Earth-abundant photoelectrodes for water splitting and alternate oxidation reactions: Recent advances and future perspectives

Solar water splitting by means of photoelectrochemical (PEC) cells offers the promise to produce cost-effective renewable and clean fuel from abundant sunlight and water. Lately, the realization of promise of concurrent hydrogen (H2) production along with alternate oxidation reaction (which is less...

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Published inProgress in materials science Vol. 134; p. 101073
Main Authors Suryawanshi, Mahesh P., Ghorpade, Uma V., Toe, Cui Ying, Suryawanshi, Umesh P., He, Mingrui, Zhang, Doudou, Jang, Jun Sung, Shin, Seung Wook, Kim, Jin Hyeok, Hao, Xiaojing, Amal, Rose
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 01.04.2023
Subjects
Alternate oxidation reactions
Clean hydrogen production
Computational screenings
Earth-abundant materials
Energy conversion
Nanomaterials
Photoanode
Photocathode
Solar water splitting
Value-added chemicals products
P-doped (ZnxCd1-x)S
OCV
IMPS
DFF
PV
STH
Cu:NiO
CBTSSe
STO
b-BiVO4@a-TiO2-x
DFT
Alternate oxidation reactions
Vo-Co3O4
VBM
FeOOH
VBO
IO
AI
Nanomaterials
DOS
PEC-PV
AM
MOCVD
EIS
AAO
Co-HAO
CCZTS
S-TNR
GLLB
TEMPO
DHA
OER
FFCA
ACZTS
Value-added chemicals products
Photocathode
a-Si
BP
SC
SnO2@BiVO4/Co-Pi
S
G@U-LDH@BVO
FTIR
Energy conversion
CZTSSe
HPLC
CB
Mo:BVO
NTs
CP
TA
Clean hydrogen production
LA
Si
M:B-Fe2O3
FE-SEM
ALD
TM
ETL
N-TiO2
MDH
SHE
PW9Co
PBE
HC-STH
CQD
EVBM
BL-BVO
mid-IR TA
BiOI
ML
α-Fe2O3
MW
VB
LSV
In:BiVO4
NC
Solar water splitting
NFs
Photoanode
FDCA
g-C3N4
Computational screenings
HTL
Eg
NP
OECs
TANF
O2
NR
Earth-abundant materials
NT
ABPE
NHE
RHE
LDH
CBO
Vo
rGO
OQMD
HMA
HMF
GO/CuTCPP
MOD
MOF
HMFCA
Zn:BVO
H2
LSPR
IPCE
MGI
PED
PEC
STEM
PC
HER
CZGTS
r-BVO
TEM
Online AccessGet full text
ISSN0079-6425
1873-2208
DOI10.1016/j.pmatsci.2023.101073

