Access to advanced sodium-ion batteries by presodiation: Principles and applications

Feasible presodiation is indispensable in improving the energy density, lifespan and rate performance of sodium ion batteries. In this contribution, the fundamentals and advancements of presodiation methodology are comprehensively interpreted, encompassing the properties, underlying principles, asso...

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Published inJournal of energy chemistry Vol. 92; pp. 162 - 175
Main Authors Zhang, Shihao, Cao, Ruoyu, Pu, Xiangjun, Zhao, Along, Chen, Weihua, Song, Chunhua, Fang, Yongjin, Cao, Yuliang
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.05.2024
Subjects
High reversible capacity
Increased coulombic efficiency
Presodiation
Sodium ion batteries
Increased coulombic efficiency
Sodium ion batteries
High reversible capacity
Presodiation
Online AccessGet full text
ISSN2095-4956
DOI10.1016/j.jechem.2024.01.029

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Abstract Feasible presodiation is indispensable in improving the energy density, lifespan and rate performance of sodium ion batteries. In this contribution, the fundamentals and advancements of presodiation methodology are comprehensively interpreted, encompassing the properties, underlying principles, associated approaches, and corresponding optimizations to present technological inferiorities. [Display omitted] Sodium-ion batteries (SIBs) are expected to offer affordability and high energy density for large-scale energy storage system. However, the commercial application of SIBs is hurdled by low initial coulombic efficiency (ICE), continuous Na loss during long-term operation, and low sodium-content of cathode materials. In this scenario, presodiation strategy by introducing an external sodium reservoir has been rationally proposed, which could supplement additional sodium ions into the system and thereby markedly improve both the cycling performance and energy density of SIBs. In this review, the significance of presodiation is initially introduced, followed by comprehensive interpretation on technological properties, underlying principles, and associated approaches, as well as our perspectives on present inferiorities and future research directions. Overall, this contribution outlines a distinct pathway towards the presodiation methodology, of significance but still in its nascent phase, which may inspire the targeted guidelines to explore new chemistry in this field.
AbstractList Feasible presodiation is indispensable in improving the energy density, lifespan and rate performance of sodium ion batteries. In this contribution, the fundamentals and advancements of presodiation methodology are comprehensively interpreted, encompassing the properties, underlying principles, associated approaches, and corresponding optimizations to present technological inferiorities. [Display omitted] Sodium-ion batteries (SIBs) are expected to offer affordability and high energy density for large-scale energy storage system. However, the commercial application of SIBs is hurdled by low initial coulombic efficiency (ICE), continuous Na loss during long-term operation, and low sodium-content of cathode materials. In this scenario, presodiation strategy by introducing an external sodium reservoir has been rationally proposed, which could supplement additional sodium ions into the system and thereby markedly improve both the cycling performance and energy density of SIBs. In this review, the significance of presodiation is initially introduced, followed by comprehensive interpretation on technological properties, underlying principles, and associated approaches, as well as our perspectives on present inferiorities and future research directions. Overall, this contribution outlines a distinct pathway towards the presodiation methodology, of significance but still in its nascent phase, which may inspire the targeted guidelines to explore new chemistry in this field.
Author Zhang, Shihao
Pu, Xiangjun
Chen, Weihua
Cao, Ruoyu
Song, Chunhua
Cao, Yuliang
Fang, Yongjin
Zhao, Along
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  organization: College of Chemistry and Molecular Sciences, Hubei Key Laboratory of Electrochemical Power Sources, Wuhan University, Wuhan 430072, Hubei, China
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Keywords Increased coulombic efficiency
Sodium ion batteries
High reversible capacity
Presodiation
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Snippet Feasible presodiation is indispensable in improving the energy density, lifespan and rate performance of sodium ion batteries. In this contribution, the...
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SubjectTerms High reversible capacity
Increased coulombic efficiency
Presodiation
Sodium ion batteries
Title Access to advanced sodium-ion batteries by presodiation: Principles and applications
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