The photocatalytic H2O2 production by metal-free photocatalysts under visible-light irradiation
The photocatalytic H2O2 production from H2O and O2 over organic polymers is a promising approach to achieve solar-to-chemical energy conversion. The continuous efforts have led to rapid development of various metal-free-based photocatalysts for specific H2O2 production, but generalizations and summa...
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| Published in | Applied catalysis. B, Environmental Vol. 341; p. 123271 |
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| Main Authors | , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.02.2024
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The photocatalytic H2O2 production from H2O and O2 over organic polymers is a promising approach to achieve solar-to-chemical energy conversion. The continuous efforts have led to rapid development of various metal-free-based photocatalysts for specific H2O2 production, but generalizations and summarization are obviously inadequate. This review mainly focuses on the state-of-the-art development process of metal-free-based photocatalysts for photocatalytic H2O2 production via combining O2 reduction and H2O oxidation reactions under visible light irradiation. The representative research work on photocatalytic H2O2 production by various metal-free-based photocatalytic systems, including graphite carbon nitride (g-C3N4), covalent organic frameworks (COFs), covalent triazine frameworks (CTFs) and covalent organic polymers (COPs) was highlighted. The strategies for structure and property optimization of metal-free-based photocatalysts at molecular-level have been proposed for improving the photocatalytic performance. The challenges and future directions have also been provided to guide the design and synthesis of metal-free-based photocatalytic system.
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•The state-of-the-art development of photocatalytic H2O2 production by metal-free photocatalysts was summarized.•Successful strategies to maximize the catalytic performance were assessed.•Representative research works on photocatalytic H2O2 production was highlighted.•Challenges and future directions discussed in the end. |
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| AbstractList | The photocatalytic H2O2 production from H2O and O2 over organic polymers is a promising approach to achieve solar-to-chemical energy conversion. The continuous efforts have led to rapid development of various metal-free-based photocatalysts for specific H2O2 production, but generalizations and summarization are obviously inadequate. This review mainly focuses on the state-of-the-art development process of metal-free-based photocatalysts for photocatalytic H2O2 production via combining O2 reduction and H2O oxidation reactions under visible light irradiation. The representative research work on photocatalytic H2O2 production by various metal-free-based photocatalytic systems, including graphite carbon nitride (g-C3N4), covalent organic frameworks (COFs), covalent triazine frameworks (CTFs) and covalent organic polymers (COPs) was highlighted. The strategies for structure and property optimization of metal-free-based photocatalysts at molecular-level have been proposed for improving the photocatalytic performance. The challenges and future directions have also been provided to guide the design and synthesis of metal-free-based photocatalytic system.
[Display omitted]
•The state-of-the-art development of photocatalytic H2O2 production by metal-free photocatalysts was summarized.•Successful strategies to maximize the catalytic performance were assessed.•Representative research works on photocatalytic H2O2 production was highlighted.•Challenges and future directions discussed in the end. |
| ArticleNumber | 123271 |
| Author | Wu, Wenxin Sui, Yan Li, Xiaodan Zhong, Hong Wen, Meicheng Xu, Xiahong Chen, Wentong Liu, Dongsheng Li, Yuntong Huang, Wei Gao, Shuang Pan, Changwang Wen, He-Rui |
| Author_xml | – sequence: 1 givenname: Xiahong surname: Xu fullname: Xu, Xiahong organization: Key Laboratory of Coordination Chemistry of Jiangxi Province, School of Chemistry and Chemical Engineering, Jinggangshan University, Ji’an, Jiangxi 343009, China – sequence: 2 givenname: Yan surname: Sui fullname: Sui, Yan organization: Key Laboratory of Coordination Chemistry of Jiangxi Province, School of Chemistry and Chemical Engineering, Jinggangshan University, Ji’an, Jiangxi 343009, China – sequence: 3 givenname: Wentong surname: Chen fullname: Chen, Wentong organization: Key Laboratory of Coordination Chemistry of Jiangxi Province, School of Chemistry and Chemical Engineering, Jinggangshan University, Ji’an, Jiangxi 343009, China – sequence: 4 givenname: Wei surname: Huang fullname: Huang, Wei organization: Key Laboratory of Coordination Chemistry of Jiangxi Province, School of Chemistry and Chemical Engineering, Jinggangshan University, Ji’an, Jiangxi 343009, China – sequence: 5 givenname: Xiaodan surname: Li fullname: Li, Xiaodan organization: Key Laboratory of Coordination Chemistry of Jiangxi Province, School of Chemistry and Chemical Engineering, Jinggangshan University, Ji’an, Jiangxi 343009, China – sequence: 6 givenname: Yuntong surname: Li fullname: Li, Yuntong organization: Key Laboratory of Coordination Chemistry of Jiangxi Province, School of Chemistry and Chemical Engineering, Jinggangshan University, Ji’an, Jiangxi 343009, China – sequence: 7 givenname: Dongsheng surname: Liu fullname: Liu, Dongsheng organization: Key Laboratory of Coordination Chemistry of Jiangxi Province, School of Chemistry and Chemical Engineering, Jinggangshan University, Ji’an, Jiangxi 343009, China – sequence: 8 givenname: Shuang surname: Gao fullname: Gao, Shuang organization: Key Laboratory of Coordination Chemistry of Jiangxi Province, School of Chemistry and Chemical Engineering, Jinggangshan University, Ji’an, Jiangxi 343009, China – sequence: 9 givenname: Wenxin surname: Wu fullname: Wu, Wenxin organization: Key Laboratory of Coordination Chemistry of Jiangxi Province, School of Chemistry and Chemical Engineering, Jinggangshan University, Ji’an, Jiangxi 343009, China – sequence: 10 givenname: Changwang surname: Pan fullname: Pan, Changwang organization: Key Laboratory of Coordination Chemistry of Jiangxi Province, School of Chemistry and Chemical Engineering, Jinggangshan University, Ji’an, Jiangxi 343009, China – sequence: 11 givenname: Hong surname: Zhong fullname: Zhong, Hong email: zhonghbush@jgsu.edu.cn organization: Key Laboratory of Coordination Chemistry of Jiangxi Province, School of Chemistry and Chemical Engineering, Jinggangshan University, Ji’an, Jiangxi 343009, China – sequence: 12 givenname: He-Rui surname: Wen fullname: Wen, He-Rui organization: School of Chemistry and Chemical Engineering, Jiangxi University of Science and Technology, Ganzhou, Jiangxi 341000, China – sequence: 13 givenname: Meicheng orcidid: 0000-0002-7394-0592 surname: Wen fullname: Wen, Meicheng email: meicheng.wen@gdut.edu.ch organization: Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and Health, Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control, School of Environmental Science and Engineering, Institute of Environmental Health and Pollution Control, Guangdong University of Technology, Guangzhou 510006, China |
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| Keywords | Heterogeneous catalysis Visible light Hydrogen peroxide Metal-free photocatalysts Photocatalysis |
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| Title | The photocatalytic H2O2 production by metal-free photocatalysts under visible-light irradiation |
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