Advances in Strain‐Induced Noble Metal Nanohybrids for Electro‐Catalysis: From Theoretical Mechanisms to Practical Use

In response to the climate goal of achieving carbon neutrality by 2050, efficient electrochemical energy conversion devices are garnering increasing attention. However, the enhancement of electrochemical performance using noble metal electrocatalysts, along with cost reduction and electrode fabricat...

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Published inChemElectroChem Vol. 11; no. 15
Main Authors Chen, Zhao‐Yang, Li, Ling‐Tong, Zhao, Feng‐Ming, Zhu, Ying‐Hong, Chu, You‐Qun
Format Journal Article
LanguageEnglish
Published Weinheim John Wiley & Sons, Inc 01.08.2024
Wiley-VCH
Subjects
Active control
Bonding strength
Catalysis
Catalysts
electrocatalysis
Electrocatalysts
Electrochemical analysis
Energy conversion
epitaxial growths
Heavy metals
Intermediates
Metal surfaces
noble metal nanohybrids
Noble metals
practical use
strain effects
Substrates
Surface layers
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Abstract In response to the climate goal of achieving carbon neutrality by 2050, efficient electrochemical energy conversion devices are garnering increasing attention. However, the enhancement of electrochemical performance using noble metal electrocatalysts, along with cost reduction and electrode fabrication, remain significant challenges. Noble metal hybrid nanostructures, possessing multiple surface functionalities, lead to outstanding electrocatalytic performances and low‐cost potential. Strain effects can bolster the bonding strength between the noble metal layers and the substrate or core layers, while simultaneously affecting electrocatalytic performance through tuning the binding strength between catalytically active sites and reactants, including intermediates. This review encapsulates the research efforts directed towards improving the performance of noble metal electrocatalysts and provides an overview of the latest advancements in controlling the surface state of noble metals by incorporating a secondary component. We discuss systematic approaches to adjusting surface strain effects on noble metals, characterization techniques, and application case studies, while extracting key design indicators for readers to consider from a macroscopic perspective. Further, we outline the challenges encountered and current solutions when advancing noble metal catalysts from theoretical mechanisms to practical use. Finally, the perspectives on the future research of noble metal surface layer control techniques were also provided. In this review, we provide a summary of recent advances in approaches to controlling noble metal nanohybrids, characterization techniques, and studies of electrocatalysis applications. Additionally, we outline the challenges encountered and current solutions when advancing noble metal catalysts from theoretical mechanisms to practical use. The perspectives on the future research of noble metal hybrid electrocatalysts were also provided.
AbstractList Abstract In response to the climate goal of achieving carbon neutrality by 2050, efficient electrochemical energy conversion devices are garnering increasing attention. However, the enhancement of electrochemical performance using noble metal electrocatalysts, along with cost reduction and electrode fabrication, remain significant challenges. Noble metal hybrid nanostructures, possessing multiple surface functionalities, lead to outstanding electrocatalytic performances and low‐cost potential. Strain effects can bolster the bonding strength between the noble metal layers and the substrate or core layers, while simultaneously affecting electrocatalytic performance through tuning the binding strength between catalytically active sites and reactants, including intermediates. This review encapsulates the research efforts directed towards improving the performance of noble metal electrocatalysts and provides an overview of the latest advancements in controlling the surface state of noble metals by incorporating a secondary component. We discuss systematic approaches to adjusting surface strain effects on noble metals, characterization techniques, and application case studies, while extracting key design indicators for readers to consider from a macroscopic perspective. Further, we outline the challenges encountered and current solutions when advancing noble metal catalysts from theoretical mechanisms to practical use. Finally, the perspectives on the future research of noble metal surface layer control techniques were also provided.
In response to the climate goal of achieving carbon neutrality by 2050, efficient electrochemical energy conversion devices are garnering increasing attention. However, the enhancement of electrochemical performance using noble metal electrocatalysts, along with cost reduction and electrode fabrication, remain significant challenges. Noble metal hybrid nanostructures, possessing multiple surface functionalities, lead to outstanding electrocatalytic performances and low‐cost potential. Strain effects can bolster the bonding strength between the noble metal layers and the substrate or core layers, while simultaneously affecting electrocatalytic performance through tuning the binding strength between catalytically active sites and reactants, including intermediates. This review encapsulates the research efforts directed towards improving the performance of noble metal electrocatalysts and provides an overview of the latest advancements in controlling the surface state of noble metals by incorporating a secondary component. We discuss systematic approaches to adjusting surface strain effects on noble metals, characterization techniques, and application case studies, while extracting key design indicators for readers to consider from a macroscopic perspective. Further, we outline the challenges encountered and current solutions when advancing noble metal catalysts from theoretical mechanisms to practical use. Finally, the perspectives on the future research of noble metal surface layer control techniques were also provided. In this review, we provide a summary of recent advances in approaches to controlling noble metal nanohybrids, characterization techniques, and studies of electrocatalysis applications. Additionally, we outline the challenges encountered and current solutions when advancing noble metal catalysts from theoretical mechanisms to practical use. The perspectives on the future research of noble metal hybrid electrocatalysts were also provided.
