Dually charged polyamide nanofiltration membranes fabricated by microwave-assisted grafting for heavy metals removal

Heavy metals pollution is an urgent problem that seriously hazards human health and ecosystems. Herein, dually charged nanofiltration (NF) membranes were prepared via a facile modification with diethylenetriamine (DETA) after interfacial polymerization. More amine groups were imported after grafting...

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Published inJournal of membrane science Vol. 640; p. 119834
Main Authors Huang, Ben-Qing, Tang, Yong-Jian, Gao, An-Ran, Zeng, Zuo-Xiang, Xue, Shuang-Mei, Ji, Chen-Hao, Tang, Chuyang Y., Xu, Zhen-Liang
Format Journal Article
LanguageEnglish
Published Elsevier B.V 15.12.2021
Subjects
Dually charged
Grafting
Heavy metals
Nanofiltration
Nanofiltration
Dually charged
Grafting
Heavy metals
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Abstract Heavy metals pollution is an urgent problem that seriously hazards human health and ecosystems. Herein, dually charged nanofiltration (NF) membranes were prepared via a facile modification with diethylenetriamine (DETA) after interfacial polymerization. More amine groups were imported after grafting and a polyamide layer with opposite charges was constructed. The as-prepared membranes had a pure water permeability of 17.0 L m−2 h−1 bar−1 and maintained ideal rejection for both Na2SO4 (98.2%) and MgCl2 (94.1%), illustrating dually charged property. In addition, the dually charged NF membranes had high rejection to a series of heavy metals, showing good application potential in heavy metals removal. [Display omitted] •The dually charged NF membranes were fabricated by microwave-assisted grafting of diethylenetriamine after interfacial polymerization.•The as-prepared membrane showed a PWP of 17.0 L m−2 h−1 bar−1 and high rejection to both Na2SO4 (98.2%) and MgCl2 (94.1%)。•The dually charged NF membranes had high rejection to a series of heavy metals, showing good application potential in heavy metals removal.
AbstractList Heavy metals pollution is an urgent problem that seriously hazards human health and ecosystems. Herein, dually charged nanofiltration (NF) membranes were prepared via a facile modification with diethylenetriamine (DETA) after interfacial polymerization. More amine groups were imported after grafting and a polyamide layer with opposite charges was constructed. The as-prepared membranes had a pure water permeability of 17.0 L m−2 h−1 bar−1 and maintained ideal rejection for both Na2SO4 (98.2%) and MgCl2 (94.1%), illustrating dually charged property. In addition, the dually charged NF membranes had high rejection to a series of heavy metals, showing good application potential in heavy metals removal. [Display omitted] •The dually charged NF membranes were fabricated by microwave-assisted grafting of diethylenetriamine after interfacial polymerization.•The as-prepared membrane showed a PWP of 17.0 L m−2 h−1 bar−1 and high rejection to both Na2SO4 (98.2%) and MgCl2 (94.1%)。•The dually charged NF membranes had high rejection to a series of heavy metals, showing good application potential in heavy metals removal.
ArticleNumber 119834
Author Ji, Chen-Hao
Huang, Ben-Qing
Xu, Zhen-Liang
Tang, Yong-Jian
Xue, Shuang-Mei
Tang, Chuyang Y.
Zeng, Zuo-Xiang
Gao, An-Ran
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  givenname: Yong-Jian
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  email: chemxuzl@ecust.edu.cn
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Snippet Heavy metals pollution is an urgent problem that seriously hazards human health and ecosystems. Herein, dually charged nanofiltration (NF) membranes were...
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StartPage 119834
SubjectTerms Dually charged
Grafting
Heavy metals
Nanofiltration
Title Dually charged polyamide nanofiltration membranes fabricated by microwave-assisted grafting for heavy metals removal
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