Achieving strength-ductility synergy in metallic glasses via electric current-enhanced structural fluctuations
•Electric currents endow Zr-based metallic glasses with an exceptional combination of ultra-high strength, considerable plasticity, and enhanced strain-hardening ability.•Electric currents construct a unique structural fluctuation featuring soft zones surrounded by hard zones.•Plausible mechanisms f...
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| Published in | International journal of plasticity Vol. 169; p. 103711 |
|---|---|
| Main Authors | , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
01.10.2023
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| Subjects | |
| Online Access | Get full text |
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| Abstract | •Electric currents endow Zr-based metallic glasses with an exceptional combination of ultra-high strength, considerable plasticity, and enhanced strain-hardening ability.•Electric currents construct a unique structural fluctuation featuring soft zones surrounded by hard zones.•Plausible mechanisms for such electric current-regulated plasticity in metallic glasses are proposed.
Structural applications of metallic glasses are limited by their room-temperature brittleness and strain-softening, associated with the extreme localization of plastic flow in shear bands. Herein, we alleviate this dilemma by the structural fluctuation induced by electric currents, achieving simultaneous improvement of strengths, compression plasticity, and strain hardening capacity. The electric current enhances the structural fluctuations at the atomic scale, introducing more soft zones while densifying their surroundings, which differs from previously reported rejuvenation strategies. This unique structural pattern featuring soft zones surrounded by hard zones leads to extensive sprouts and interactions of shear bands, capturing substantial atoms to participate in the deformation. The plausible mechanism behind the electric current-influenced dynamic evolution of amorphous clusters is proposed. Electric current introduces interatomic electrostatic forces between shell atoms of amorphous clusters through charge transfer. This force decreases the coordination of Zr- and Cu-centered clusters and increases the Al-centered icosahedra in the glassy matrix. Differential evolution of clusters under electric currents enhances atomic structural fluctuations and originates from the cohesion mechanism determined by electron distribution. These findings are suggestive of vanishing room-temperature brittleness and shed atomic-scale light on modulations of the structure and properties of metallic glasses by electric currents.
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| AbstractList | •Electric currents endow Zr-based metallic glasses with an exceptional combination of ultra-high strength, considerable plasticity, and enhanced strain-hardening ability.•Electric currents construct a unique structural fluctuation featuring soft zones surrounded by hard zones.•Plausible mechanisms for such electric current-regulated plasticity in metallic glasses are proposed.
Structural applications of metallic glasses are limited by their room-temperature brittleness and strain-softening, associated with the extreme localization of plastic flow in shear bands. Herein, we alleviate this dilemma by the structural fluctuation induced by electric currents, achieving simultaneous improvement of strengths, compression plasticity, and strain hardening capacity. The electric current enhances the structural fluctuations at the atomic scale, introducing more soft zones while densifying their surroundings, which differs from previously reported rejuvenation strategies. This unique structural pattern featuring soft zones surrounded by hard zones leads to extensive sprouts and interactions of shear bands, capturing substantial atoms to participate in the deformation. The plausible mechanism behind the electric current-influenced dynamic evolution of amorphous clusters is proposed. Electric current introduces interatomic electrostatic forces between shell atoms of amorphous clusters through charge transfer. This force decreases the coordination of Zr- and Cu-centered clusters and increases the Al-centered icosahedra in the glassy matrix. Differential evolution of clusters under electric currents enhances atomic structural fluctuations and originates from the cohesion mechanism determined by electron distribution. These findings are suggestive of vanishing room-temperature brittleness and shed atomic-scale light on modulations of the structure and properties of metallic glasses by electric currents.
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| ArticleNumber | 103711 |
| Author | Gong, Pan Peng, Zhen Ding, Huaping Jin, Junsong Zhang, Mao Xie, Guoqiang Bu, Hengtong Deng, Lei Yao, Ke-fu Wang, Xinyun Tang, Xuefeng Chen, Wen Schroers, Jan |
| Author_xml | – sequence: 1 givenname: Huaping orcidid: 0000-0003-2267-0227 surname: Ding fullname: Ding, Huaping organization: State Key Laboratory of Materials Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China – sequence: 2 givenname: Pan orcidid: 0000-0002-3833-8440 surname: Gong fullname: Gong, Pan email: pangong@hust.edu.cn organization: State Key Laboratory of Materials Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China – sequence: 3 givenname: Wen surname: Chen fullname: Chen, Wen organization: Department of Mechanical and Industrial Engineering, University of Massachusetts, Amherst, MA, 01003, United States – sequence: 4 givenname: Zhen surname: Peng fullname: Peng, Zhen organization: School of Materials Science and Engineering, Jiangsu University, Zhenjiang 212013, China – sequence: 5 givenname: Hengtong surname: Bu fullname: Bu, Hengtong organization: School of Materials Science and Engineering, Tsinghua University, Beijing 100084, China – sequence: 6 givenname: Mao surname: Zhang fullname: Zhang, Mao organization: State Key Laboratory of Materials Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China – sequence: 7 givenname: Xuefeng surname: Tang fullname: Tang, Xuefeng organization: State Key Laboratory of Materials Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China – sequence: 8 givenname: Junsong surname: Jin fullname: Jin, Junsong organization: State Key Laboratory of Materials Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China – sequence: 9 givenname: Lei surname: Deng fullname: Deng, Lei email: denglei@hust.edu.cn organization: State Key Laboratory of Materials Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China – sequence: 10 givenname: Guoqiang orcidid: 0000-0003-3396-7974 surname: Xie fullname: Xie, Guoqiang organization: School of Materials Science and Engineering, Harbin Institute of Technology, Shenzhen 518055, China – sequence: 11 givenname: Xinyun surname: Wang fullname: Wang, Xinyun email: wangxy_hust@hust.edu.cn organization: State Key Laboratory of Materials Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China – sequence: 12 givenname: Ke-fu surname: Yao fullname: Yao, Ke-fu organization: School of Materials Science and Engineering, Tsinghua University, Beijing 100084, China – sequence: 13 givenname: Jan surname: Schroers fullname: Schroers, Jan organization: Department of Mechanical Engineering and Materials Science, Yale University, New Haven, CT 06511, United States |
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