In response to the climate goal of achieving carbon neutrality by 2050, efficient electrochemical energy conversion devices are garnering increasing attention. However, the enhancement of electrochemical performance using noble metal electrocatalysts, along with cost reduction and electrode fabrication, remain significant challenges. Noble metal hybrid nanostructures, possessing multiple surface functionalities, lead to outstanding electrocatalytic performances and low‐cost potential. Strain effects can bolster the bonding strength between the noble metal layers and the substrate or core layers, while simultaneously affecting electrocatalytic performance through tuning the binding strength between catalytically active sites and reactants, including intermediates. This review encapsulates the research efforts directed towards improving the performance of noble metal electrocatalysts and provides an overview of the latest advancements in controlling the surface state of noble metals by incorporating a secondary component. We discuss systematic approaches to adjusting surface strain effects on noble metals, characterization techniques, and application case studies, while extracting key design indicators for readers to consider from a macroscopic perspective. Further, we outline the challenges encountered and current solutions when advancing noble metal catalysts from theoretical mechanisms to practical use. Finally, the perspectives on the future research of noble metal surface layer control techniques were also provided.
Author Li, Ling‐Tong
Chu, You‐Qun
Chen, Zhao‐Yang
Zhao, Feng‐Ming
Zhu, Ying‐Hong
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  surname: Chu
  fullname: Chu, You‐Qun
  email: chenzhy@zjut.edu.cn, chuyq@zjut.edu.cn
  organization: Zhejiang University of Technology
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2016; 28
2008; 130
2016; 9
2016; 22
2017; 42
2023; 35
2013; 25
2023; 39
2020; 120
1986; 33
2017; 46
2008; 7
2020; 59
2021; 121
2020; 8
2020; 6
2020; 3
2023; 23
2013; 13
2023; 26
2021; 598
2013; 12
2023; 656
2016; 354
2016; 353
2016; 352
2010; 70
2014; 8
2012; 336
2006; 128
2009; 323
2009; 324
2021; 9
2021; 8
2023; 10
2021; 7
2015; 6
2021; 5
2021; 4
2023; 14
2023; 11
2021; 3
2021; 2
2023; 17
2023; 15
2023; 640
2023; 19
2020; 78
2017; 29
2020; 102
2021; 1
2015; 9
2015; 7
2008; 91
2022; 435
2004; 93
2023
2017; 17
2017; 13
2010; 132
2009; 9
2016; 138
2003; 423
2022; 304
2007; 46
2013; 4
2022; 23
2023; 622
1998; 81
2011; 59
2024
2013; 6
2014; 136
2023; 62
2018; 9
2018; 8
2018; 3
2012; 134
2024; 8
2018; 1
2007; 6
2014; 14
2018; 30
2022; 30
2022; 32
2015; 91
2023; 614
2022; 33
2017; 202
1989; 39
2019; 7
2019; 9
2019; 4
2019; 6
2023; 56
2019; 2
2015; 51
2021; 380
2024; 124
2021; 143
2018; 17
2023; 47
2007; 317
2007; 315
2023; 45
2006; 45
2023; 48
2022; 12
1985; 156
1981; 14
2022; 13
2021; 371
2022; 14
2022; 10
1998; 74
2018; 12
2023; 958
2022; 16
2017; 7
2017; 8
2012; 285
2021; 21
2017; 2
2017; 3
2023; 4
2023; 5
2023; 6
2023; 8
2023; 145
2022; 68
2019; 366
2011; 11
2019; 125
2023; 944
2023; 2
2015; 348
2021; 31
2021; 33
2015; 44
2022; 929
2019; 359
2015; 15
2015; 14
2018; 140
2023; 123
2015; 328
2019; 141
2005; 44
2016; 55
2021; 14
2022; 144
2021; 13
2012; 3
2015; 27
2021; 12
2021; 11
2022; 61
2021; 17
2013; 135
2005; 54
2012; 6
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e_1_2_9_289_1
e_1_2_9_205_1
e_1_2_9_5_1
e_1_2_9_281_1
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e_1_2_9_118_1
e_1_2_9_133_1
e_1_2_9_179_1
e_1_2_9_349_1
e_1_2_9_156_2
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e_1_2_9_69_1
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e_1_2_9_171_1
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e_1_2_9_77_2
e_1_2_9_31_2
e_1_2_9_54_1
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e_1_2_9_294_1
e_1_2_9_339_2
e_1_2_9_92_1
e_1_2_9_109_1
e_1_2_9_271_1
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e_1_2_9_331_1
e_1_2_9_354_1
e_1_2_9_101_1
e_1_2_9_147_1
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e_1_2_9_16_2
e_1_2_9_185_1
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e_1_2_9_39_2
Zhu J. (e_1_2_9_136_1) 2023; 6
e_1_2_9_244_2
e_1_2_9_20_1
e_1_2_9_89_1
e_1_2_9_221_2
e_1_2_9_66_2
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e_1_2_9_267_1
e_1_2_9_43_2
e_1_2_9_327_2
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e_1_2_9_211_2
e_1_2_9_78_1
e_1_2_9_55_1
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e_1_2_9_32_2
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e_1_2_9_257_2
e_1_2_9_317_1
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Zheng C. (e_1_2_9_226_1) 2023
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Snippet In response to the climate goal of achieving carbon neutrality by 2050, efficient electrochemical energy conversion devices are garnering increasing attention....
Abstract In response to the climate goal of achieving carbon neutrality by 2050, efficient electrochemical energy conversion devices are garnering increasing...
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SubjectTerms Active control
Bonding strength
Catalysis
Catalysts
electrocatalysis
Electrocatalysts
Electrochemical analysis
Energy conversion
epitaxial growths
Heavy metals
Intermediates
Metal surfaces
noble metal nanohybrids
Noble metals
practical use
strain effects
Substrates
Surface layers
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Title Advances in Strain‐Induced Noble Metal Nanohybrids for Electro‐Catalysis: From Theoretical Mechanisms to Practical Use
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