) electrodes deliver high capacity of 640 mA h g−1 and 580 mA h g−1 at 10 C after 1200 and 3400 cycles, respectively, and reveals long-term cyclic stability with capacity retention over 90%. This work provides new ideas for the anode synthesis of aqueous rechargeable zinc metal batteries and other batteries.
•Bi2O3/In2O3 doped ZnO@C are synthesized in one step by a simple MOF-5 pyrolysis route.•Bi2O3/In2O3 doped ZnO@C anode achieves ultra-long cycle stability at a high rate.•The dual regulation mechanism of MOF and Bi2O3/In2O3 inhibit the growth of dendrites and the occurrence of HER. |
| ArticleNumber | 169870 |
| Author | Wang, Jianglin Su, Qingsong Li, Shandong Xu, Jiancheng Yang, Zhanhong Liang, Hanhao |
| Author_xml | – sequence: 1 givenname: Hanhao surname: Liang fullname: Liang, Hanhao organization: Hunan Province Key Laboratory of Chemical Power Source, College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China – sequence: 2 givenname: Qingsong surname: Su fullname: Su, Qingsong organization: Hunan Province Key Laboratory of Chemical Power Source, College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China – sequence: 3 givenname: Jiancheng surname: Xu fullname: Xu, Jiancheng organization: Hunan Province Key Laboratory of Chemical Power Source, College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China – sequence: 4 givenname: Zhanhong orcidid: 0000-0002-7964-1200 surname: Yang fullname: Yang, Zhanhong email: zhyangcsu611@163.com organization: Hunan Province Key Laboratory of Chemical Power Source, College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China – sequence: 5 givenname: Shandong surname: Li fullname: Li, Shandong organization: Hunan Province Key Laboratory of Chemical Power Source, College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China – sequence: 6 givenname: Jianglin surname: Wang fullname: Wang, Jianglin organization: Hunan Province Key Laboratory of Chemical Power Source, College of Chemistry and Chemical Engineering, Central South University, Changsha 410083, China |
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| Keywords | Long-term cyclic stability Zinc anode MOF pyrolysis Zinc-nickel rechargeable batteries |
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