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Abstract Solar water splitting by means of photoelectrochemical (PEC) cells offers the promise to produce cost-effective renewable and clean fuel from abundant sunlight and water. Lately, the realization of promise of concurrent hydrogen (H2) production along with alternate oxidation reaction (which is less energetically demanding than the water oxidation reaction) has also become a subject of intense global research interests. At present, developing inexpensive, non-toxic, and earth-abundant semiconductor-based photoelectrodes (i.e. photocathode and photoanode) with a high stability is of great importance in achieving economically viable H2 production and value-added chemicals. This review summarizes recent advances in these photoelectrodes along with contemporary understanding of key factors responsible for high solar-to-hydrogen efficiency, device stability, and highlights a promising new research trend of alternate oxidation reactions at photoanodes. First, we outline recent developments of novel photoelectrode materials using high-throughput computational screening integrated with ab-initio calculations. We proceed to discuss the merits and major challenges of these novel and existing photoelectrodes and links the strategies used to overcome these challenges to achieve economically viable solar H2 generation. Several important studies on the emerging new trend of alternate oxidations reactions at photoanodes toward value-added chemicals are then detailed with particular emphasis is placed on dependency of photoanode design on type of organic feedstocks and desired products from the oxidation reaction. We also emphasize the development of tandem devices for overall water splitting using these photoelectrodes with high onset potentials. Finally, we provide not only promising future directions for each material system, but also a critical assessment and outlook on how these earth-abundant photoelectrodes could lead to a potential large-scale implementation of water splitting devices.
AbstractList Solar water splitting by means of photoelectrochemical (PEC) cells offers the promise to produce cost-effective renewable and clean fuel from abundant sunlight and water. Lately, the realization of promise of concurrent hydrogen (H2) production along with alternate oxidation reaction (which is less energetically demanding than the water oxidation reaction) has also become a subject of intense global research interests. At present, developing inexpensive, non-toxic, and earth-abundant semiconductor-based photoelectrodes (i.e. photocathode and photoanode) with a high stability is of great importance in achieving economically viable H2 production and value-added chemicals. This review summarizes recent advances in these photoelectrodes along with contemporary understanding of key factors responsible for high solar-to-hydrogen efficiency, device stability, and highlights a promising new research trend of alternate oxidation reactions at photoanodes. First, we outline recent developments of novel photoelectrode materials using high-throughput computational screening integrated with ab-initio calculations. We proceed to discuss the merits and major challenges of these novel and existing photoelectrodes and links the strategies used to overcome these challenges to achieve economically viable solar H2 generation. Several important studies on the emerging new trend of alternate oxidations reactions at photoanodes toward value-added chemicals are then detailed with particular emphasis is placed on dependency of photoanode design on type of organic feedstocks and desired products from the oxidation reaction. We also emphasize the development of tandem devices for overall water splitting using these photoelectrodes with high onset potentials. Finally, we provide not only promising future directions for each material system, but also a critical assessment and outlook on how these earth-abundant photoelectrodes could lead to a potential large-scale implementation of water splitting devices.
ArticleNumber 101073
Author Shin, Seung Wook
Amal, Rose
Zhang, Doudou
Suryawanshi, Mahesh P.
Ghorpade, Uma V.
Jang, Jun Sung
Hao, Xiaojing
Toe, Cui Ying
Suryawanshi, Umesh P.
He, Mingrui
Kim, Jin Hyeok
Author_xml – sequence: 1
  givenname: Mahesh P.
  surname: Suryawanshi
  fullname: Suryawanshi, Mahesh P.
  email: m.suryawanshi@unsw.edu.au
  organization: School of Photovoltaic and Renewable Energy Engineering, University of New South Wales, Sydney, NSW 2052, Australia
– sequence: 2
  givenname: Uma V.
  surname: Ghorpade
  fullname: Ghorpade, Uma V.
  organization: School of Photovoltaic and Renewable Energy Engineering, University of New South Wales, Sydney, NSW 2052, Australia
– sequence: 3
  givenname: Cui Ying
  surname: Toe
  fullname: Toe, Cui Ying
  organization: Particles and Catalysis Research Group, School of Chemical Engineering, University of New South Wales, Sydney 2052, Australia
– sequence: 4
  givenname: Umesh P.
  surname: Suryawanshi
  fullname: Suryawanshi, Umesh P.
  organization: Optoelectronics Convergence Research Center and Department of Materials Science and Engineering, Chonnam National University, 300, Yongbong-Dong, Buk-Gu, Gwangju 61186, South Korea
– sequence: 5
  givenname: Mingrui
  surname: He
  fullname: He, Mingrui
  organization: School of Photovoltaic and Renewable Energy Engineering, University of New South Wales, Sydney, NSW 2052, Australia
– sequence: 6
  givenname: Doudou
  surname: Zhang
  fullname: Zhang, Doudou
  organization: Research School of Electrical, Energy and Materials Engineering, The Australian National University, Canberra 2601, Australia
– sequence: 7
  givenname: Jun Sung
  surname: Jang
  fullname: Jang, Jun Sung
  organization: Optoelectronics Convergence Research Center and Department of Materials Science and Engineering, Chonnam National University, 300, Yongbong-Dong, Buk-Gu, Gwangju 61186, South Korea
– sequence: 8
  givenname: Seung Wook
  surname: Shin
  fullname: Shin, Seung Wook
  email: swshin@ekr.or.kr
  organization: Future Agricultural Research Division, Water Resource and Environment Research Group, Rural Research Institute, Korea Rural Community Corporation, Ansan-Si, Gyeonggi-do 15634, South Korea
– sequence: 9
  givenname: Jin Hyeok
  surname: Kim
  fullname: Kim, Jin Hyeok
  email: jinhyeok@chonnam.ac.kr
  organization: Optoelectronics Convergence Research Center and Department of Materials Science and Engineering, Chonnam National University, 300, Yongbong-Dong, Buk-Gu, Gwangju 61186, South Korea
– sequence: 10
  givenname: Xiaojing
  surname: Hao
  fullname: Hao, Xiaojing
  email: xj.hao@unsw.edu.au
  organization: School of Photovoltaic and Renewable Energy Engineering, University of New South Wales, Sydney, NSW 2052, Australia
– sequence: 11
  givenname: Rose
  surname: Amal
  fullname: Amal, Rose
  organization: Particles and Catalysis Research Group, School of Chemical Engineering, University of New South Wales, Sydney 2052, Australia
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Keywords P-doped (ZnxCd1-x)S
OCV
IMPS
DFF
PV
STH
Cu:NiO
CBTSSe
STO
b-BiVO4@a-TiO2-x
DFT
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FeOOH
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AI
Nanomaterials
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EIS
AAO
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CCZTS
S-TNR
GLLB
TEMPO
DHA
OER
FFCA
ACZTS
Value-added chemicals products
Photocathode
a-Si
BP
SC
SnO2@BiVO4/Co-Pi
S
G@U-LDH@BVO
FTIR
Energy conversion
CZTSSe
HPLC
CB
Mo:BVO
NTs
CP
TA
Clean hydrogen production
LA
Si
M:B-Fe2O3
FE-SEM
ALD
TM
ETL
N-TiO2
MDH
SHE
PW9Co
PBE
HC-STH
CQD
EVBM
BL-BVO
mid-IR TA
BiOI
ML
α-Fe2O3
MW
VB
LSV
In:BiVO4
NC
Solar water splitting
NFs
Photoanode
FDCA
g-C3N4
Computational screenings
HTL
Eg
NP
OECs
TANF
O2
NR
Earth-abundant materials
NT
ABPE
NHE
RHE
LDH
CBO
Vo
rGO
OQMD
HMA
HMF
GO/CuTCPP
MOD
MOF
HMFCA
Zn:BVO
H2
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STEM
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HER
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TEM
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Snippet Solar water splitting by means of photoelectrochemical (PEC) cells offers the promise to produce cost-effective renewable and clean fuel from abundant sunlight...
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StartPage 101073
SubjectTerms Alternate oxidation reactions
Clean hydrogen production
Computational screenings
Earth-abundant materials
Energy conversion
Nanomaterials
Photoanode
Photocathode
Solar water splitting
Value-added chemicals products
Title Earth-abundant photoelectrodes for water splitting and alternate oxidation reactions: Recent advances and future perspectives
URI https://dx.doi.org/10.1016/j.pmatsci.2023.101073
Volume 134
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