A bifunctional ethylene-vinyl acetate copolymer protective layer for dendrites-free lithium metal anodes

Lithium metal batteries are strongly considered as one of the most promising candidates for next-generation high-performance battery systems. However, the uncontrollable growth of lithium dendrites and the highly reactive lithium metal result in the severe safety risks and the short lifespan for hig...

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Published inJournal of energy chemistry Vol. 48; pp. 203 - 207
Main Authors Liang, Yeru, Xiao, Ye, Yan, Chong, Xu, Rui, Ding, Jun-Fan, Liang, Ji, Peng, Hong-Jie, Yuan, Hong, Huang, Jia-Qi
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.09.2020
Subjects
Air-stable and anti-water
Bifunctional copolymer layer
Dendrites-free
Lithium metal anode
Solid electrolyte interphase (SEI)
Air-stable and anti-water
Bifunctional copolymer layer
Dendrites-free
Solid electrolyte interphase (SEI)
Lithium metal anode
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Abstract Lithium metal batteries are strongly considered as one of the most promising candidates for next-generation high-performance battery systems. However, the uncontrollable growth of lithium dendrites and the highly reactive lithium metal result in the severe safety risks and the short lifespan for high-energy-density rechargeable batteries. Here, we demonstrate a hydrophobic and ionically conductive ethylene-vinyl acetate (EVA) copolymer layer can not only endow lithium metal anodes with an air-stable and anti-water surface, but also efficiently suppress the lithium-dendrites growth during the electrochemical cycling process. Therefore, the introduction of the EVA copolymer as a bifunctional protection layer simultaneously improves the anti-water/air performance and electrochemical cycling stability of lithium metal anode. Hydrophobic and ionically conductive ethylene-vinyl acetate copolymer is proposed as a bifunctional protection layer to fabricate stable and dendrites-free lithium metal anodes. [Display omitted]
AbstractList Lithium metal batteries are strongly considered as one of the most promising candidates for next-generation high-performance battery systems. However, the uncontrollable growth of lithium dendrites and the highly reactive lithium metal result in the severe safety risks and the short lifespan for high-energy-density rechargeable batteries. Here, we demonstrate a hydrophobic and ionically conductive ethylene-vinyl acetate (EVA) copolymer layer can not only endow lithium metal anodes with an air-stable and anti-water surface, but also efficiently suppress the lithium-dendrites growth during the electrochemical cycling process. Therefore, the introduction of the EVA copolymer as a bifunctional protection layer simultaneously improves the anti-water/air performance and electrochemical cycling stability of lithium metal anode. Hydrophobic and ionically conductive ethylene-vinyl acetate copolymer is proposed as a bifunctional protection layer to fabricate stable and dendrites-free lithium metal anodes. [Display omitted]
Author Xu, Rui
Xiao, Ye
Yuan, Hong
Liang, Yeru
Ding, Jun-Fan
Huang, Jia-Qi
Liang, Ji
Peng, Hong-Jie
Yan, Chong
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  surname: Liang
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  organization: College of Materials and Energy, South China Agricultural University, Guangzhou 510642, Guangdong, China
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  fullname: Xiao, Ye
  organization: School of Materials Science and Engineering, Beijing Institute of Technology, Beijing 100081, China
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  fullname: Yan, Chong
  organization: School of Materials Science and Engineering, Beijing Institute of Technology, Beijing 100081, China
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  organization: Institute for Superconducting & Electronic Materials, Australian Institute of Innovative Materials, University of Wollongong, North Wollongong, NSW 2500, Australia
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  givenname: Hong-Jie
  surname: Peng
  fullname: Peng, Hong-Jie
  organization: Department of Chemical Engineering, Stanford University, Stanford, California, 94305, United States
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  orcidid: 0000-0001-7394-9186
  surname: Huang
  fullname: Huang, Jia-Qi
  email: jqhuang@bit.edu.cn
  organization: School of Materials Science and Engineering, Beijing Institute of Technology, Beijing 100081, China
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Keywords Air-stable and anti-water
Bifunctional copolymer layer
Dendrites-free
Solid electrolyte interphase (SEI)
Lithium metal anode
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Snippet Lithium metal batteries are strongly considered as one of the most promising candidates for next-generation high-performance battery systems. However, the...
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Publisher
StartPage 203
SubjectTerms Air-stable and anti-water
Bifunctional copolymer layer
Dendrites-free
Lithium metal anode
Solid electrolyte interphase (SEI)
Title A bifunctional ethylene-vinyl acetate copolymer protective layer for dendrites-free lithium metal anodes
URI https://dx.doi.org/10.1016/j.jechem.2020.01.027
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