Studies of the effectiveness of the chemical decomposition of polychlorinated biphenyls in alluvial meadow soils in situ under the influence of special physicochemical active compounds
Polychlorinated biphenyls (PCB) are persistent organic pollutants used worldwide up 1990s. Although their use has been heavily restricted, PCB can be found in contaminated soils and sediments. The interaction of polychlorobiphenyls (PCBs) in soils with an alkaline amino acid reagent (NaL) and humic...
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| Published in | IOP conference series. Materials Science and Engineering Vol. 848; no. 1; pp. 12114 - 12120 |
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| Language | English |
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01.05.2020
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| Abstract | Polychlorinated biphenyls (PCB) are persistent organic pollutants used worldwide up 1990s. Although their use has been heavily restricted, PCB can be found in contaminated soils and sediments. The interaction of polychlorobiphenyls (PCBs) in soils with an alkaline amino acid reagent (NaL) and humic acids was studied. According to IR spectroscopy, intermolecular interaction of PCBs with NaL reagent was revealed. Chromatography and IR spectroscopy revealed the transformation and removal of chlorine in the aromatic ring of PCB macromolecules under the influence of an amino acid reagent. In the experiment, from 32 to 77% of PCBs undergo soil degradation, depending on the concentration of the reagent and the frequency of its introduction into soil samples. |
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| AbstractList | Polychlorinated biphenyls (PCB) are persistent organic pollutants used worldwide up 1990s. Although their use has been heavily restricted, PCB can be found in contaminated soils and sediments. The interaction of polychlorobiphenyls (PCBs) in soils with an alkaline amino acid reagent (NaL) and humic acids was studied. According to IR spectroscopy, intermolecular interaction of PCBs with NaL reagent was revealed. Chromatography and IR spectroscopy revealed the transformation and removal of chlorine in the aromatic ring of PCB macromolecules under the influence of an amino acid reagent. In the experiment, from 32 to 77% of PCBs undergo soil degradation, depending on the concentration of the reagent and the frequency of its introduction into soil samples. Abstract Polychlorinated biphenyls (PCB) are persistent organic pollutants used worldwide up 1990s. Although their use has been heavily restricted, PCB can be found in contaminated soils and sediments. The interaction of polychlorobiphenyls (PCBs) in soils with an alkaline amino acid reagent (NaL) and humic acids was studied. According to IR spectroscopy, intermolecular interaction of PCBs with NaL reagent was revealed. Chromatography and IR spectroscopy revealed the transformation and removal of chlorine in the aromatic ring of PCB macromolecules under the influence of an amino acid reagent. In the experiment, from 32 to 77% of PCBs undergo soil degradation, depending on the concentration of the reagent and the frequency of its introduction into soil samples. |
| Author | Yu Aladin, D Ph Deeva, N Demin, D V Sevostyanov, S M |
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| Cites_doi | 10.1016/j.scitotenv.2017.07.246 10.1016/0048-9697(95)04927-4 10.1016/0045-6535(83)90198-4 10.1016/j.envint.2008.07.025 10.1016/j.scitotenv.2012.11.098 10.1016/j.envint.2009.07.015 10.1016/j.chemosphere.2009.03.058 10.1006/rtph.2002.1539 10.1016/j.jhazmat.2009.07.117 10.1016/S0956-053X(03)00029-1 |
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| References_xml | – volume: 610-611 start-page: 1 year: 2018 ident: MSE_848_1_012114bib4 article-title: Results of the second national forest soil inventory in Germany - Interpretation of level and stock profiles for PCDD/F and PCB in terms of vegetation and humus type publication-title: Science of the Total Environment doi: 10.1016/j.scitotenv.2017.07.246 contributor: fullname: Pandelova – volume: 175 start-page: 275 year: 1995 ident: MSE_848_1_012114bib6 article-title: Degradation of PCB in different soils by inoculated Alcaligenes xylosoxidans publication-title: Science of the Total Environment doi: 