Flexible carbon nanofiber film with diatomic Fe-Co sites for efficient oxygen reduction and evolution reactions in wearable zinc-air batteries
Carbon nanofiber (CNF) papers have been widely used in many renewable energy systems, and the development of its catalytic function is of great significance and a major challenge. In this work, we pioneer a time- and cost-efficient strategy for the preparation of large-area flexible CNF films with u...
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| Published in | Nano energy Vol. 87; p. 106147 |
|---|---|
| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
01.09.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Carbon nanofiber (CNF) papers have been widely used in many renewable energy systems, and the development of its catalytic function is of great significance and a major challenge. In this work, we pioneer a time- and cost-efficient strategy for the preparation of large-area flexible CNF films with uniformly distributed diatomic FeN3-CoN3 sites (Fe1Co1-CNF). Due to the excellent compatibility and similar functionality of the pre-designed ZnFeCo-NC precursors (ZnFeCo-pre) with the electrospun polymer polyacrylonitrile (PAN), the mixture of ZnFeCo-pre and PAN can be co-electrospun and subject to a standard CNF fabrication process. The resulting Fe1Co1-CNF exhibits excellent bifunctional catalytic performance for both oxygen reduction reaction (ORR) and oxygen evolution reaction (OER), attributing to the abundant dual catalytic FeN3-CoN3 sites which are mutually beneficial for attaining optimal electronic properties for the adsorption/desorption of reaction intermediates. The assembled liquid-electrolyte ZAB provides a high specific power of 201.7 mW cm−2 and excellent cycling stability. More importantly, due to the good mechanical strength and flexibility of Fe1Co1-CNF, portable ZAB with exceptional shape deformability and stability can be demonstrated, in which Fe1Co1-CNF utility as an integrated free-standing membrane electrode. These findings provide a facile strategy for manufacturing flexible multi-functional catalytic electrodes with high production.
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•Large-area self-standing flexible CNF film with diatomic Fe-Co sites was developed.•The diatomic Fe-Co sites render optimized adsorption of O-containing intermediates.•The Fe1Co1-CNF exhibits superior bifunctional ORR/OER performance.•The Fe1Co1-CNF shows great potential in liquid/flexible Zn-air battery. |
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| AbstractList | Carbon nanofiber (CNF) papers have been widely used in many renewable energy systems, and the development of its catalytic function is of great significance and a major challenge. In this work, we pioneer a time- and cost-efficient strategy for the preparation of large-area flexible CNF films with uniformly distributed diatomic FeN3-CoN3 sites (Fe1Co1-CNF). Due to the excellent compatibility and similar functionality of the pre-designed ZnFeCo-NC precursors (ZnFeCo-pre) with the electrospun polymer polyacrylonitrile (PAN), the mixture of ZnFeCo-pre and PAN can be co-electrospun and subject to a standard CNF fabrication process. The resulting Fe1Co1-CNF exhibits excellent bifunctional catalytic performance for both oxygen reduction reaction (ORR) and oxygen evolution reaction (OER), attributing to the abundant dual catalytic FeN3-CoN3 sites which are mutually beneficial for attaining optimal electronic properties for the adsorption/desorption of reaction intermediates. The assembled liquid-electrolyte ZAB provides a high specific power of 201.7 mW cm−2 and excellent cycling stability. More importantly, due to the good mechanical strength and flexibility of Fe1Co1-CNF, portable ZAB with exceptional shape deformability and stability can be demonstrated, in which Fe1Co1-CNF utility as an integrated free-standing membrane electrode. These findings provide a facile strategy for manufacturing flexible multi-functional catalytic electrodes with high production.
[Display omitted]
•Large-area self-standing flexible CNF film with diatomic Fe-Co sites was developed.•The diatomic Fe-Co sites render optimized adsorption of O-containing intermediates.•The Fe1Co1-CNF exhibits superior bifunctional ORR/OER performance.•The Fe1Co1-CNF shows great potential in liquid/flexible Zn-air battery. |
| ArticleNumber | 106147 |
| Author | Silva, S. Ravi P. Zhang, Peng Li, Zongge Yan, Zifeng Cai, Qiong Liu, Jian Zhang, Ying Sun, Xiaoming Wang, Yiyan Pan, Yuan Zhang, Guoxin |
| Author_xml | – sequence: 1 givenname: Yiyan surname: Wang fullname: Wang, Yiyan organization: State Key Laboratory of Heavy Oil Processing, China University of Petroleum (East China), Qingdao, Shandong 266580, PR China – sequence: 2 givenname: Zongge surname: Li fullname: Li, Zongge organization: State Key Laboratory of Heavy Oil Processing, China University of Petroleum (East China), Qingdao, Shandong 266580, PR China – sequence: 3 givenname: Peng surname: Zhang fullname: Zhang, Peng organization: State Key Laboratory of Heavy Oil Processing, China University of Petroleum (East China), Qingdao, Shandong 266580, PR China – sequence: 4 givenname: Yuan surname: Pan fullname: Pan, Yuan organization: State Key Laboratory of Heavy Oil Processing, China University of Petroleum (East China), Qingdao, Shandong 266580, PR China – sequence: 5 givenname: Ying surname: Zhang fullname: Zhang, Ying organization: State Key Laboratory of Heavy Oil Processing, China University of Petroleum (East China), Qingdao, Shandong 266580, PR China – sequence: 6 givenname: Qiong surname: Cai fullname: Cai, Qiong organization: DICP-Surrey Joint Centre for Future Materials, Department of Chemical and Process Engineering, and Advanced Technology Institute, University of Surrey, Guilford, Surrey GU2 7XH, UK – sequence: 7 givenname: S. Ravi P. surname: Silva fullname: Silva, S. Ravi P. organization: DICP-Surrey Joint Centre for Future Materials, Department of Chemical and Process Engineering, and Advanced Technology Institute, University of Surrey, Guilford, Surrey GU2 7XH, UK – sequence: 8 givenname: Jian surname: Liu fullname: Liu, Jian email: jian.liu@surrey.ac.uk organization: DICP-Surrey Joint Centre for Future Materials, Department of Chemical and Process Engineering, and Advanced Technology Institute, University of Surrey, Guilford, Surrey GU2 7XH, UK – sequence: 9 givenname: Guoxin surname: Zhang fullname: Zhang, Guoxin email: zhanggx@sdust.edu.cn organization: Department of Electrical Engineering and Automation, Shandong University of Science and Technology, Qingdao, Shandong 266590, PR China – sequence: 10 givenname: Xiaoming surname: Sun fullname: Sun, Xiaoming organization: State Key Laboratory of Heavy Oil Processing, China University of Petroleum (East China), Qingdao, Shandong 266580, PR China – sequence: 11 givenname: Zifeng surname: Yan fullname: Yan, Zifeng email: zfyancat@upc.edu.cn organization: State Key Laboratory of Heavy Oil Processing, China University of Petroleum (East China), Qingdao, Shandong 266580, PR China |
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| Keywords | Carbon nanofiber Electrospinning Bifunctional electro-catalyst Zn-air battery Dual-site catalyst |
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| Title | Flexible carbon nanofiber film with diatomic Fe-Co sites for efficient oxygen reduction and evolution reactions in wearable zinc-air batteries |
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