Construction of multi-dimensional NiCo/C/CNT/rGO aerogel by MOF derivative for efficient microwave absorption
The development of high-performance microwave absorption materials is currently imperative in order to solve the problem of electromagnetic pollution. Herein, we successfully obtained a multi-dimensional graphene-based aerogel (NiCo/C/CNT/rGO aerogel) decorated with one-dimensional carbon nanotubes...
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| Published in | Carbon (New York) Vol. 205; pp. 411 - 421 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
05.03.2023
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The development of high-performance microwave absorption materials is currently imperative in order to solve the problem of electromagnetic pollution. Herein, we successfully obtained a multi-dimensional graphene-based aerogel (NiCo/C/CNT/rGO aerogel) decorated with one-dimensional carbon nanotubes (CNTs) and metal-organic framework (MOF) derivatives. The introduction of rGO aerogel significantly modifies the phase composition (NiCo/C/CNT and rGO) and hierarchical structure (1D CNT, 3D NiCo/C/CNT and rGO aerogel) of the composite, resulting in a multi-dimensional gradient, defects, heterogeneous interfaces, and superior microwave absorption properties. The optimum electromagnetic wave absorption performance of −58.8 dB is achieved at a filler loading of 20 wt%, with a thickness of 1.8 mm and an effective absorption bandwidth of 7.6 GHz, covering the entire Ku-band. The excellent electromagnetic wave absorption performance can be attributed to the synergistic effect of impedance matching, electromagnetic attenuation capability, unique multi-dimensional porous structure, abundant defects and interfaces. In summary, the present work provides a novel approach for the synthesis of multi-dimensional lightweight magnetic/dielectric microwave absorbers.
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| AbstractList | The development of high-performance microwave absorption materials is currently imperative in order to solve the problem of electromagnetic pollution. Herein, we successfully obtained a multi-dimensional graphene-based aerogel (NiCo/C/CNT/rGO aerogel) decorated with one-dimensional carbon nanotubes (CNTs) and metal-organic framework (MOF) derivatives. The introduction of rGO aerogel significantly modifies the phase composition (NiCo/C/CNT and rGO) and hierarchical structure (1D CNT, 3D NiCo/C/CNT and rGO aerogel) of the composite, resulting in a multi-dimensional gradient, defects, heterogeneous interfaces, and superior microwave absorption properties. The optimum electromagnetic wave absorption performance of −58.8 dB is achieved at a filler loading of 20 wt%, with a thickness of 1.8 mm and an effective absorption bandwidth of 7.6 GHz, covering the entire Ku-band. The excellent electromagnetic wave absorption performance can be attributed to the synergistic effect of impedance matching, electromagnetic attenuation capability, unique multi-dimensional porous structure, abundant defects and interfaces. In summary, the present work provides a novel approach for the synthesis of multi-dimensional lightweight magnetic/dielectric microwave absorbers.
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| Author | Cheng, Runrun Li, Yongfei Lu, Zhao Wang, Nian Yang, Longqi Wang, Yan |
| Author_xml | – sequence: 1 givenname: Longqi surname: Yang fullname: Yang, Longqi – sequence: 2 givenname: Yan orcidid: 0000-0001-5231-275X surname: Wang fullname: Wang, Yan email: wangyan287580632@126.com – sequence: 3 givenname: Zhao surname: Lu fullname: Lu, Zhao – sequence: 4 givenname: Runrun surname: Cheng fullname: Cheng, Runrun – sequence: 5 givenname: Nian surname: Wang fullname: Wang, Nian – sequence: 6 givenname: Yongfei surname: Li fullname: Li, Yongfei |
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