10.1016/0048-9697(95)04927-4 contributor: fullname: Haluška – start-page: 462 year: 1994 ident: MSE_848_1_012114bib16 contributor: fullname: Sokolov – start-page: 52 year: 1992 ident: MSE_848_1_012114bib10 – volume: 73 start-page: 610 year: 2000 ident: MSE_848_1_012114bib11 article-title: Polychlorodiphenyls in reactions with alcohols publication-title: Zh. adj. chemistry contributor: fullname: Gorbunova – volume: 525 year: 2019 ident: MSE_848_1_012114bib17 article-title: Structural - chemical studies of the destruction oforganochlorine compounds publication-title: IOP Conf. Series: Materials Science and Engineering contributor: fullname: Demin – volume: 2 start-page: 139 year: 2005 ident: MSE_848_1_012114bib12 article-title: Investigation of alkoxy derivatives of polychlorinated biphenyls by gas chromatography/mass spectrometry publication-title: Mass spectrometry contributor: fullname: Zabelina – volume: 12 start-page: 487 year: 1983 ident: MSE_848_1_012114bib9 article-title: Formation of polychlorodibenzofurans (PCDFs) by the photolysis of polychlorobenzenes (PCBs) in aqueous acetonitrile containing phenols publication-title: Chemosphere doi: 10.1016/0045-6535(83)90198-4 contributor: fullname: Choudhry – volume: 35 start-page: 76 year: 2009 ident: MSE_848_1_012114bib5 article-title: Environmental impact and human exposure to PCBs in Guiyu, an electronic waste recycling site in China publication-title: Environment International doi: 10.1016/j.envint.2008.07.025 contributor: fullname: Xing – volume: 408 start-page: 5165 year: 2010 ident: MSE_848_1_012114bib2 publication-title: Environmental contaminants and human health in the Canadian Arctic. Sci Total Environ contributor: fullname: Donaldson – volume: 445 start-page: 237 year: 2013 ident: MSE_848_1_012114bib8 article-title: Overview of in situ and ex situ remediation technologies for PCB-contaminated soils and sediments and obstacles for full-scale application publication-title: Science of the Total Environment doi: 10.1016/j.scitotenv.2012.11.098 contributor: fullname: Gomes – volume: 36 start-page: 901 year: 2010 ident: MSE_848_1_012114bib14 article-title: The effects of individual PCB congeners on the soil bacterial community structure and the abundance of biphenyl dioxygenase genes publication-title: Environ. Int. doi: 10.1016/j.envint.2009.07.015 contributor: fullname: Correa – volume: 76 start-page: 185 year: 2009 ident: MSE_848_1_012114bib3 article-title: Cumulative exposure estimates for polychlorinated biphenyls using a job-exposure matrix publication-title: Chemosphere doi: 10.1016/j.chemosphere.2009.03.058 contributor: fullname: Hopf – volume: 35 start-page: 289 year: 2002 ident: MSE_848_1_012114bib15 article-title: Dermal absorption in rhesus monkeys of polychlorinated biphenyls from soil contaminated with Aroclor 1260 publication-title: Regul Toxicol Pharmacol doi: 10.1006/rtph.2002.1539 contributor: fullname: Mayes – volume: 2 start-page: 20 year: 2017 ident: MSE_848_1_012114bib1 article-title: Analysis of pollution with oil products and organochlorines of soils in the vicinity of Russian Antarctic stations publication-title: Theoretic and applied ecology contributor: fullname: Lupachev – volume: 172 start-page: 1156 year: 2009 ident: MSE_848_1_012114bib7 article-title: Dionysiou A feasibility study on Pd/Mg application in historically contaminated sediments and PCB spiked substrates publication-title: J. Hazard. Mater. doi: 10.1016/j.jhazmat.2009.07.117 contributor: fullname: Agarwal – volume: 23 start-page: 315 year: 2003 ident: MSE_848_1_012114bib13 article-title: Solid state dehalogenation of PCBs in contaminated soil using NaBH4 publication-title: Waste Manag. doi: 10.1016/S0956-053X(03)00029-1 contributor: fullname: Aresta |
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| SubjectTerms | Amino acids Aromatic compounds Chlorine Humic acids Infrared spectroscopy Macromolecules PCB Pollutants Polychlorinated biphenyls Reagents Sediments Soil contamination Spectrum analysis |
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| Title | Studies of the effectiveness of the chemical decomposition of polychlorinated biphenyls in alluvial meadow soils in situ under the influence of special physicochemical active compounds |
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