Real‐Time Dilation Observation of Si‐Alloy Electrode Using Thermally Treated Poly (Amide‐Imide) as a Binder for Lithium Ion Battery
Real time dilation behaviors of a Si‐Ti‐Fe‐Al alloy electrode adopting a poly (amide‐imide) binder were investigated to understand the effects of thermal treatment temperature for PAI binder on the electrochemical performance of the Si‐alloy electrode using an in‐situ electrochemical dilatometer. In...
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| Published in | Bulletin of the Korean Chemical Society Vol. 40; no. 3; pp. 248 - 253 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
Wiley‐VCH Verlag GmbH & Co. KGaA
01.03.2019
대한화학회 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1229-5949 0253-2964 1229-5949 |
| DOI | 10.1002/bkcs.11674 |
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| Abstract | Real time dilation behaviors of a Si‐Ti‐Fe‐Al alloy electrode adopting a poly (amide‐imide) binder were investigated to understand the effects of thermal treatment temperature for PAI binder on the electrochemical performance of the Si‐alloy electrode using an in‐situ electrochemical dilatometer. In situ measurement of the electrode thickness showed that the changes in the volume of the Si electrode was suppressed by heat treatment greater than 300 °C, which well agreed with the improved cycle performance of the Si‐alloy electrode thermally treated at the same temperature. Differential dilation plots of the Si‐alloy electrodes were found to reveal more detailed changes in the volume of the Si‐alloy electrode, thus showing that the enhanced mechanical strength of thermally treated PAI effectively could control the expansion and contraction of the Si‐alloy electrode and ensuring a more stable cycle performance of the Si‐alloy electrode. |
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| AbstractList | Real time dilation behaviors of a Si-Ti-Fe-Al alloy electrode adopting a poly (amide-imide) binder were investigated to understand the effects of thermal treatment temperature for PAI binder on the electrochemical performance of the Si-alloy electrode using an in-situ electrochemical dilatometer. In situ measurement of the electrode thickness showed that the changes in the volume of the Si electrode was suppressed by heat treatment greater than 300 °C, which well agreed with the improved cycle performance of the Si-alloy electrode thermally treated at the same temperature. Differential dilation plots of the Si-alloy electrodes were found to reveal more detailed changes in the volume of the Si-alloy electrode, thus showing that the enhanced mechanical strength of thermally treated PAI effectively could control the expansion and contraction of the Si-alloy electrode and ensuring a more stable cycle performance of the Si-alloy electrode. KCI Citation Count: 2 Real time dilation behaviors of a Si‐Ti‐Fe‐Al alloy electrode adopting a poly (amide‐imide) binder were investigated to understand the effects of thermal treatment temperature for PAI binder on the electrochemical performance of the Si‐alloy electrode using an in‐situ electrochemical dilatometer. In situ measurement of the electrode thickness showed that the changes in the volume of the Si electrode was suppressed by heat treatment greater than 300 °C, which well agreed with the improved cycle performance of the Si‐alloy electrode thermally treated at the same temperature. Differential dilation plots of the Si‐alloy electrodes were found to reveal more detailed changes in the volume of the Si‐alloy electrode, thus showing that the enhanced mechanical strength of thermally treated PAI effectively could control the expansion and contraction of the Si‐alloy electrode and ensuring a more stable cycle performance of the Si‐alloy electrode. Real time dilation behaviors of a Si‐Ti‐Fe‐Al alloy electrode adopting a poly (amide‐imide) binder were investigated to understand the effects of thermal treatment temperature for PAI binder on the electrochemical performance of the Si‐alloy electrode using an in‐situ electrochemical dilatometer. In situ measurement of the electrode thickness showed that the changes in the volume of the Si electrode was suppressed by heat treatment greater than 300 °C, which well agreed with the improved cycle performance of the Si‐alloy electrode thermally treated at the same temperature. Differential dilation plots of the Si‐alloy electrodes were found to reveal more detailed changes in the volume of the Si‐alloy electrode, thus showing that the enhanced mechanical strength of thermally treated PAI effectively could control the expansion and contraction of the Si‐alloy electrode and ensuring a more stable cycle performance of the Si‐alloy electrode. |
| Author | Sohn, Myungbeom Lee, Dong Geun Park, Hyeong‐Il Kim, Hansu Chung, Dong Jae Park, Cheolho |
| Author_xml | – sequence: 1 givenname: Hyeong‐Il surname: Park fullname: Park, Hyeong‐Il organization: Hanyang University – sequence: 2 givenname: Dong Geun surname: Lee fullname: Lee, Dong Geun organization: Hanyang University – sequence: 3 givenname: Dong Jae surname: Chung fullname: Chung, Dong Jae organization: Hanyang University – sequence: 4 givenname: Myungbeom surname: Sohn fullname: Sohn, Myungbeom organization: Hanyang University – sequence: 5 givenname: Cheolho surname: Park fullname: Park, Cheolho organization: Next‐G Institute of Technology, Iljin Electric Co., Ltd – sequence: 6 givenname: Hansu surname: Kim fullname: Kim, Hansu email: khansu@hanyang.ac.kr organization: Hanyang University |
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| Snippet | Real time dilation behaviors of a Si‐Ti‐Fe‐Al alloy electrode adopting a poly (amide‐imide) binder were investigated to understand the effects of thermal... Real time dilation behaviors of a Si-Ti-Fe-Al alloy electrode adopting a poly (amide-imide) binder were investigated to understand the effects of thermal... |
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| SubjectTerms | Binder In situ dilatometer Poly (amide‐imide) Si‐based electrode Volume expansion 화학 |
| Title | Real‐Time Dilation Observation of Si‐Alloy Electrode Using Thermally Treated Poly (Amide‐Imide) as a Binder for Lithium Ion Battery |
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