Internal electric field engineering for steering photogenerated charge separation and enhancing photoactivity

Photocatalysis as a desirable technology shows great potential in environmental remediation and renewable energy generation, but the recombination of photogenerated carriers is a key limiting factor for efficiency in artificial photosynthesis. Internal electric field (IEF, also known as built‐in ele...

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Published inEcoMat (Beijing, China) Vol. 1; no. 1
Main Authors Guo, Yan, Shi, Wenxin, Zhu, Yongfa
Format Journal Article
LanguageEnglish
Published Hoboken, USA John Wiley & Sons, Inc 01.12.2019
Subjects
built‐in electric field
internal electric field
photocatalysis
photogenerated charge separation
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Abstract Photocatalysis as a desirable technology shows great potential in environmental remediation and renewable energy generation, but the recombination of photogenerated carriers is a key limiting factor for efficiency in artificial photosynthesis. Internal electric field (IEF, also known as built‐in electric field) engineering acts an emerging and clearly viable route to increase photocatalytic efficiency by facilitating charge separation and transfer. This review summarizes the basic principles of IEF including the source, the strategies for the enhancement and the measurement of IEF. Highlight is the recent progress in steering photogenerated charge separation of photocatalysts by IEF engineering and related mechanisms. Finally, the challenges in IEF engineering and exciting opportunities to further enhancing charge separation and photocatalytic performance are discussed. In this review, we traced the source of IEF, summarized the enhancement methods of IEF and gave the measurement of IEF source. Highlight is the application advances in IEF for photocatalysis, firstly demonstrating that IEF engineering, an important, exciting, and highly potential emerging research area, is a whole new angle of view for steering the photogenerated charge.
AbstractList Photocatalysis as a desirable technology shows great potential in environmental remediation and renewable energy generation, but the recombination of photogenerated carriers is a key limiting factor for efficiency in artificial photosynthesis. Internal electric field (IEF, also known as built‐in electric field) engineering acts an emerging and clearly viable route to increase photocatalytic efficiency by facilitating charge separation and transfer. This review summarizes the basic principles of IEF including the source, the strategies for the enhancement and the measurement of IEF. Highlight is the recent progress in steering photogenerated charge separation of photocatalysts by IEF engineering and related mechanisms. Finally, the challenges in IEF engineering and exciting opportunities to further enhancing charge separation and photocatalytic performance are discussed. In this review, we traced the source of IEF, summarized the enhancement methods of IEF and gave the measurement of IEF source. Highlight is the application advances in IEF for photocatalysis, firstly demonstrating that IEF engineering, an important, exciting, and highly potential emerging research area, is a whole new angle of view for steering the photogenerated charge.
Author Shi, Wenxin
Zhu, Yongfa
Guo, Yan
Author_xml – sequence: 1
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  surname: Guo
  fullname: Guo, Yan
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– sequence: 2
  givenname: Wenxin
  surname: Shi
  fullname: Shi, Wenxin
  organization: Chongqing University
– sequence: 3
  givenname: Yongfa
  orcidid: 0000-0002-0042-7069
  surname: Zhu
  fullname: Zhu, Yongfa
  email: zhuyf@mail.tsinghua.edu.cn
  organization: Tsinghua University
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Snippet Photocatalysis as a desirable technology shows great potential in environmental remediation and renewable energy generation, but the recombination of...
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SubjectTerms built‐in electric field
internal electric field
photocatalysis
photogenerated charge separation
Title Internal electric field engineering for steering photogenerated charge separation and enhancing photoactivity
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