Visible fluorescence characteristics of Dy3+ doped zinc alumino bismuth borate glasses for optoelectronic devices
Zinc Alumino Bismuth borate (ZnAlBiB) optical glasses of different compositions doped with 1mol% of Dy3+ ions were prepared by the conventional melt quenching technique and investigated by the XRD, optical absorption, photoluminescence and decay curve analysis. The glassy nature of ZnAlBiB host has...
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| Published in | Ceramics international Vol. 39; no. 7; pp. 8459 - 8465 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
01.09.2013
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Zinc Alumino Bismuth borate (ZnAlBiB) optical glasses of different compositions doped with 1mol% of Dy3+ ions were prepared by the conventional melt quenching technique and investigated by the XRD, optical absorption, photoluminescence and decay curve analysis. The glassy nature of ZnAlBiB host has been confirmed through XRD measurements. From the absorption spectral measurements, the three phenomenological intensity parameters Ωλ (λ=2,4 and 6) have been determined from the Judd–Ofelt (J–O) theory. By using JO intensity parameters, several radiative properties such as transition probability (AR), branching ratio (βR) and radiative lifetimes (τR) have been determined. The room temperature photoluminescence spectra of Dy3+ ions doped ZnAlBiB glasses gave two relatively intense emission bands 4F9/2→6H15/2 (blue), 4F9/2→6H13/2 (yellow) along with one faint band. The higher values of branching ratios and stimulated emission cross-sections for the 4F9/2→6H13/2 transition suggest the utility of these glasses as potential laser materials. The decay curves have been recorded for all the ZnAlBiB glasses to measure the quantum efficiency of these glasses by measuring the experimental lifetime (τexp). The radiative properties and CIE chromaticity co-ordinates have been evaluated from the emission spectra to understand the feasibility of these glasses for optoelectronic devices. |
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| AbstractList | Zinc Alumino Bismuth borate (ZnAlBiB) optical glasses of different compositions doped with 1mol% of Dy3+ ions were prepared by the conventional melt quenching technique and investigated by the XRD, optical absorption, photoluminescence and decay curve analysis. The glassy nature of ZnAlBiB host has been confirmed through XRD measurements. From the absorption spectral measurements, the three phenomenological intensity parameters Ωλ (λ=2,4 and 6) have been determined from the Judd–Ofelt (J–O) theory. By using JO intensity parameters, several radiative properties such as transition probability (AR), branching ratio (βR) and radiative lifetimes (τR) have been determined. The room temperature photoluminescence spectra of Dy3+ ions doped ZnAlBiB glasses gave two relatively intense emission bands 4F9/2→6H15/2 (blue), 4F9/2→6H13/2 (yellow) along with one faint band. The higher values of branching ratios and stimulated emission cross-sections for the 4F9/2→6H13/2 transition suggest the utility of these glasses as potential laser materials. The decay curves have been recorded for all the ZnAlBiB glasses to measure the quantum efficiency of these glasses by measuring the experimental lifetime (τexp). The radiative properties and CIE chromaticity co-ordinates have been evaluated from the emission spectra to understand the feasibility of these glasses for optoelectronic devices. Zinc alumino bismuth borate (ZnAlBiB) optical glasses with different compositions doped with 1 mol% of Dy3+ ions were prepared by the conventional melt quenching technique and investigated by the XRD, optical absorption, photoluminescence and decay curve analysis. The glassy nature of the ZnAlBiB host was confirmed by XRD. From the absorption spectra, the three phenomenological intensity parameters omega-lambda (lambda = 2,4 and 6) were determined from the Judd-Ofelt (J-O) theory. Using JO intensity parameters, several radiative properties including transition probability (AR), branching ratio (beta-R) and radiative lifetimes (tau-R) were determined. The room temperature photoluminescence spectra of Dy3+ ion-doped ZnAlBiB glasses gave two relatively intense emission bands 4F9/2 to 6H15/2 (blue), 4F9/2 to 6H13/2 (yellow) along with one faint band. The higher values of branching ratios and stimulated emission cross-sections for the 4F9/2 to 6H13/2 transition suggested the use of these glasses as potential laser materials. The decay curves were recorded for all the ZnAlBiB glasses to measure the quantum efficiency of these glasses by measuring the experimental lifetime (tau-exp). The radiative properties and CIE chromaticity co-ordinates were evaluated from the emission spectra to understand the feasibility of these glasses for optoelectronic devices. |
| Author | Rama Moorthy, L. Mahamuda, Sk Sasikala, T. Swapna, K. Jayasimhadri, M. Srinivasa Rao, A. |
| Author_xml | – sequence: 1 givenname: K. surname: Swapna fullname: Swapna, K. organization: Department of Physics, K L University, Green Fields, Vaddeswaram 522502, AP, India – sequence: 2 givenname: Sk surname: Mahamuda fullname: Mahamuda, Sk organization: Department of Physics, K L University, Green Fields, Vaddeswaram 522502, AP, India – sequence: 3 givenname: A. surname: Srinivasa Rao fullname: Srinivasa Rao, A. email: drsrallam@yahoo.co.in organization: Department of Physics, K L University, Green Fields, Vaddeswaram 522502, AP, India – sequence: 4 givenname: M. surname: Jayasimhadri fullname: Jayasimhadri, M. organization: Department of Applied Physics, Delhi Technological University, Delhi 110042, India – sequence: 5 givenname: T. surname: Sasikala fullname: Sasikala, T. organization: Department of Physics, S V University, Tirupathi 517502, AP, India – sequence: 6 givenname: L. surname: Rama Moorthy fullname: Rama Moorthy, L. organization: Department of Physics, S V University, Tirupathi 517502, AP, India |
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| Snippet | Zinc Alumino Bismuth borate (ZnAlBiB) optical glasses of different compositions doped with 1mol% of Dy3+ ions were prepared by the conventional melt quenching... Zinc alumino bismuth borate (ZnAlBiB) optical glasses with different compositions doped with 1 mol% of Dy3+ ions were prepared by the conventional melt... |
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| SubjectTerms | Band spectra Bismuth Borates Decay Fluorescence properties Glass Glasses Judd–Ofelt theory Optoelectronic devices Photoluminescence Rare-earths Zinc |
| Title | Visible fluorescence characteristics of Dy3+ doped zinc alumino bismuth borate glasses for optoelectronic devices |
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