Sol–gel coatings doped with organosilane and cerium to improve the properties of hot-dip galvanized steel

•Tetraethyl orthosilicate sol was roll coated on hot-dip galvanized steels.•Organosilane doping eliminated cracks on tetraethyl orthosilicate coating.•Organosilane doping improved the corrosion resistance of tetraethyl orthosilicate coating.•The hybrid sol–gel doped with cerium salts exhibited self-...

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Published inCorrosion science Vol. 102; pp. 63 - 71
Main Authors Su, Hsiang-Yu, Chen, Pei-Li, Lin, Chao-Sung
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 01.01.2016
Subjects
EIS
EPMA
Passive films
XPS
Zinc
Passive films
XPS
Zinc
EIS
EPMA
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Abstract •Tetraethyl orthosilicate sol was roll coated on hot-dip galvanized steels.•Organosilane doping eliminated cracks on tetraethyl orthosilicate coating.•Organosilane doping improved the corrosion resistance of tetraethyl orthosilicate coating.•The hybrid sol–gel doped with cerium salts exhibited self-healing capability. An inorganic sol–gel coating and an inorganic/organic hybrid sol–gel coating without and with cerium nitrate were made on hot-dip galvanized steel via a roll coating process. Results showed that the corrosion resistance of the hot-dip galvanized steel was improved with the inorganic coating; however, cracks were present in the coating. Cracks were effectively eliminated and paintability of the sol–gel coating was enhanced while doped with organic precursor. The corrosion resistance and self-healing capability were further enhanced when cerium cation was doped. Finally, the corrosion protection mechanism of the various coatings was discussed in detail.
AbstractList •Tetraethyl orthosilicate sol was roll coated on hot-dip galvanized steels.•Organosilane doping eliminated cracks on tetraethyl orthosilicate coating.•Organosilane doping improved the corrosion resistance of tetraethyl orthosilicate coating.•The hybrid sol–gel doped with cerium salts exhibited self-healing capability. An inorganic sol–gel coating and an inorganic/organic hybrid sol–gel coating without and with cerium nitrate were made on hot-dip galvanized steel via a roll coating process. Results showed that the corrosion resistance of the hot-dip galvanized steel was improved with the inorganic coating; however, cracks were present in the coating. Cracks were effectively eliminated and paintability of the sol–gel coating was enhanced while doped with organic precursor. The corrosion resistance and self-healing capability were further enhanced when cerium cation was doped. Finally, the corrosion protection mechanism of the various coatings was discussed in detail.
Author Lin, Chao-Sung
Chen, Pei-Li
Su, Hsiang-Yu
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  givenname: Chao-Sung
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  surname: Lin
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Snippet •Tetraethyl orthosilicate sol was roll coated on hot-dip galvanized steels.•Organosilane doping eliminated cracks on tetraethyl orthosilicate...
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SubjectTerms EIS
EPMA
Passive films
XPS
Zinc
Title Sol–gel coatings doped with organosilane and cerium to improve the properties of hot-dip galvanized steel
URI https://dx.doi.org/10.1016/j.corsci.2015.09.019
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